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AIP conference proceedings

On the measurement of forbidden 21S0 – 23S1 transition frequency in helium by the method of stimulated Raman scattering

P.V. Pokasov, А. В. Тайченачев, E. V. Baklanov

Published Jan 1, 2019• 0 citations
Publisher

Abstract

In this paper, the possibility of measuring the forbidden 21S0 – 23S1 transition frequency (1557 nm) of a helium atom by the method of stimulated Raman scattering through the intermediate 23P1 level is demonstrated. The transition is important for the spectroscopy of the helium atom because it relates the singlet and triplet parts of the spectrum.

DOI
10.1063/1.5098156

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Quantum Electronics•May 31, 1997•3 citations
In this paper, the possibility of measuring the forbidden 21S0 – 23S1 transition frequency (1557 nm) of a helium atom by the method of stimulated Raman scattering through the intermediate 23P1 level is demonstrated. The transition is important for the spectroscopy of the helium atom because it relates the singlet and triplet parts of the spectrum.
Resonant stimulated Raman scattering (SRS) on the 23S-11S forbidden transition of the helium atom (62.6 nm) through the intermediate 23P1 level is considered. The 23S metastable state has the lowest energy in the triplet part of the spectrum (He *), and the 11S state is the ground state. For the density matrix, shortened kinetic equations are derived, which are used to analyze the SRS resonance. Expressions for field broadening and resonance shift are obtained, Doppler broadening is taken into account, and numerical estimates are made.
Abstract The possibility of precision measurements of frequencies of forbidden transitions of cold atoms in a trap using stimulated Raman scattering is shown. Transition 1S–2S in a hydrogen atom, in which the atom passes from level 1S to level 2S via intermediate level 3P is considered in detail. In this case, the frequency of the pump field (103 nm) is close to the frequency of the 3P–1S transition, while the stimulated scattering frequency (656 nm) is close to the frequency of the 3P–2S transition.
Resonant stimulated Raman scattering (SRS) from the 23S−11S{{2}^{3}}S{-} {{1}^{1}}S23S−11S forbidden transition in a helium atom (62.6 nm) via the intermediate 23P1{{2}^{3}}{{P}_{1}}23P1​ level has been considered. The metastable 23S{{2}^{3}}S23S state has the lowest energy in the triplet spectral region (He*), and the ground state is 11S{{1}^{1}}S11S . The reduced kinetic equations for the density matrix, which are used to analyze the SRS resonance, have been derived. The expressions for the field broadening and resonance shift are obtained, the Doppler broadening is taken into account, and numerical estimations are performed.