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International Conference on Micro- and Nano-Electronics (ICMNE)

Homogeneous atomic ensembles and single-mode field: review of simulation results

Nikita A. Skovoroda, A. V. Kulagin, Vitalii Y. Ladunov, Nadezda B. Victorova, Yuri Ozhigov

Published Mar 15, 2019• 8 citations
Publisher

Abstract

We consider ensembles of two level atoms interacting with the field in one mode resonator; such ensembles are homogeneous, if the force of interaction is the same for all atoms. We represent the results of numerical simulation of the following effects: relaxation of atomic excitation for one atom, dephasing assisted transport of energy along the chain of optical cavities (DAT), optical conductivity of a network of cavities, quantum bottleneck, thermal attractors for two atomic systems and ensemble Rabi oscillation for a hundred of atoms and dark states. The last effect required the supercomputer simulation on Lomonosov-2. DAT and quantum bottleneck play the peculiar role in biology (FMO light harvesting complex in green sulfur bacteria), dark states are significant for quantum computations. This elucidates the special role of dark states in such ensembles and the power of finite dimension models of QED, which allow inclusion of dipole-dipole interaction and nonlinearity that makes such models very powerful.

DOI
10.1117/12.2521763

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We consider ensembles of two level atoms interacting with the field in one mode resonator; such ensembles are homogeneous, if the force of interaction is the same for all atoms. We represent the results of numerical simulation of the following effects: relaxation of atomic excitation for one atom, dephasing assisted transport of energy along the chain of optical cavities (DAT), optical conductivity of a network of cavities, quantum bottleneck, thermal attractors for two atomic systems and ensemble Rabi oscillation for a hundred of atoms and dark states. The last effect required the supercomputer simulation on Lomonosov-2. DAT and quantum bottleneck play the peculiar role in biology (FMO light harvesting complex in green sulfur bacteria), dark states are significant for quantum computations. This elucidates the special role of dark states in such ensembles and the power of finite dimension models of QED, which allow inclusion of dipole-dipole interaction and nonlinearity that makes such models very powerful.
Many effects in the interaction between atoms and a cavity that are usually de-scribed in quantum mechanical terms (cavity quantum electrodynamics, cavity QED) can be understood and quantitatively analyzed within a classical framework. We adopt such a classical picture of a radiating dipole oscillator to derive explicit ex- pressions for the coupling of single atoms and atomic ensembles to Gaussian modes in free space and in an optical resonator. The cooperativity parameter of cavity QED is shown to play a central role, and is given a geometrical interpretation. The classical analysis yields transparent, intuitive results that are useful for analyzing applications of cavity QED such as atom detection and counting, cavity cooling, cavity spin squeezing, cavity spin optomechanics, or phase transitions associated with the self-organization of the ensemble-light system.
An ensemble of identical two level atoms in dark state neither adsorbs nor emits photons due to destructive interference. Dark states have numerous applications. It can be used for the source of energy for nano-devices; the space of dark states is decoherence free and can serve as the carrier for the fault tolerant quantum computations, etc. Since a dark state does not interact with the electromagnetic field it is an eigenstate of Tavis-Cummings Hamiltonian and the preparation of such states requires the exit from this model. We show how to prepare a dark state by the photon pumping and drain from the optical cavity with two atoms, one from which has Stark or Zeeman splitting of energy levels. This splitting is removed before photon drain from the cavity. The dark state yield after one such cycle has the order of energy level splitting. We show the scheme of the experiment, in which such cycles repeat until the dark state is produced with high probability and the results of its computer simulation. The structure of dark states is briefly discussed.
We have investigated nonlinear atom optical effects which arise from atom-atom collisional interactions in a single-mode atomic Fabry-Perot cavity driven by a coherent cw atom laser beam. When the nonlinear interaction energy per single atom is small, the exact numerical solution of the master equation is well reproduced by a mean-field treatment in which quantum fluctuations are included linearizing the stochastic equations of the Positive-P representation. On the other hand, when the damping of the cavity mode is very weak and its wave-function is tightly confined in space, a regime of strong nonlinearity can be achieved. For the specific case of an incident atom laser frequency at resonance with the empty cavity, the numerical calculations predict a sort of atom blockade effect, which is a sort of atom optical analog of the well-known Coulomb blockade effect of electronic transport through microscopic structures: only one atom can occupy the cavity mode at a time and the statistical properties of the transmitted beam, being very similar to the resonance fluorescence from a single two-level system, show definitely nonclassical behaviors such as antibunching. Only at very large incident intensities, more than one atom can be simultaneously forced inside the cavity mode: in this regime, the results of the numerical calculations can be successfully interpreted using a dressed cavity model. From the formal analogy between atomic matter waves and optical light waves in nonlinear media, it follows that the same results hold for photonic systems.
The dynamics of an ensemble of two-level atoms moving through a single-mode lossless cavity is investigated in the semiclassical and rotating-wave approximations. The dynamical system for the expectation values of the atomic and field observables is considered as a perturbation to one of the following integrable versions: (i) a model with atoms moving through a spatially inhomogeneous resonant field, and (ii) a model with atoms interacting with a nonresonant eigenmode which is assumed to be homogeneous on the cavity size. We find the general exact solutions for both the models and show that they contain special solutions describing a coherent effect of population and radiation trapping. Using the Melnikov method, we prove analytically transverse intersections of stable and unstable manifolds of a hyperbolic fixed point under a small modulation of the vacuum Rabi frequency. These intersections are believed to provide the Smale horseshoe mechanism of Hamiltonian chaos. The analytical results are accompanied with direct computation of topographical maps of maximal Lyapunov exponents that give a representative image of regularity and chaos in the atom-field system in different ranges of its control parameters--the frequency detuning, the number, and the velocity of atoms.
The Rabi Hamiltonian, describing the interaction between a two-level atomic system and a single-cavity mode of the electromagnetic field, is one of the fundamental models in quantum optics. The model becomes exactly solvable by considering an atom without permanent dipole moments, whose excitation energy is quasiresonant with the cavity photon energy, and by neglecting the nonresonant (counter-rotating) terms. In this case, after including the decay of either the atom or the cavity mode to a continuum, one can derive the well-known phenomenology of quasiresonant transitions, including the fluorescence triplets. In this work we consider the most general Rabi model, incorporating the effects of permanent atomic electric dipole moments. Based on a perturbative analysis, we compare the intensities of emission lines induced by rotating terms, counter-rotating terms, and parity-symmetry-breaking terms in order to identify the parameter regimes in which these different contributions play a significant role. The analysis reveals that the emission strength related to the existence of permanent dipoles may surpass the one due to the counter-rotating interaction terms but is usually much weaker than the emission due to the main, resonant coupling. This ratio can be modified in systems with a reduced dimensionality or by engineering the energy spectral density of the continuum.
One of the simplest nontrivial problems involving the atom–field interaction is the coupling of a two-level atom with a single mode of the electromagnetic field. A two-level atom description is valid if the two atomic levels involved are resonant or nearly resonant with the driving field, while all other levels are highly detuned. Under certain realistic approximations, it is possible to reduce this problem to a form which can be solved exactly; allowing essential features of the atom-field interaction to be extracted. In this chapter we present a semiclassical theory of the interaction of a single two-level atom with a single mode of the field in which the atom is treated as a quantum two-level system and the field is treated classically. A fully quantum mechanical theory will be presented in Chapter 6. A two-level atom is formally analogous to a spin-1/2 system with two possible states. In the dipole approximation, when the field wavelength is larger than the atomic size, the atom–field interaction problem is mathematically equivalent to a spin-1/2 particle interacting with a time-dependent magnetic field. Just as the spin-1/2 system undergoes the so-called Rabi oscillations between the spin-up and spin-down states under the action of an oscillating magnetic field, the two-level atom also undergoes optical Rabi oscillations under the action of the driving electromagnetic field. These oscillations are damped if the atomic levels decay. An understanding of this simple model of the atom–field interaction enables us to consider more complicated problems involving an ensemble of atoms interacting with the field.