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Cambridge University Press eBooks

Atom–field interaction – semiclassical theory

Marlan O. Scully, Muhammad Suhail Zubairy

Published Sep 4, 1997• 5 citations
Publisher

Abstract

One of the simplest nontrivial problems involving the atom–field interaction is the coupling of a two-level atom with a single mode of the electromagnetic field. A two-level atom description is valid if the two atomic levels involved are resonant or nearly resonant with the driving field, while all other levels are highly detuned. Under certain realistic approximations, it is possible to reduce this problem to a form which can be solved exactly; allowing essential features of the atom-field interaction to be extracted. In this chapter we present a semiclassical theory of the interaction of a single two-level atom with a single mode of the field in which the atom is treated as a quantum two-level system and the field is treated classically. A fully quantum mechanical theory will be presented in Chapter 6. A two-level atom is formally analogous to a spin-1/2 system with two possible states. In the dipole approximation, when the field wavelength is larger than the atomic size, the atom–field interaction problem is mathematically equivalent to a spin-1/2 particle interacting with a time-dependent magnetic field. Just as the spin-1/2 system undergoes the so-called Rabi oscillations between the spin-up and spin-down states under the action of an oscillating magnetic field, the two-level atom also undergoes optical Rabi oscillations under the action of the driving electromagnetic field. These oscillations are damped if the atomic levels decay. An understanding of this simple model of the atom–field interaction enables us to consider more complicated problems involving an ensemble of atoms interacting with the field.

DOI
10.1017/cbo9780511813993.007

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One of the simplest nontrivial problems involving the atom–field interaction is the coupling of a two-level atom with a single mode of the electromagnetic field. A two-level atom description is valid if the two atomic levels involved are resonant or nearly resonant with the driving field, while all other levels are highly detuned. Under certain realistic approximations, it is possible to reduce this problem to a form which can be solved exactly; allowing essential features of the atom-field interaction to be extracted. In this chapter we present a semiclassical theory of the interaction of a single two-level atom with a single mode of the field in which the atom is treated as a quantum two-level system and the field is treated classically. A fully quantum mechanical theory will be presented in Chapter 6. A two-level atom is formally analogous to a spin-1/2 system with two possible states. In the dipole approximation, when the field wavelength is larger than the atomic size, the atom–field interaction problem is mathematically equivalent to a spin-1/2 particle interacting with a time-dependent magnetic field. Just as the spin-1/2 system undergoes the so-called Rabi oscillations between the spin-up and spin-down states under the action of an oscillating magnetic field, the two-level atom also undergoes optical Rabi oscillations under the action of the driving electromagnetic field. These oscillations are damped if the atomic levels decay. An understanding of this simple model of the atom–field interaction enables us to consider more complicated problems involving an ensemble of atoms interacting with the field.
In the preceding chapters concerning the interaction of a radiation field with matter, we assumed the field to be classical. In many situations this assumption is valid. There are, however, many instances where a classical field fails to explain experimentally observed results and a quantized description of the field is required. This is, for example, true of spontaneous emission in an atomic system which was described phenomenologically in Chapter 5. For a rigorous treatment of the atomic level decay in free space, we need to consider the interaction of the atom with the vacuum modes of the universe. Even in the simplest system involving the interaction of a single-mode radiation field with a single two-level atom, the predictions for the dynamics of the atom are quite different in the semiclassical theory and the fully quantum theory. In the absence of the decay process, the semiclassical theory predicts Rabi oscillations for the atomic inversion whereas the quantum theory predicts certain collapse and revival phenomena due to the quantum aspects of the field. These interesting quantum field theoretical predictions have been experimentally verified. In this chapter we discuss the interaction of the quantized radiation field with the two-level atomic system described by a Hamiltonian in the dipole and the rotating-wave approximations. For a single-mode field it reduces to a particularly simple form. This is a very interesting Hamiltonian in quantum optics for several reasons. First, it can be solved exactly for arbitrary coupling constants and exhibits some true quantum dynamical effects such as collapse followed by periodic revivals of the atomic inversion.
Abstract This chapter presents some of the models describing the time-dependent interaction between a simple atom and a field, which may be described either classically or fully quantum mechanically. A number of equivalent interaction pictures and the important rotating-wave approximation are introduced. The two-state dynamics of an atom coupled to a classical field is solved, starting with perturbation theory. Non-perturbative behaviour is analysed, leading to Rabi oscillations of the atomic probabilities. The Jaynes–Cummings model of the dynamics of a single two-state atom coupled to a single quantized mode of the electromagnetic field is solved leading to collapses and revivals of the excited state probability. An exactly soluble model of the coupling of a single state to a Bixon–Jortner quasi-continuum of discrete levels is analysed. Finally, the coherent interactions between two field modes, of the type common in nonlinear optics, are discussed.
One of the simplest models involving the atom-field interaction is the coupling of a single two-level atom with single-mode optical field. Under the rotating wave approximation, this problem is reduced to a form that can be solved exactly. But the approximation is only valid when the two levels are resonant or nearly resonant with the applied electromagnetic radiation. Here we present an analytical solution without the rotating wave approximation and applicable to general atom-field interaction far away from the resonance. We find that there exists remarkable influence of the initial phase of optical field on the Rabi oscillations and Rabi splitting, and this issue cannot be explored in the context of the rotating wave approximation. Due to the retention of the counter-rotating terms, higher-order harmonic appears during the Rabi splitting. The analytical solution suggests a way to regulate and control the quantum dynamics of a two-level atom and allows for exploring more essential features of the atom-field interaction.
The interaction of electromagnetic fields with atomic/molecular systems is the genesis of most optical phenomena observed to date. To explain these effects, we need two broad classifications based on both classical and quantum theories. This strategy involves treating (1) fields as classical systems and atoms as quantum systems having discrete energy, (2) fields as quantum systems (particles rather than waves) and atomic systems as classical, or (3) both as quantum systems. Of course, schemes 1 and 2 are easy to solve and visualize, while scheme 3 is the most accurate description but complex in nature. In general, quantum approaches do not lead to exact solutions and require assumptions and simplifications to achieve a reasonably approximate solution. Thus, it is important to choose an appropriate strategy for solving a particular problem. The problem associated with atom–field interactions will also be subjected to different strategies to understand some of the experimentally observed phenomena such as Rabi oscillations. In this chapter, we will derive a master equation that serves as the starting point for solving a large number of problems associated with atom–field interactions.
We considered the semiclassical Rabi model: a two-level atom fixed at a position and interacting with a classical, monochromatic electromagnetic field. In resonance and for an arbitrary initial state of the system, we obtained an approximate, analytic solution that takes into account the counterrotating terms and that is accurate as long as the Rabi frequency is smaller than or equal to 1/21/21/2 (1/41/41/4) of the angular frequency of the field and 111 (101010) Rabi oscillations are considered. In addition, the approximate solution has the same level of complexity as that obtained with the rotating-wave-approximation (RWA) and the approximate solution also leads to a simple criterion that allows one to determine the accuracy of the solution in the RWA. We found that the approximate solution is composed of the the solution in the RWA plus terms that oscillate at the angular frequency of the field and at the Rabi frequency. Moreover, these corrections are proportional to the Rabi frequency divided by two times the angular frequency of the field.
We compare the semiclassical and quantum predictions for the unitary dynamics of a two-level atom interacting with a single-mode electromagnetic field under parametric modulation of the atomic parameters in the regime of multiphoton atom–field resonances. We derive approximate analytic solutions for the semiclassical Rabi model when the atomic transition frequency and the atom–field coupling strength undergo harmonic external modulations. These solutions are compared to the predictions of the quantum Rabi model, which we solve numerically for an initial coherent state with a large average photon number (on the order of 104), in the regime of three-photon resonance. We show that, for short enough times and sufficiently intense coherent states, the semiclassical dynamics agrees quite well with the quantum dynamics, although it inevitably fails at longer times due to the absence of collapse–revival behavior. Furthermore, we describe how the field state evolves throughout the interaction, presenting numerical results for the average photon number, entropies (related to atom–field entanglement), and other quantities characterizing the photon number statistics of the electromagnetic field.