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Chinese Physics B

Controllable photon echo phase induced by modulated pulses and chirped beat detection

Xian-Yang Zhang, Shuanggen Zhang, Huadi Zhang, Xiurong Ma

Published Feb 1, 2019• 1 citation
Publisher

Abstract

In this paper, we propose a scheme for photon echo chirped detection process composed of additional modulation pulses to obtain controllable geometric phase. The geometric phases are observed and measured by a beat signal between the photon echo field and the chirped field. The chirped detection model reveals that the period of the beat signal increases as the chirped rate and delay time increase. Additionally, a two-fold relationship between the modulation phase and the echo shift phase is obtained. The numerical simulations accord with the theoretical results obtained by the finite difference time domain (FDTD) method.

DOI
10.1088/1674-1056/28/2/024207

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In this paper, we propose a scheme for photon echo chirped detection process composed of additional modulation pulses to obtain controllable geometric phase. The geometric phases are observed and measured by a beat signal between the photon echo field and the chirped field. The chirped detection model reveals that the period of the beat signal increases as the chirped rate and delay time increase. Additionally, a two-fold relationship between the modulation phase and the echo shift phase is obtained. The numerical simulations accord with the theoretical results obtained by the finite difference time domain (FDTD) method.
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The role of weakly chirped pulses (time bandwidth product, DeltanuDeltatau<0.61) on three-pulse photon echo signals has been systematically studied. Pulses with varying chirp were characterized with frequency resolved optical gating (FROG) and used to measure spectrally resolved three-pulse photon echoes of a dye in solution. The weakly chirped pulses give rise to markedly different echo signals for population times below approximately 100 fs. The chirped pulses can decrease or enhance spectral signatures of an excited state absorption transition in the echo signal. Furthermore, the observed dephasing dynamics depend on the phase of the electric fields. Simulations based on a three-level model and the electric fields retrieved from the FROG traces give a good agreement for photon echo experiments with both transform limited and chirped pulses. The simulations also allow for a numerical investigation of effects of chirp in two-dimensional spectroscopy. For a two-level system, the chirped pulses result in nonelliptical two-dimensional spectra that can erroneously be interpreted as spectral heterogeneity with frequency dependent dephasing dynamics. Furthermore, chirped pulses can give rise to "false" cross peaks when strong vibrational modes are involved in the system-bath interaction.
We report on the dynamics of two-pulse photon echoes in a two-level system. We consider two different types of excitation pulse pairs: pulses with the same carrier envelope phases (CEP pulse pairs) and pulse pairs cut from the same carrier wave train (labeled as normal pulse pairs). We show that for CEP pulse pairs when the pulses overlap somewhat the photon-echo emission time is strongly sensitive to the relative phase (i.e., delay time) between the two pulses. We also show how the photon-echo emission time for such CEP pulse pairs depends on the dephasing time of the polarization (T2{T}_{2}T2​) and the pulse width of the applied pulses. This phase sensitivity can be utilized to control the emission time of the photon echo which may prove useful in storing and retrieving light signals from an atomic ensemble. Our results also inform the interpretation of photon-echo signals at short delay time when used to measure fast coherence decay rates.
We demonstrate coherent control over interference between different Liouville-space pathways that describe the generation of the nonlinear optical polarization in a stimulated photon echo. This control was exercised by phase-locking of the excitation pulses and observed in the heterodyne detected echo signal. A theoretical analysis of the effect is presented and found to be in good agreement with the obtained results. The relation between this novel time-domain interference effect and the pressure-induced extra resonance in four-wave mixing spectroscopy is discussed.
A new method for waveform measurement of photon echoes using a modified Michelson interferometer has been developed. The experimental setup uses collinear geometry, and photon echo signals are detected using a double-phase modulation technique. The amplitude and phase of photon echoes and those of excitation pulses are simultaneously measured by this technique. The method has been applied to a photon echo experiment on a dye solution. The results are explained using a stochastic modulation model with an accumulation effect of population grating.
It is predicted that linearly chirped optical excitation pulses give rise to photon echoes whose shortness is limited only by the total material bandwidth that contributes to the echo signal. The photon echo process acts as a frequency-dependent optical delay line whose dispersion is determined by the chirp rate of the excitation pulses rather than by their bandwidth. Consequently, long and short pulses can be compressed with equal facility without complicated alignment procedure. Accumulated echoes have similar properties and can be used with trains of weak excitation pulses.