J. D. Fletcher, Nathan Johnson, Elina Locane, Patrick See, Jonathan P. Griffiths, Ian A. Farrer, D. A. Ritchie, Piet W. Brouwer, Vyacheslavs Kashcheyevs, M. Kataoka
Initializing and measuring the wave-function of single freely-propagating particles are challenging but fundamental tasks for applications in quantum information processing and enhanced sensing. Recently, continuous-variable quantum tomography techniques developed for atomic beams and photonic modes have been adapted for on-demand electronic excitations but are limited to the region in energy-time phase space immediately around the Fermi level. Here we present a general, broad-band method for mapping the single-particle phase space Wigner distribution. We reconstruct the Wigner representation of the mixed-state density matrix for \textit{solitary} electrons emitted by an on-demand source. This reveals highly localised distributions isolated from the Fermi sea. Our method can be used to test the degree of `quantumness' of an electron source from measurements of the phase-space density. While both source purity and detector fidelity are suppressed by classical fluctuations, here we resolve fine structure of the wavepackets (a chirp controlled by emission conditions) and find that the resolution should be sufficient to enable quantum-limited measurements. Our technique will provide key information required to master electron coherence and entanglement at the individual particle level, for instance to create excitations from multiple sources that are indistinguishable.
Initializing and measuring the wave-function of single freely-propagating particles are challenging but fundamental tasks for applications in quantum information processing and enhanced sensing. Recently, continuous-variable quantum tomography techniques developed for atomic beams and photonic modes have been adapted for on-demand electronic excitations but are limited to the region in energy-time phase space immediately around the Fermi level. Here we present a general, broad-band method for mapping the single-particle phase space Wigner distribution. We reconstruct the Wigner representation of the mixed-state density matrix for \textit{solitary} electrons emitted by an on-demand source. This reveals highly localised distributions isolated from the Fermi sea. Our method can be used to test the degree of `quantumness' of an electron source from measurements of the phase-space density. While both source purity and detector fidelity are suppressed by classical fluctuations, here we resolve fine structure of the wavepackets (a chirp controlled by emission conditions) and find that the resolution should be sufficient to enable quantum-limited measurements. Our technique will provide key information required to master electron coherence and entanglement at the individual particle level, for instance to create excitations from multiple sources that are indistinguishable.
A method for characterising the wave-function of freely-propagating particles would provide a useful tool for developing quantum-information technologies with single electronic excitations. Previous continuous-variable quantum tomography techniques developed to analyse electronic excitations in the energy-time domain have been limited to energies close to the Fermi level. We show that a wide-band tomography of single-particle distributions is possible using energy-time filtering and that the Wigner representation of the mixed-state density matrix can be reconstructed for solitary electrons emitted by an on-demand single-electron source. These are highly localised distributions, isolated from the Fermi sea. While we cannot resolve the pure state Wigner function of our excitations due to classical fluctuations, we can partially resolve the chirp and squeezing of the Wigner function imposed by emission conditions and quantify the quantumness of the source. This tomography scheme, when implemented with sufficient experimental resolution, will enable quantum-limited measurements, providing information on electron coherence and entanglement at the individual particle level.
A method for characterising the wave-function of freely-propagating particles would provide a useful tool for developing quantum-information technologies with single electronic excitations. Previous continuous-variable quantum tomography techniques developed to analyse electronic excitations in the energy-time domain have been limited to energies close to the Fermi level. We show that a wide-band tomography of single-particle distributions is possible using energy-time filtering and that the Wigner representation of the mixed-state density matrix can be reconstructed for solitary electrons emitted by an on-demand single-electron source. These are highly localised distributions, isolated from the Fermi sea. While we cannot resolve the pure state Wigner function of our excitations due to classical fluctuations, we can partially resolve the chirp and squeezing of the Wigner function imposed by emission conditions and quantify the quantumness of the source. This tomography scheme, when implemented with sufficient experimental resolution, will enable quantum-limited measurements, providing information on electron coherence and entanglement at the individual particle level.
Determining the quantum state of a given quantum-mechanical system is a fundamental task in physics. Quantum-state tomography has been pivotal for establishing quantum optics [1-4] and for revealing the properties of bound charges in materials [5-7]. An emerging other object for studying and utilizing quantum effects are free electrons, elementary particles that are central to high-resolution microscopy [8,9], electron-based quantum optics [10-17], ul-trafast electron microscopy [18-24] and particle accelerators [25-27]. However, free electrons are intrinsically incoherent, and we lack a broadly applicable method to measure and control their quantum state beyond special cases with discrete energy sidebands [28,29]. Here, we report a universal approach to measure arbitrary free-electron quantum states in continuous variables. Two monochromatic but spectrally shifted laser waves produce interfering quan-tum paths that directly reveal the density matrix and thus all essential properties of the pure wavepackets, the ensemble, and their interlinks. As a first application, we show how the quantum state of a single electron is modified by many-body Coulomb interactions of a sur-rounding electron gas. The reported concepts and results provide insight into otherwise hid-den correlations in electron beams and enable the controlled optimization of exceptional quantum states for free-electron quantum optics or quantum electron microscopy.
There is a growing interest in reconstructing the density matrix of photoelectron wavepackets, in particular in complex systems where decoherence can be introduced either by a partial measurement of the system or through coupling with a stochastic environment. To this end, several methods to reconstruct the density matrix, quantum state tomography protocols, have been developed and tested on photoelectrons ejected from noble gases following absorption of extreme ultraviolet (XUV) photons from attosecond pulses. It remains a challenge to obtain model-free, single scan protocols that can reconstruct the density matrix with high fidelities. Current methods require extensive measurements or involve complex fitting of the signal. Efficient single-scan reconstructions would be of great help to increase the number of systems that can be studied. We propose a new and more efficient protocol that is able to reconstruct the continuous variable density matrix of a photoelectron in a single time delay scan. It is based on measuring the coherences of a photoelectron created by absorption of an XUV pulse using a broadband infrared (IR) probe that is scanned in time and a narrowband IR reference that is temporally fixed to the XUV pulse. We illustrate its performance for a Fano resonance in He as well as mixed states in Ar arising from spin-orbit splitting. We show that the protocol results in excellent fidelities and near-perfect estimation of the purity.
To quantify the effect of decoherence in quantum measurements, it is desirable to measure not merely the square modulus of the spatial wave function, but the entire density matrix, whose phases carry information about momentum and how pure the state is. An experimental setup is presented that can measure the density matrix (or equivalently, the Wigner function) of a beam of identically prepared charged particles to an arbitrary accuracy, limited only by count statistics and detector resolution. The particles enter into an electric field, causing simple harmonic oscillation in the transverse direction. This corresponds to rotating the Wigner function in phase space. With a slidable detector, the marginal distribution of the Wigner function can be measured from all angles. Thus the phase-space tomography formalism can be used to recover the Wigner function by the standard inversion of the radon transform. By applying this technique to, for instance, double-slit experiments with various degrees of environment-induced decoherence, it should be possible to make our understanding of decoherence and apparent wave-function collapse less qualitative and more quantitative. \textcopyright{} 1996 The American Physical Society.
The physical properties of a quantum system, whether pure or mixed, are described fully by its density matrix. Recovery of the density matrix through projective measurements -- referred to as quantum state tomography -- is a cornerstone of quantum optics and metrology. The implementation of this approach in transmission electron microscopy, in particular for the characterisation of an electron beam after inelastic scattering, has remained a longstanding challenge as a result of the complexity of scanning high-dimensional phase spaces, with the number of required measurements growing quadratically with space dimensionality. Here, we introduce a simplified approach by restricting tomography to the electron orbital angular momentum (OAM) subspace. By using an electron optical device known as an OAM sorter, we discretise the phase space into a finite set of measurable states, thus significantly reducing the experimental and computational burden. The resulting measurements suffice to probe essential features of inelastic scattering. We demonstrate the technique by studying the inelastic scattering of a structured electron probe exciting volume plasmons in a carbon film. The combined use of a structured beams and OAM-resolved quantum tomography reveals symmetry-breaking effects and offers insight into the coherence and evolution of the scattered quantum states. Analysis of the diagonalised density matrices further reveals the nature of the induced state transitions, demonstrating the power of the approach for quantum tomography of electron scattering.