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Nature Materials

Quantum nonlinearities at the single-particle level

Dario Gerace, Fabrice P. Laussy, D. Sanvitto

Published Feb 18, 2019• 16 citations
Publisher
DOI
10.1038/s41563-019-0298-3

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We present the experimental observation of photon-photon interactions at the single-particle level. The linearly polarized signal beam undergoes Faraday rotation by a nonlinear effective magnetic field induced by a very weak circularly polarized control beam due to the giant Kerr-like interactions between exciton-polaritons in our quantum well-based 0D microcavity structures. We measure a phase shift with a slope of 3.5×10^-3 radians per particle for low cavity occupancies between 0.1 and 3 excited by the control beam. These experimental findings are in agreement with theoretical models and pave the way towards the development of scalable photonic quantum gates.
A general method for extending a nondissipative nonlinear Schr\"odinger and Liouville--von Neumann one-particle dynamics to an arbitrary number of particles is described. It is shown at a general level that the dynamics so obtained is completely separable, which is the strongest condition one can impose on dynamics of composite systems. It requires that for all initial states (entangled or not) not only can a subsystem not be influenced by any action undertaken by an observer in a separated system (strong separability), but additionally the self-consistency condition ${\mathrm{Tr}\mathrm{}}_{2}\ensuremath{\circ}{\ensuremath{\varphi}}_{1+2}^{t}={\ensuremath{\varphi}}_{1}^{t}\ensuremath{\circ}{\mathrm{Tr}\mathrm{}}_{2}$ is fulfilled. It is shown that a correct extension to NNN particles involves integro-differential equations, which, in spite of their nonlocal appearance, make the theory fully local. As a consequence, a much larger class of nonlinearities satisfying the complete separability condition is allowed than has been assumed so far. In particular all nonlinearities of the form $F(|\ensuremath{\psi}(x)|)$ are acceptable. This shows that the locality condition does not single out logarithmic or one-homogeneous nonlinearities.