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Joint Conference of the European Frequency and Time Forum and IEEE International Frequency Control Symposium (EFTF/IFCS)

The Lasing Realization of Rb Four-Level Active Optical Clock

Pengyuan Chang, Shengnan Zhang, Haosen Shang, Jingbiao Chen

Published May 1, 2018• 0 citations
Publisher

Abstract

Since the concept of active optical clock has been proposed, the experimental research of Rb four-level active optical clock has never been carried out, but it has great value in research and application. First the Rb atoms are pumped from ground state 5S1/2to 6P3/2excited state by a narrow-linewidth 420 nm laser, and then decay to lower energy levels by spontaneous transitions, and immediately are pumped by pumping laser again. This process continues until the population inversion is established between 6 S and 5P states. Once the population inversion is built up, a Fabry-Perot type resonator, at a bad cavity regime whose cavity mode linewidth is much wider than that of the laser gain profile, is used to realize 1367 nm active optical clock laser output. As Rb atom 1367 nm 5P-6S excited state transition is in the communication E band, it can be used as a narrow-linewidth communication band optical frequency standard, which greatly improves the communication rate and accuracy.

DOI
10.1109/fcs.2018.8597455

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Since the concept of active optical clock has been proposed, the experimental research of Rb four-level active optical clock has never been carried out, but it has great value in research and application. First the Rb atoms are pumped from ground state 5S1/2to 6P3/2excited state by a narrow-linewidth 420 nm laser, and then decay to lower energy levels by spontaneous transitions, and immediately are pumped by pumping laser again. This process continues until the population inversion is established between 6 S and 5P states. Once the population inversion is built up, a Fabry-Perot type resonator, at a bad cavity regime whose cavity mode linewidth is much wider than that of the laser gain profile, is used to realize 1367 nm active optical clock laser output. As Rb atom 1367 nm 5P-6S excited state transition is in the communication E band, it can be used as a narrow-linewidth communication band optical frequency standard, which greatly improves the communication rate and accuracy.
Two feasible schemes are proposed by laser cooling of alkali atoms to realize the narrow-linewidth, continual superradiant lasing. Utilizing the D1 gray molasses to realize a cloud of cold Cs atoms for the two-level Faraday active optical clock (AOC), the effect of Doppler broadening on the transmission bandwidth of Faraday atomic filter will be effectively suppressed to the level of natural linewidth. Thus, the influence of mechanical or thermal vibrations of cavity mirrors on the clock laser will be decreased by about 102 times, which is expected to further narrow the laser linewidth by two orders of magnitude compared with the thermal atomic Faraday AOC to Hz level. Moreover, the four-level AOC based on the narrow linewidth cooling of Cs atoms using the 6S-7P transition is proposed. The 455 nm laser at 6S1/2-7P3/2transition plays two roles simultaneously, one is the cooling laser for a magneto-optical trap (MOT), another is the pumping laser for population inversion of 1470 nm clock transition, which is helpful to improve the compactness of the system. In the four-level structure, the frequency of pumping laser is far detuning from that of clock laser, therefore, the light shift resulting from the 455 nm laser is negligible. This four-level AOC based on cold atoms will further reduce the collision shift in thermal atom system to achieve a high-precision optical frequency reference.
An active optical clock can provide laser light source with potential much narrower linewidth than that of conventional cavity stabilized laser for optical clocks since many cavity noises, including the Brownian thermal noise, can be reduced by orders of magnitude. In this report, a scheme of active optical clock based on Sr atomic beam is proposed. The experimental work of population inversion has been done. A 689 nm laser is used to realize the population inversion between (5s5p)3P1state and (5s2)1S0state by the method of adiabatic rapid passage. A pumping rate of 59% is obtained. In order to establish the population inversion more effectively, an experimental scheme is proposed with a 483 nm pumping laser. A 687 nm laser is used for verification of pumping effectiveness. The atoms left in ground state after 689 nm laser and 687 nm laser pumping is about 7%, which may mainly result from87Sr isotope.
We realize the lasing of cesium active optical clock with 459 nm laser pumping, which operates deep in the optical bad-cavity regime. The ratio between cavity bandwidth and gain bandwidth is 55.08 theoretically. With 459 nm laser pumping, the population inversion occurs between the cesium 7S1/2state and 6P3/2state, and the stimulated radiation between the two states is realized. The 1469.9 nm output signal of cesium active optical clock can reach a power of 8 μW. The output power also shows a threshold character with pumping laser power and can be influenced by the Cs cell temperature. This active optical clock has an advantage in stability over the conventional optical clocks, due to its suppression of cavity pulling effect, which is also demonstrated experimentally.
We present an active optical clock scheme with a four-level quantum potassium system. We calculate the population probabilities of each state using the density matrix. At the steady state, ρ 33 and ρ 55 are equal to 8.3% and 3.5%, respectively, and the population inversion between the 5S 1/2 and 4P 3/2 states is built up in the thermal potassium cell with a 404.7 nm pumping laser. According to the mechanism of the active optical clock, under the action of the 404.7 nm pumping laser, the scheme can output a 1252.2 nm quantum-limited-linewidth laser, which can be directly used as an active optical frequency standard.
We experimentally demonstrate the collective emission behavior and suppressed cavity-pulling effect of four-level active optical clock with Cesium atoms. Thermal Cesium atoms in a glass cell velocity selective pumped with a 455.5 nm laser operating at 6S1/2_{1/2}1/2​ to 7P3/2_{3/2}3/2​ transition are used as lasing medium. Population inverted Cesium atoms between 7S1/2_{1/2}1/2​ and 6P3/2_{3/2}3/2​ levels are optical weakly coupled by a pair cavity mirrors working at deep bad-cavity regime with a finesse of 4.3, and the ratio between cavity bandwidth and gain bandwidth is approximately 45. With increased 455.5 nm pumping laser intensity, the output power of cesium active optical clock at 1469.9 nm from 7S1/2_{1/2}1/2​ level to 6P3/2_{3/2}3/2​ level shows a threshold and reach a power of 13 μμμW. Active optical clock would dramatically improve the optical clock stability since the lasing frequency does not follow the cavity length variation exactly, but in a form of suppressed cavity pulling effect. In this letter the cavity pulling effect is measured using a Fabry-Perot interferometer (FPI) to be reduced by a factor of 38.2 and 41.4 as the detuning between the 1469.9 nm cavity length of the Cs active optical clock and the Cs 1469.9 nm transition is set to be 140.8 MHz and 281.6 MHz respectively. The mechanism demonstrated here is of great significance for new generation optical clocks and can be applied to improve the stability of best optical clocks by at least two orders of magnitude.