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Cavity Quantum Electrodynamics in a wide aperture spherical resonator. Part II: Vacuum-field atom trapping

Jean-Marc Daul, Philippe Grangier

Published Jan 1, 2003• 0 citations
OpenAlex

Abstract

We consider the situation where a two-level atom is placed in the vicinity of the center of a spherical cavity with a large numerical aperture. The vacuum field at the center of the cavity is actually equivalent to the one obtained in a microcavity, and both the dissipative and the reactive parts of the atom's spontaneous emission are significantly modified. Using an explicit calculation of the spatial dependence of the radiative relaxation rate and of the associated level shift, we show that for a weakly excitating light field, the atom can be attracted to the center of the cavity by vacuum-induced light shifts.

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We consider the situation where a two-level atom is placed in the vicinity of the center of a spherical cavity with a large numerical aperture. The vacuum field at the center of the cavity is actually equivalent to the one obtained in a microcavity, and both the dissipative and the reactive parts of the atom's spontaneous emission are significantly modified. Using an explicit calculation of the spatial dependence of the radiative relaxation rate and of the associated level shift, we show that for a weakly excitating light field, the atom can be attracted to the center of the cavity by vacuum-induced light shifts.
We present a general formalism for studying the cavity quantum electrodynamics for an atom or a radiating dipole inside a hollow spherical cavity. The atomic-energy-level shifts and the modified dipolar decay rates are calculated in specific cases. In particular, the energy shifts for an atom located at the center of an empty sphere (radius a) vary as 1/a4{\mathit{a}}^{4}a4 for large ka and 1/a2{\mathit{a}}^{2}a2 for small ka, where k is the wave number. We attribute these variations to the retarded Casimir-Polder interaction and the state-independent vacuum-field contribution, respectively. \textcopyright{} 1996 The American Physical Society.
We present a general, semimicroscopic, self-consistent treatment of spontaneous emission for a two-level atom in a dielectric microcavity with arbitrary shape. Both lossless and absorbing media are considered. Our approach is based on linear-response theory and the coupled-dipole method. We illustrate our method on spherical and cubic cavities. We discuss the Purcell effect, the frequency shift, the local-field effect, and the dipole-dipole coupling experienced by a source placed in a microcavity.
We revisit the problem of spontaneous emission by a two-level system in a cavity, concentrating in particular on those aspects associated with the finite propagation time of light between the atom and the cavity boundaries. We find that spontaneous emission always occurs first at the free space rate and there is then an abrupt change in these dynamics when light reflected by the cavity mirrors returns to the atom, leading to interference effects that result either in an enhancement or a reduction of this rate or in a periodic exchange of excitation between the atom and the cavity field. From this point of view, reversible spontaneous emission in terms of single-mode ``vacuum Rabi oscillations'' can be interpreted as resulting from the interference between the multimode partial waves reflected at the cavity mirrors and the instantaneously radiated light. \textcopyright{} 1996 The American Physical Society.
A formalism for studying spontaneous decay of an excited two-level atom in the presence of dispersing and absorbing dielectric bodies is developed. An integral equation, which is suitable for numerical solution, is derived for the atomic upper-state-probability amplitude. The emission pattern and the power spectrum of the emitted light are expressed in terms of the Green tensor of the dielectric-matter formation, including absorption and dispersion. The theory is applied to the spontaneous decay of an excited atom at the center of a three-layered spherical cavity, with the cavity wall being modeled by a band-gap dielectric of Lorentz type. Both weak and strong coupling are studied, the latter with a special emphasis on cases where the atomic transition is (i) in the normal-dispersion zone near the medium resonance, and (ii) in the anomalous-dispersion zone associated with the band gap. In a single-resonance approximation, conditions of the appearance of Rabi oscillations and closed solutions to the evolution of the atomic state population are derived, which are in good agreement with the exact numerical results.
Introduction Ever since 1916/17 when Einstein argued [45] [46] that spontaneous emission must occur if matter and radiation are to achieve thermal equilibrium, physicists have believed that spontaneous emission is an inherent quantum mechanical property of atoms and that excited atoms inevitably radiate. This view, however, overlooks the fact that spontaneous emission is a consequence of the coupling of quantized energy states of atoms with the quantized radiation field, and is a manifestation of quantum noise or of emission ‘stimulated’ by ‘vacuum fluctuations’. An infinity of vacuum states is available to the photon radiated by an excited atom placed in free space, leading to the effective irreversibility of such emissions. If these vacuum states are modified, as for example by placing an excited atom between closely spaced mirrors or in a small cavity (essentially the Casimir effect), spontaneous emission can be greatly inhibited or enhanced or even made reversible. Recent advances in atomic and optical techniques have made it possible to control and manipulate spontaneous emission. A whole new branch of quantum optics called ‘cavity QED’ has developed since 1987 utilizing these dramatic changes in spontaneous emission rates in cavities to construct new kinds of microscopic masers or micromasers that operate with a single atom and a few photons or with photons emitted in pairs in a two-photon transition.
The aim of this work is to find ways to trap an atom in a cavity. In contrast to other approaches, we propose a method where the cavity is basically in the vacuum state and the atom is in the ground state. The idea is to induce a spatial dependent ac-Stark shift by irradiating the atom with a weak laser field, so that the atom experiences a trapping force. The main feature of our setup is that dissipation can be strongly suppressed. We estimate the lifetime of the atom as well as the trapping potential parameters, and compare our estimations with numerical simulations.