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Physical Review A

Spontaneous emission in microcavity electrodynamics

Adel Rahmani, Garnett W. Bryant

Published Feb 20, 2002• 23 citations
Publisher

Abstract

We present a general, semimicroscopic, self-consistent treatment of spontaneous emission for a two-level atom in a dielectric microcavity with arbitrary shape. Both lossless and absorbing media are considered. Our approach is based on linear-response theory and the coupled-dipole method. We illustrate our method on spherical and cubic cavities. We discuss the Purcell effect, the frequency shift, the local-field effect, and the dipole-dipole coupling experienced by a source placed in a microcavity.

DOI
10.1103/physreva.65.033817

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•Jan 1, 2003•0 citations
We present a general, semimicroscopic, self-consistent treatment of spontaneous emission for a two-level atom in a dielectric microcavity with arbitrary shape. Both lossless and absorbing media are considered. Our approach is based on linear-response theory and the coupled-dipole method. We illustrate our method on spherical and cubic cavities. We discuss the Purcell effect, the frequency shift, the local-field effect, and the dipole-dipole coupling experienced by a source placed in a microcavity.
Starting from a quantum Maxwell equation for the vector potential operator, we study the spontaneous emission properties of a two-level atom interacting with the electromagnetic field in a lossless and inhomogeneous dielectric structure and express the spontaneous emission rate, the external quantum efficiency, and the spontaneous emission factor in terms of the classical Green function of the dielectric structure. Comparing these results with the corresponding classical results, we show that the above quantities can be calculated from the radiation field of a classical dipole. Based on this correspondence, a numerical algorithm is developed to calculate the modification of spontaneous emission in microcavities. The line shape of the emission spectrum of the light source and the decay of the cavity resonant modes are automatically taken into account in this algorithm. The approximate expressions for the spontaneous emission rate and the spontaneous emission factor are discussed.
The theory of spontaneous emission in dielectric media is extended to take proper account of dispersion and local field corrections. For the case of spontaneous emission in a plasma or radiative electron-hole recombination in a semiconductor, there are effectively no local field corrections. A shift of emission lines due to a dispersive host medium is predicted and interpreted. The corrections to spontaneous and stimulated emission due to dielectric interfaces in microcavity lasers are discussed.
Summary form only given. The feasibility of cavity-controlled spontaneous emission of a motionless two level atom is analyzed quantum mechanically and nonperturbatively. It is proposed to control the emission by putting the excited atom into the combined field of two lossless modes with their frequencies /spl omega//sub 2,1/ detuned symmetrically about the atomic one /spl omega//sub /spl alpha//, i.e. /spl omega//sub 2,1/=/spl omega//sub /spl alpha///spl plusmn//spl Delta/. The controlling /spl omega//sub 2,1/ modes are isolated from the free radiation field by an one-dimensional ideal cavity (or by two crossed ones) at zero temperature. These modes are taken to be linearly polarized in the same plane. Because the wavelength and cavity dimensions are assumed to be of the same order, the retardation effects are neglected. The spontaneous emission is treated as a radiative decay of the macromolecule-like "atom+/spl omega//sub 2,1/ modes"-subsystem (the H/sub s/-one) under its interaction with the free H/sub k/-field.
We consider the situation where a two-level atom is placed in the vicinity of the center of a spherical cavity with a large numerical aperture. The vacuum field at the center of the cavity is actually equivalent to the one obtained in a microcavity, and both the dissipative and the reactive parts of the atom's spontaneous emission are significantly modified. Using an explicit calculation of the spatial dependence of the radiative relaxation rate and of the associated level shift, we show that for a weakly excitating light field, the atom can be attracted to the center of the cavity by vacuum-induced light shifts.