Ultracold Bose gases as precise quantum simulators have emerged amongst the leaders in the current race – a second quantum revolution – toward the promise of unfathomable sensitivity, scope, and speed of a new era of technology. The only path leading to these advancements is through many-body descriptions, especially in regimes where interatomic interactions render many approximations incompatible with the physics. The research in this dissertation unlocks a piece of this mystery through investigations of many-body quantum tunneling of ultracold bosons in optical lattices. A key mechanism to characterizing the dynamics, matrix product state simulations equip the many-body toolbox with efficient optimization of large Hilbert spaces together with correlation and entropy measures that help clarify when semiclassical or mean-field approximations fail. In this thesis we obtain the following results. Macroscopic quantum tunneling escape of a Bose-Einstein condensate – comprised of tens of thousands of 87Rb atoms – from a single well, as portrayed through both experiment and theory, highlights non-exponential decay in the number of atoms trapped behind the barrier. Additionally, explicit symmetry breaking of a biperiodic optical lattice ring trap to a uniform one illustrates a critical symmetry-breaking strength at which the system transitions from a state of remembering to a state of forgetting its initial symmetry state; this symmetry memory indicates a new form of quantum dynamics that requires the quantum advantage for scaling up particle number and lattice sites. Extensive characterization of dynamical regimes in a bosonic Josephson junction – underlaid by an optical lattice as described by the Bose-Hubbard model – reveal substantial deviation of many body dynamics from the mean field or semiclassical predictions underlying the usual operating regime of Josephson junctions. Initial state population and phase yield insight into dynamic tunneling regimes of a quasi one-dimensional double well potential, through the Z2 spontaneous symmetry-breaking phase transition from Josephson oscillations to macroscopic self-trapping. We demonstrate that with increasing repulsive interaction strength, the U(1) superfluid-Mott insulator phase transition induces localized dynamics in the number density, such as particle-hole and soliton formation. Moreover, g^(2) correlations unveil a new dynamic regime – the Fock flashlight. The new field of atomtronics – or atomic circuits – has emerged with many studies of weakly-interacting condensates. In contrast, and building on our work on many-body effects in the double wells underlying Josephson junctions, we present a proof-of-principle of a Mott-insulating atomtronic switch that requires strongly-interacting bosons. Through transient analysis, we reveal that hole conductance can be modulated via tuning interaction strength through a critical value, thus propelling the state to the next ``wedding cake'' layer of the Mott insulating structure. This critical interaction strength is a…
Ultracold Bose gases as precise quantum simulators have emerged amongst the leaders in the current race – a second quantum revolution – toward the promise of unfathomable sensitivity, scope, and speed of a new era of technology. The only path leading to these advancements is through many-body descriptions, especially in regimes where interatomic interactions render many approximations incompatible with the physics. The research in this dissertation unlocks a piece of this mystery through investigations of many-body quantum tunneling of ultracold bosons in optical lattices. A key mechanism to characterizing the dynamics, matrix product state simulations equip the many-body toolbox with efficient optimization of large Hilbert spaces together with correlation and entropy measures that help clarify when semiclassical or mean-field approximations fail. In this thesis we obtain the following results. Macroscopic quantum tunneling escape of a Bose-Einstein condensate – comprised of tens of thousands of 87Rb atoms – from a single well, as portrayed through both experiment and theory, highlights non-exponential decay in the number of atoms trapped behind the barrier. Additionally, explicit symmetry breaking of a biperiodic optical lattice ring trap to a uniform one illustrates a critical symmetry-breaking strength at which the system transitions from a state of remembering to a state of forgetting its initial symmetry state; this symmetry memory indicates a new form of quantum dynamics that requires the quantum advantage for scaling up particle number and lattice sites. Extensive characterization of dynamical regimes in a bosonic Josephson junction – underlaid by an optical lattice as described by the Bose-Hubbard model – reveal substantial deviation of many body dynamics from the mean field or semiclassical predictions underlying the usual operating regime of Josephson junctions. Initial state population and phase yield insight into dynamic tunneling regimes of a quasi one-dimensional double well potential, through the Z2 spontaneous symmetry-breaking phase transition from Josephson oscillations to macroscopic self-trapping. We demonstrate that with increasing repulsive interaction strength, the U(1) superfluid-Mott insulator phase transition induces localized dynamics in the number density, such as particle-hole and soliton formation. Moreover, g^(2) correlations unveil a new dynamic regime – the Fock flashlight. The new field of atomtronics – or atomic circuits – has emerged with many studies of weakly-interacting condensates. In contrast, and building on our work on many-body effects in the double wells underlying Josephson junctions, we present a proof-of-principle of a Mott-insulating atomtronic switch that requires strongly-interacting bosons. Through transient analysis, we reveal that hole conductance can be modulated via tuning interaction strength through a critical value, thus propelling the state to the next ``wedding cake'' layer of the Mott insulating structure. This critical interaction strength is a…
In this thesis we investigate strongly-correlated states of ultracold bosonic atoms in rotating ring lattices and arrays of double-well potentials. In the first part of the thesis, we study the tunneling dynamics of ultracold bosons in double-well potentials. In the non-interacting limit single-particle transitions dominate, while in the interaction-dominated regime correlated tunneling of all particles prevails. At intermediate times of the many-particle flopping process correlated states occur, but the timescales of these processes increase dramatically with the number of particles. Using an array of double-well potentials, a large number of such few-particle superposition states can be produced in parallel. In the second part of the thesis, we study the effects of rotation on ultracold bosons confined to one-dimensional ring lattices. We find that at commensurate filling there exists a critical rotation frequency, at which the ground state of the weakly-interacting gas is fragmented into a macroscopic superposition of different quasi-momentum states. We demonstrate that the generation of such superposition states using slightly non-uniform ring lattices has several practical advantages. Moreover, we show that different quasi-momentum states can be distinguished in time-of-flight absorption imaging and propose to probe correlations via the many-body oscillations induced by a sudden change in the rotation frequency. Finally, we compare these macroscopic superposition states to those occurring in superconducting quantum interference devices. In the third part of the thesis, we demonstrate the creation of entangled states with ultracold bosonic atoms by dynamical manipulation of the shape of the lattice potential. To this end, we consider an optical superlattice that allows both the splitting of each site into a double-well potential and the variation of the height of the potential barrier between the sites. We show how to use this array of double-well potentials to perform entangling operations between neighboring qubits encoded on the Zeeman levels of the atoms. As one possible application, we present a method of realizing a resource state for measurement-based quantum computation via Bell-pair measurements. In the final part of the thesis, we study ultracold bosons on a two-dimensional square lattice in the presence of an effective magnetic field and point out a couple of features this system has in common with ultracold bosons in one-dimensional rotating ring lattices.
Quantum tunneling remains unexplored in many regimes of many-body quantum physics, including the effect of quantum phase transitions on tunneling dynamics. In general, the quantum phase is a statement about the ground state and has no relation to far-from-equilibrium dynamics. Although tunneling is a highly dynamical process involving many excited states, we find that the quantum phase of the Bose-Hubbard model determines phase-dependent tunneling outcomes for the quantum tunneling escape, or quasi-bound problem. Superfluid and Mott insulator correlations lead to a new quantum tunneling rate, the quantum fluctuation rate. This rate shows surprising and highly dynamical features, such as oscillatory interference between trapped and escaped atoms and a completely different macroscopic quantum tunneling behavior for superfluid and Mott insulator phases. In the superfluid phase we find that escape dynamics are wave-like and coherent, leading to interference patterns in the density with a rapid decay process which is non-exponential. Quantum entropy production peaks when about half the atoms have escaped. In the Mott phase, despite stronger repulsive interactions, tunneling is significantly slowed by the presence of a Mott gap, creating an effective extra barrier to overcome. Only one atom can tunnel at a time, yet the decay process is nearly linear, completely defying the single-particle exponential model. Moreover, quantum entropy peaks when only about one quarter of the atoms have escaped. These and many other such effects go beyond the usual notions of single-particle quantum tunneling, quantum statistical effects on tunneling, and well-known semi-classical approaches from WKB to instanton theory. These results thus open up a new regime of exploration of far-from-equilibrium dynamics for quantum simulators and quantum dynamics.
Ultracold atoms in optical lattices constitute a versatile many-body platform with highly tunable parameters, allowing us to emulate a multitude of complex quantum systems, in the laboratory, even those eluding analytical treatment. In particular, the nonequilibrium dynamics of strongly correlated many-body systems represents one of the most challenging problems of modern quantum physics, with applications ranging from thermalization dynamics and transport properties to the management of correlations and the control of the dynamics. Understanding nonequilibrium phenomena of strongly correlated systems is a formidable task. A very promising route to gain insight into such systems is to examine few-body setups which contain only a few relevant degrees of freedom, yet incorporating the quantum correlations between the particles.
The present dissertation contributes to the understanding of the nonequilibrium dynamics of strongly-correlated quantum many-body systems by exploring systems of few-bosons − of one or two species − trapped in optical lattices. The systems are driven out-of-equilibrium either by performing a quench of a Hamiltonian parameter or by considering a time-periodic modulation of the external confinement. In the course of several consecutive works, we showcase different ways to couple the nonequilibrium modes, while unveiling their correlated nature and microscopic origin. To simulate the nonequilibrium dynamics, a sophisticated, highly flexible ab-initio method for numerically solving the time-dependent many-body Schrodinger equation is utilized, namely the Multi-Layer Multi-Configuration Time-Dependent Hartree Method for Atomic Mixtures (ML-MCTDHX).
Within the first part we study in six consecutive works the correlated nonequilibrium dynamics of few-boson systems in one-dimensional finite lattices. Starting from weak interactions, it is shown that a sudden increase of the interaction strength generates a global density-wave tunneling dynamics as well as intrawell breathing and cradle-like excited-band processes. The cradle process is a dipole-like process generated by the quench-induced over-barrier transport and it is one of the central results of the present thesis. Remarkably enough, the interaction quenches couple the density-wave and cradle modes, inducing resonance phenomena between the inter and intrawell dynamics. We further show that the cradle mode is inherently related to the initial delocalization and, following a quench from strong-to-weak interactions, can be excited only for incommensurate setups with filling larger than unity. Alternatively, a sudden ramping down of the lattice depth which favors the spatial delocalization is employed to access the cradle mode for setups with filling smaller than unity. Following a multiple interaction quench protocol, we observe the rise of several lowest-band tunneling modes as well as the cradle and the breathing mode. Besides the cradle mode, all other excited modes are highly tunable possessing different frequencies during and in between the quenches. In the excitation dynamics a monotonic behavior with increasing quench amplitude and a non-linear dependence on the duration of the application of the quenched interaction strength is revealed. Additionally, a periodic population transfer between momenta for quenches of increasing interaction is observed, with a power-law frequency dependence on the quench amplitude. Linear interaction quenches from a superfluid to a Mott-insulator state excite various inter- and intraband tunneling modes. The competition between the quench rate and the interparticle repulsion leads to a resonant dynamical response, at moderate ramp times, being related to avoided-crossings in the many-body eigenspectrum.
The resultant higher-band excitation dynamics is shown to obey an exponential decay possessing two distinct time scales with varying ramp time. Inspecting the crossover from shallow to deep lattices we find that for a diabatic quench the excited-band fraction decreases, while approaching the adiabatic limit it exhibits a nonlinear behavior for increasing height of the potential barrier. Quenching from strong-to-weak interactions leads to a melting of the Mott-insulator and negligible higher-band excitations.
Performing quenches either on the wavevector or the phase of a spatially dependent interaction profile triggers various tunneling channels and a rich excitation dynamics which is amplified for increasing inhomogeneity amplitude. Most importantly, the phase quench is shown to induce a directional transport enabling us to discern, otherwise, energetically degenerate tunneling pathways.
Finally, a periodic population transfer between distinct momenta for quenches of increasing wavevector and a directed occupation of higher momenta following a phase quench is observed. Employing a quench of an additional harmonic trap from strong-to-weak confinement, we find that the competition between the initial localization and the repulsive interaction leads to a resonant response of the system related to avoided-crossings in the many-body eigenspectrum with varying final trap frequency. Furthermore, we show that these avoided-crossings can be utilized to prepare the system in a desired state.
The second part comprises two efforts and is devoted to the study of the nonequilibrium dynamics of finite ultracold bosonic ensembles in periodically driven one-dimensional optical lattices. For a shaken lattice, a wide range of driving frequencies is covered and a resonant behavior of the intrawell dynamics is revealed and found to be related to a rich intraband excitation spectrum.
Moreover, it is shown that for increasing repulsion a strong suppression of the interwell tunneling and an enhanced excitation dynamics occurs. For a vibrating lattice, an additional interaction quench gives rise to admixtures of different excitations in the outer wells, an enhanced breathing in the center and an amplification of the emerging tunneling dynamics. The occurence of multiple resonances between the inter- and intrawell dynamics at different quench amplitudes is revealed, with the position of the resonances being tunable via the driving frequency and thus allowing for further control of the mode coupling in optical lattices.
In the third and final part of this thesis we unravel the quench dynamics of a Bose-Bose and a Bose-Fermi mixture. Utilizing an interspecies interaction quench we cross the miscibility-immiscibility threshold in a harmonically confined Bose-Bose mixture. We show that increasing the interspecies repulsion coefficient results in a filamentation of the density of each species, with the spontaneously generated filaments being strongly correlated and exhibiting domain-wall structures. Strikingly, by following the reverse quench protocol, i.e., upon decreasing the interspecies interaction strength, the formation of multiple dark-antidark solitary waves is observed. These solitary wave structures are found to decay into the many-body environment, soon after their generation in sharp contrast to the predictions of the mean-field approximation. To relate our findings with possible experimental realizations, we simulate, for the first time for binary mixtures, single-shot images showcasing that the growth rate of the variance of a sample of single-shots probes the degree of entanglement inherent in the system. As a next step we investigate the expansion dynamics of a mass balanced Bose-Fermi mixture confined in a one-dimensional optical lattice upon quenching an imposed harmonic trap from strong-to-weak confinement. Tuning the interspecies interaction strength we realize the immiscible and miscible correlated ground state phases. We further show that the system's dynamical response crucially depends on the initial phase and consists of an expansion of each cloud and an interwell tunneling dynamics. Varying the quench amplitude and referring to a fixed phase a multitude of response regimes is unveiled, being richer within the immiscible phase, which are described by distinct expansion strengths and tunneling channels. Finally, in the expansion dynamics a two-body anti-correlated behavior between the predominantly occupied wells is unveiled.
Abstract Typical treatments of superconducting or superfluid Josephson junctions rely on mean-field or two-mode models; we explore many-body dynamics of an isolated, ultracold, Bose-gas long Josephson junction using time-evolving block decimation simulations. We demonstrate that with increasing repulsive interaction strength, localized dynamics emerge that influence macroscopic condensate behavior and can lead to the formation of solitons that directly oppose the symmetry of the junction. Initial state population and phase yield insight into dynamic tunneling regimes of a quasi one-dimensional double well potential, from Josephson oscillations to macroscopic-self-trapping. Population imbalance simulations reveal substantial deviation of many-body dynamics from mean-field Gross–Pitaevskii predictions, particularly as the barrier height and interaction strength increase. In addition, the sudden approximation supports localized particle–hole formation after a diabatic quench, and correlation measures unveil a new dynamic regime: the Fock flashlight.
We explore the interplay between tunneling and interatomic interactions in the dynamics of a bosonic Josephson junction. We tune the scattering length of an atomic ^{39}K Bose-Einstein condensate confined in a double-well trap to investigate regimes inaccessible to other superconducting or superfluid systems. In the limit of small-amplitude oscillations, we study the transition from Rabi to plasma oscillations by crossing over from attractive to repulsive interatomic interactions. We observe a critical slowing down in the oscillation frequency by increasing the strength of an attractive interaction up to the point of a quantum phase transition. With sufficiently large initial oscillation amplitude and repulsive interactions, the system enters the macroscopic quantum self-trapping regime, where we observe coherent undamped oscillations with a self-sustained average imbalance of the relative well population. The exquisite agreement between theory and experiments enables the observation of a broad range of many body coherent dynamical regimes driven by tunable tunneling energy, interactions and external forces, with applications spanning from atomtronics to quantum metrology.
In this thesis, the behavior of ultracold bosonic systems in external potentials is investigated. Such systems are typically realized as Bose-Einstein condensates, where dilute atomic gases cooled to extremely low temperatures exhibit collective quantum behavior. Because of the large degree of control they allow over the external potential and over the interaction parameters of the many-body system, Bose-Einstein condensates constitute a testing ground for the dedicated study of coherence, correlations, and quantum phase transitions in interacting bosonic systems. This thesis presents an investigation of the many-body physics of ultracold bosons, focusing specifically on how the many-body properties of these ultracold bosonic systems change with changing external potential, how they manifest themselves in experimentally accessible observables, and how these properties can be analyzed using both numerical many-body methods and data-driven approaches. The first part of this thesis focuses on the theoretical description of ultracold bosonic systems in external trapping potentials. Using the multiconfigurational time-dependent Hartree method for bosons (MCTDH-X), numerically exact simulations were performed that allow the calculation of reduced density matrices, natural orbitals, and correlation functions. These quantities were used to analyze the coherence properties and fragmentation of trapped bosonic systems. In particular, double-well systems were investigated as model scenarios in which the gradual formation of a central barrier leads to a redistribution of natural occupations and a transition from a condensed to a fragmented many-body state. In this context, we demonstrate the usefulness of single-shot images, which represent projective measurements of the many-body wave function, for the experimental investigation of the many-body physics of fragmenting system. Single-shot images can be simulated numerically using MCTDH-X, but they are more commonly obtained through experimental measurements. The possibility of extracting many-body information in an experimental context, where said many-body information is not otherwise accessible, is discussed. Supervised machine learning models were trained on simulated single-shot data sets to investigate whether information about the underlying many-body state can be inferred directly from measurement outcomes. The results show that machine learning models are capable of learning patterns in the single-shot images that correlate with properties of the underlying many-body state and can therefore predict density-related quantities with good accuracy. The second part of this thesis focuses on a joint theoretical and experimental investigation of a system of ultracold bosons coupled to an optical cavity. In this system, the atoms interact with a dynamically generated optical potential produced by the cavity field. We use a new theoretical framework that combines a mean-field treatment of the cavity field with a many-body description of the atomic degrees of freedom to be able to capture the emergence of a superradiant self-organized phase and the subsequent transition to a self-organized Mott-insulating state. Our simulations show good agreement with the experimental results, and we discuss where the use of a beyond mean-field treatment in the simulations becomes essential in describing the physics of the different involved phases and quantum states. In summary, the results presented in this thesis demonstrate how numerical many-body simulations and machine learning methods can be used to analyze experimentally accessible observables and to gain insight into the many-body physics of ultracold bosonic systems.