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Journal of Experimental and Theoretical Physics

Specific Features of Interatomic Dipole–Dipole Interaction near a Perfectly Conducting Charged Surface

A. S. Kuraptsev, Igor M. Sokolov

Published Sep 1, 2018• 14 citations
Publisher

Abstract

Specific features of dipole–dipole interaction between two motionless point atoms located near a perfectly conducting charged plate are investigated theoretically within a consistent quantum microscopic approach. These features are analyzed on the basis of the dynamics of cooperative spontaneous decay of excited states of a diatomic quasimolecule. The decay rate is investigated as a function of the interatomic distance, the orientation angle of the quasimolecule with respect to the plane of the plate, and the distance between the quasimolecule and the plate. It is shown that the conducting plate significantly modifies the character of dipole–dipole interaction even when the plate is not charged. When the plate is charged, the Stark splitting of atomic levels leads to an additional modification of the interatomic interaction. The features observed are explained on the basis of the analysis of the spectrum of collective states of diatomic molecules.

DOI
10.1134/s1063776118090169

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Specific features of dipole–dipole interaction between two motionless point atoms located near a perfectly conducting charged plate are investigated theoretically within a consistent quantum microscopic approach. These features are analyzed on the basis of the dynamics of cooperative spontaneous decay of excited states of a diatomic quasimolecule. The decay rate is investigated as a function of the interatomic distance, the orientation angle of the quasimolecule with respect to the plane of the plate, and the distance between the quasimolecule and the plate. It is shown that the conducting plate significantly modifies the character of dipole–dipole interaction even when the plate is not charged. When the plate is charged, the Stark splitting of atomic levels leads to an additional modification of the interatomic interaction. The features observed are explained on the basis of the analysis of the spectrum of collective states of diatomic molecules.
Abstract On the basis of a quantum microscopic approach, we study the excitation dynamics of two motionless point atoms located in fixed positions near a perfectly conductive charged surface. We analyze the spontaneous decay rate of individual atoms near the plate, as well as the strength of the dipole–dipole interaction between different atoms. It is shown that the spontaneous decay rate of an excited atom depends to a significant extent on its distance from the mirror. In the case where the interatomic separation is smaller than or comparable to the wavelength of the resonant radiation, the spontaneous decay dynamics of an excited atom is cooperative, so it is described by a multi-exponential law. It is shown that an electrostatic field caused by the charged plate modifies the character of the dipole–dipole interaction.
Abstract On the basis of the general quantum microscopic theory we study the process of spontaneous decay of an excited atom in a dense and disordered ensemble of point-like impurity atoms embedded into transparent dielectric and located near a charged perfectly conducting surface. We have analyzed the simultaneous influence of the modified spatial structure of field modes near the conductive surface and the electric field on the character of interatomic dipole-dipole interaction. This leads to the modification of the transition spectrum of an excited atom inside an ensemble and the spontaneous decay dynamics. We have shown that the electric field changes the cooperative Lamb shift, as well as the character of sub- and superradiant decay.
On the basis of quantum microscopic approach we study the excitation dynamics of two motionless point atoms located near the perfectly conducting mirror. We have analyzed the spontaneous decay rate of individual atoms near the mirror as well as the strength of dipole-dipole interaction between different atoms. It is shown that the spontaneous decay rate of an excited atom significantly depends on the distance from this atom to the mirror. In the case when the interatomic separation is less or comparable with the wavelength of resonant radiation, the spontaneous decay dynamics of an excited atom is described by multi-exponential law. It depends both the interatomic separation and the spatial orientation of diatomic quasimolecule.
On the basis of a quantum microscopic approach we study the cooperative effects induced by the dipole-dipole interaction in an ensemble of pointlike impurity centers located near a charged perfectly conducting surface. We analyze the simultaneous influence of the modified spatial structure of field modes near the conductive surface and the electric field on the transition spectrum of an excited atom inside an ensemble and on the radiation trapping. We show that the electric field modifies the cooperative Lamb shift, as well as the character of sub- and super-radiant decay. We also demonstrate that electro-optical effects in the presence of a surface are essentially different in comparison with those in free space. The nonmonotonic behavior of electro-optical effects in the presence of a surface with increasing of the electric field has been shown.
In free space, the presence of an atom in its ground state near an excited atom undergoing an electric dipole transition, leads to a modification of the transition rate. This is shown to be modified further if the system of two atoms is located near a macroscopic surface. For small inter-atomic separations, R<< lambda 0 , ( lambda 0 is the reduced electric dipole wavelength) and for distances z,z<< lambda 0 /2 of the system from a perfectly conducting surface, the transition rate for the symmetric state, when both atomic dipoles are oriented perpendicular to the surface, is four times the rate for an isolated single atom. The antisymmetric state is stable. For a configuration in which dipoles are oriented parallel to the surface, both the symmetric and the antisymmetric states are stable. When the behaviour of the same system is investigated near the surface of a semi-infinite electron plasma, serving as a model for a metal, it is found that, in addition to the behaviour in the perfect conductor case, contributions from surface plasmon modes, and other contributions accounting for the finiteness of the plasma frequency are also exhibited.
We compute the energies of the interaction between two atoms placed in the middle of a perfectly reflecting planar cavity, in the weak-coupling nondegenerate regime. Both inhibition and enhancement of the interactions can be obtained by varying the size of the cavity. We derive exact expressions for the dyadic Green's function of the cavity field which mediates the interactions and apply time-dependent quantum perturbation theory in the adiabatic approximation. We provide explicit expressions for the van der Waals potentials of two polarizable atomic dipoles and the electrostatic potential of two induced dipoles. We compute the van der Waals potentials in three different scenarios: two atoms in their ground states, two atoms excited, and two dissimilar atoms with one of them excited. In addition, we calculate the phase-shift rate of the two-atom wave function in each case. The effect of the two-dimensional confinement of the electromagnetic field on the dipole-dipole interactions is analyzed. This effect depends on the atomic polarization. For dipole moments oriented parallel to the cavity plates, both the electrostatic and the van der Waals interactions are exponentially suppressed for values of the cavity width much less than the interatomic distance, whereas for values of the width close to the interatomic distance, the strength of both interactions is higher than their values in the absence of cavity. For dipole moments perpendicular to the plates, the strength of the van der Waals interaction decreases for values of the cavity width close to the interatomic distance, while it increases for values of the width much less than the interatomic distance with respect to its strength in the absence of cavity. We illustrate these effects by computing the dipole-dipole interactions between two alkali atoms in circular Rydberg states.