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Theoretical and Mathematical Physics

Algebraic Aspects of the Dynamics of Quantum Multilevel Systems in the Projection Operator Technique

N. N. Bogolyubov, Andrey Vladimirovich Soldatov

Published Feb 1, 2018• 0 citations
Publisher

Abstract

Using the projection operator method, we obtain approximate time-local and time-nonlocal master equations for the reduced statistical operator of a multilevel quantum system with a finite number N of quantum eigenstates coupled simultaneously to arbitrary classical fields and a dissipative environment. We show that the structure of the obtained equations is significantly simplified if the free Hamiltonian dynamics of the multilevel system under the action of external fields and also its Markovian and non-Markovian evolutions due to coupling to the environment are described via the representation of the multilevel system in terms of the SU(N) algebra, which allows realizing effective numerical algorithms for solving the obtained equations when studying real problems in various fields of theoretical and applied physics.

DOI
10.1134/s0040577918020034

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Using the projection operator method, we obtain approximate time-local and time-nonlocal master equations for the reduced statistical operator of a multilevel quantum system with a finite number N of quantum eigenstates coupled simultaneously to arbitrary classical fields and a dissipative environment. We show that the structure of the obtained equations is significantly simplified if the free Hamiltonian dynamics of the multilevel system under the action of external fields and also its Markovian and non-Markovian evolutions due to coupling to the environment are described via the representation of the multilevel system in terms of the SU(N) algebra, which allows realizing effective numerical algorithms for solving the obtained equations when studying real problems in various fields of theoretical and applied physics.
Exact and approximate master equations were derived by the projection operator method for the reduced statistical operator of a multi-level quantum system with finite number N of quantum eigenstates interacting with arbitrary external classical fields and dissipative environment simultaneously. It was shown that the structure of these equations can be simplified significantly if the free Hamiltonian driven dynamics of an arbitrary quantum multi-level system under the influence of the external driving fields as well as its Markovian and non-Markovian evolution, stipulated by the interaction with the environment, are described in terms of the SU(N) algebra representation. As a consequence, efficient numerical methods can be developed and employed to analyze these master equations for real problems in various fields of theoretical and applied physics. It was also shown that literally the same master equations hold not only for the reduced density operator but also for arbitrary nonequilibrium multi-time correlation functions as well under the only assumption that the system and the environment are uncorrelated at some initial moment of time. A calculational scheme was proposed to account for these lost correlations in a regular perturbative way, thus providing additional computable terms to the correspondent master equations for the correlation functions.
Exact and approximate master equations were derived by the projection operator method for the reduced statistical operator of a multi-level open quantum system with finite number NNN of quantum eigenstates interacting with arbitrary external deterministic fields and dissipative environment simultaneously. Unlike conventional master equations derived by the projection operator method for the quantum systems of this kind so far, these equations are homogeneous in the reduced statistical operator while, at the same time, taking into account initial correlations between the multi-level system and the environment. Consistent representation of the multi-level system evolution in terms of the SU(N)SU(N)SU(N) operator algebra facilitates efficient numerical analysis of these equations derived for various physically realistic quantum models.
We study the non-Markovian dynamics of multilevel quantum systems coupled with a bosonic dissipative environment. Based on the known exact quantum-state diffusion (QSD) equations, we propose a systematic approach to derive exact time-convolutionless master equations for multilevel quantum systems. Through a combination of analytical and numerical approaches, we extract the non-Markovian dynamics of quantum interference in different time scales. Also, we demonstrate the evolution of quantum interference in a four-level system controlled by an external electromagnetic field. Our findings are extended to few-body quantum networks, with a universal formalism established.
Abstract This chapter is devoted to the foundations and to the basic mathematical structure of the non-Markovian quantum dynamics of open systems. It gives a survey of the Nakajima–Zwanzig projection operator methods with the help of which one derives so-called generalized master equations for the reduced system dynamics. In the non-Markovian regime, these master equations involve a retarded memory kernel, i.e. a time-convolution integral taken over the history of the reduced system. The chapter also describes an alternative method of particular relevance in many applications, which is based on a time-local quantum master equation, and which is known as the time-convolutionless projection operator method. This method serves as a starting point for a systematic expansion in terms of ordered cumulants and forms the basis for a non-Markovian stochastic unravelling of the reduced system dynamics.
An extremely useful evolution equation that allows systematically calculating the two-time correlation functions (CF's) of system operators for non-Markovian open (dissipative) quantum systems is derived. The derivation is based on perturbative quantum master equation approach, so non-Markovian open quantum system models that are not exactly solvable can use our derived evolution equation to easily obtain their two-time CF's of system operators, valid to second order in the system-environment interaction. Since the form and nature of the Hamiltonian are not specified in our derived evolution equation, our evolution equation is applicable for bosonic and/or fermionic environments and can be applied to a wide range of system-environment models with any factorized (separable) system-environment initial states (pure or mixed). When applied to a general model of a system coupled to a finite-temperature bosonic environment with a system coupling operator L in the system-environment interaction Hamiltonian, the resultant evolution equation is valid for both L = L(†) and L ≠ L(†) cases, in contrast to those evolution equations valid only for L = L(†) case in the literature. The derived equation that generalizes the quantum regression theorem (QRT) to the non-Markovian case will have broad applications in many different branches of physics. We then give conditions on which the QRT holds in the weak system-environment coupling case and apply the derived evolution equation to a problem of a two-level system (atom) coupled to the finite-temperature bosonic environment (electromagnetic fields) with L ≠ L(†).
This article reviews from both theoretical and numerical aspects three non-equivalent complete second-order formulations of quantum dissipation theory, in which both the reduced dynamics and the initial canonical thermal equilibrium are properly treated in the weak system-bath coupling limit. Two of these formulations are rather familiar as the time-local and the memory-kernel prescriptions, while another which can be termed as correlated driving-dissipation equations of motion will be shown to have the combined merits of the two conventional formulations. By exploiting the exact solutions to the driven Brownian oscillator system, we demonstrate that the time-local and correlated driving-dissipation equations of motion formulations are usually better than their memory-kernel counterparts, in terms of their applicability to a broad range of system-bath coupling, non-Markovian, and temperature parameters. Numerical algorithms are detailed for an efficient evaluation of both the reduced canonical thermal equilibrium state, and the non-Markovian evolution at any temperature, in the presence of arbitrary time-dependent external fields.