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The Journal of Physical Chemistry A

Real Gentile Statistical Systems: N-Annulenes

Yao Shen, Yulin Zhao

Published Jul 13, 2018• 2 citations
Publisher

Abstract

Gentile statistics, which is famous for its advantages in dealing with composite particle systems, is a kind of fractional statistics. Lately, researchers are concentrating on finding real systems that obey Gentile statistics. Five years ago, we discovered that the cyclic hydrocarbon polyenes called N-annulenes in the Hückel model had certain correspondence with Gentile oscillators. According to their rotation and dihedral symmetry, these two systems had the same energy levels and partition functions. In this paper, we give further discussions. We discuss the transformations of wave functions between N-annulenes and Gentile oscillators, the creation and annihilation operators in site pictures of N-annulenes, the coherent state, and the mathematical proofs of the intermediate commutation relations of operators. All of our works prove that N-annulenes in the Hückel model are real Gentile statistical systems and offer a new algebraic method to deal with the problems of electron-electron and electron-phonon interactions.

DOI
10.1021/acs.jpca.8b05121

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Gentile statistics, which is famous for its advantages in dealing with composite particle systems, is a kind of fractional statistics. Lately, researchers are concentrating on finding real systems that obey Gentile statistics. Five years ago, we discovered that the cyclic hydrocarbon polyenes called N-annulenes in the Hückel model had certain correspondence with Gentile oscillators. According to their rotation and dihedral symmetry, these two systems had the same energy levels and partition functions. In this paper, we give further discussions. We discuss the transformations of wave functions between N-annulenes and Gentile oscillators, the creation and annihilation operators in site pictures of N-annulenes, the coherent state, and the mathematical proofs of the intermediate commutation relations of operators. All of our works prove that N-annulenes in the Hückel model are real Gentile statistical systems and offer a new algebraic method to deal with the problems of electron-electron and electron-phonon interactions.
Abstract Gentile statistics describes fractional statistical systems in the occupation number representation. Anyon statistics researches those systems in the winding number representation. Both of them are intermediate statistics between Bose–Einstein and Fermi–Dirac statistics. The second quantization of Gentile statistics shows a lot of advantages. According to the symmetry requirement of the wave function and the property of braiding, we give the general construction of transformation between anyon and Gentile statistics. In other words, we introduce the second quantization form of anyons in an easier way. This construction is a correspondence between two fractional statistics and gives a new description of anyon. Basic relations of second quantization operators, the coherent state and Berry phase are also discussed.
After a brief mention of Bose and Fermi oscillators and of particles which obey other types of statistics, including intermediate statistics, parastatistics, paronic statistics, anyon statistics and infinite statistics, I discuss the statistics of ``quons'' (pronounced to rhyme with muons), particles whose annihilation and creation operators obey the qqq-deformed commutation relation (the quon algebra or q-mutator) which interpolates between fermions and bosons. I emphasize that the operator for interaction with an external source must be an effective Bose operator in all cases. To accomplish this for parabose, parafermi and quon operators, I introduce parabose, parafermi and quon Grassmann numbers, respectively. I also discuss interactions of non-relativistic quons, quantization of quon fields with antiparticles, calculation of vacuum matrix elements of relativistic quon fields, demonstration of the TCP theorem, cluster decomposition, and Wick's theorem for relativistic quon fields, and the failure of local commutativity of observables for relativistic quon fields. I conclude with the bound on the parameter qqq for electrons due to the Ramberg-Snow experiment.
Closed form, analytical results for the finite-temperature one-body density matrix, and Wigner function of a d -dimensional, harmonically trapped gas of particles obeying exclusion statistics are presented. As an application of our general expressions, we consider the intermediate particle statistics arising from the Gentile statistics, and compare its thermodynamic properties to the Haldane fractional exclusion statistics. At low temperatures, the thermodynamic quantities derived from both distributions are shown to be in excellent agreement. As the temperature is increased, the Gentile distribution continues to provide a good description of the system, with deviations only arising well outside of the degenerate regime. Our results illustrate that the exceedingly simple functional form of the Gentile distribution is an excellent alternative to the generally only implicit form of the Haldane distribution at low temperatures.
Identical quantum particles exhibit only two types of statistics: bosonic and fermionic. Theoretically, this restriction is commonly established through the symmetrization postulate or (anti)commutation constraints imposed on the algebra of creation and annihilation operators. The physical motivation for these axioms remains poorly understood, leading to various generalizations by modifying the mathematical formalism in somewhat arbitrary ways. In this work, we take an opposing route and classify quantum particle statistics based on operationally well-motivated assumptions. Specifically, we consider that a) the standard (complex) unitary dynamics defines the set of single-particle transformations, and b) phase transformations act locally in the space of multi-particle systems. We develop a complete characterization, which includes bosons and fermions as basic statistics with minimal symmetry. Interestingly, we have discovered whole families of novel statistics (dubbed transtatistics) accompanied by hidden symmetries, generic degeneracy of ground states, and spontaneous symmetry breaking – effects that are (typically) absent in ordinary statistics.
A new fundamental theory of composite particles in nonrelativistic many-body systems is developed. The theory is constructed making use solely of the physical Fock space for the basic elementary particles which comprise the many-body system. In this manner exchange symmetry in the elementary particles is exact. Physical composite particle creation and annihilation operators are introduced and these operators satisfy exact Bose (Fermi) commutation (anticommutati$\stackrel{\mathrm{\ifmmode \dot{}\else \.{}\fi{}}}{\mathrm{o}}$n) relations depending on whether the composites correspond to bosons or to fermions. Commuting physical occupation number operators for composite particles are then constructed in the usual manner from the composite creation and annihilation operators. These number operators are highly dressed in terms of the basic elementary particle operators. Finally, the foundations of statistical mechanics for bound composite particles are formulated in terms of the appropriate occupation number operators.