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Review of Scientific Instruments

Note: Pulsed optically pumped atomic clock based on a paraffin-coated cell

Haixiao Lin, Jianliao Deng, Jinda Lin, Song Zhang, Yao Hu, Yuzhu Wang

Published Jun 1, 2018• 4 citations
Publisher

Abstract

We report on the implementation of a pulsed optically pumped atomic clock based on a paraffin-coated cell. The relaxation times are measured, with the longitudinal relaxation time, T1 = 9.7 ± 0.4 ms, and the transversal relaxation time, T2 = 0.40 ± 0.03 ms. We demonstrated that the measured frequency stability of the clock is 3.9 × 10−13 τ−1/2 (1 s ≤ τ ≤ 100 s) and reaches a value of 3.1 × 10−14 for τ = 1000 s, where τ is the averaging time. This is an unprecedented result for a paraffin-coated vapor cell clock, and it makes significant contributions toward improving the performance of the wall-coated vapor cell atomic clock.

DOI
10.1063/1.5030956

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We report on the implementation of a pulsed optically pumped atomic clock based on a paraffin-coated cell. The relaxation times are measured, with the longitudinal relaxation time, T1 = 9.7 ± 0.4 ms, and the transversal relaxation time, T2 = 0.40 ± 0.03 ms. We demonstrated that the measured frequency stability of the clock is 3.9 × 10−13 τ−1/2 (1 s ≤ τ ≤ 100 s) and reaches a value of 3.1 × 10−14 for τ = 1000 s, where τ is the averaging time. This is an unprecedented result for a paraffin-coated vapor cell clock, and it makes significant contributions toward improving the performance of the wall-coated vapor cell atomic clock.
We have realized and studied a rubidium atomic frequency standard based on a paraffin-coated cell, exhibiting a short-term frequency stability <3 × 10−12 τ−1/2 between τ = 1 and 100 s. Characterization of the wall-coating is performed by measuring the T1 and T2 relaxation times. Perturbations of the medium- to long-term clock stability, due to variations in the laser-intensity, laser frequency, the microwave power shift, and the shifts due to temperature variations are measured and analyzed. A method for reducing the intensity light-shift by detuning the laser frequency and the resulting improvement in clock stability is demonstrated. This work is of relevance for further improvements on Rb cell standards using anti-relaxation wall-coating technology.
In this paper, we present the performance of a vapor-cell rubidium frequency standard working in the pulsed regime, in which the clock signal is represented by a Ramsey pattern observed on an optically detected laser absorption signal. The main experimental results agree with previously reported theoretical predictions. In particular, we measured a relative frequency stability of σy(τ) - 1.6 × 10(-13)τ-1/2 for integration times, τ, up to 200 s, which represents a record in short-term stability for a vapor-cell clock. We also discuss the most important physical phenomena that contribute to this result.
In this paper we discuss how to improve both short and medium-long term frequency stability of a vapor cell frequency standard working in pulsed regime. We propose in particular a multi-step pumping technique that is able to put almost all the atoms in one of the two clock levels, increasing in this way the signal-to-noise ratio with respect to the usual optical pumping made with a single laser pulse. Moreover, we discuss the phenomena affecting the medium-long term frequency stability and how it is possible to control them, making the overall clock stability compatible with sigmay(tau) =3x10-13tau-frac12for integration times up to tau = 105s.
In this paper we report the results we obtained with a prototype of pulsed optically pumped (POP) Rb clock. In terms of frequency stability, an Allan deviation σy(τ)=1.7 ×10-13τ-1/2has been measured, where τ is the integration time. In addition, the long term frequency drift results below 10-14/day. In the paper we also describe a technique to stabilize the amplitude of the microwave signal using the atoms themselves as discriminator. Moreover, an anomalously large temperature sensitivity of the clock frequency and a technique to keep it under control are also reported. Finally, we describe some non linear effects that modify the shape of the clock signal represented by the Ramsey central fringe.