Photon catalysis is a technique by which a readily available Gaussian state of light prepared in one mode is incident upon a beam splitter with a discrete number of photons, q, prepared in another mode; the resulting two-mode state is then subjected to single-photon resolving detection for q photons on one of the output modes. By employing beam splitters of different transmissivities and reflectivities, the subsequent single-mode state is shown to possess nonclassical properties such as quadrature squeezing and sub-Poissonian statistics. We consider the case in which the input state is the most general of pure single-mode Gaussian states: a squeezed coherent state. Noting the Gaussianity of the initial state, we demonstrate non-Gaussianity of the photon-catalyzed state by analyzing the quadrature uncertainty product and explicitly illustrate it through the Wigner quasi-probability distribution. We extend this technique to the two-mode squeezed states, whereby we perform photon catalysis on one mode of a two-mode squeezed vacuum state. The resulting correlated two-mode state may have applications in fundamental tests of quantum mechanics, such as violations of Bell’s inequalities, as the detection loophole can be closed due to the non-Gaussianity of the photon-catalyzed state. We also generalize our method to include state projective measurements for l≠q photons.
Photon catalysis is a technique by which a readily available Gaussian state of light prepared in one mode is incident upon a beam splitter with a discrete number of photons, q, prepared in another mode; the resulting two-mode state is then subjected to single-photon resolving detection for q photons on one of the output modes. By employing beam splitters of different transmissivities and reflectivities, the subsequent single-mode state is shown to possess nonclassical properties such as quadrature squeezing and sub-Poissonian statistics. We consider the case in which the input state is the most general of pure single-mode Gaussian states: a squeezed coherent state. Noting the Gaussianity of the initial state, we demonstrate non-Gaussianity of the photon-catalyzed state by analyzing the quadrature uncertainty product and explicitly illustrate it through the Wigner quasi-probability distribution. We extend this technique to the two-mode squeezed states, whereby we perform photon catalysis on one mode of a two-mode squeezed vacuum state. The resulting correlated two-mode state may have applications in fundamental tests of quantum mechanics, such as violations of Bell’s inequalities, as the detection loophole can be closed due to the non-Gaussianity of the photon-catalyzed state. We also generalize our method to include state projective measurements for l≠q photons.
Abstract Multiphoton catalysis is a non-Gaussian operation which has aroused interest recently in quantum information processing. There are two schemes of multiphoton catalysis in the current literature: one uses a beam splitter, while the other uses an optical parametric amplifier. We derive the catalysis operator in the Fock basis for each scheme and find a close relationship between them. We propose to enhance quantum entanglement of the two-mode squeezed vacuum state by performing two-mode multiphoton catalysis independently using two beam splitters. We calculate the optimal entanglement, which is maximized over two independent transmissivities, for the catalyzed states with various pairs of catalysis photon numbers, and find that in each case entanglement is enhanced only when the squeezing parameter is below a certain threshold. We also find that the optimal entanglement is nonzero in the limit of low squeezing, and deduce the analytical forms of the limiting catalyzed state and its entanglement in each case from numerical coefficients.
A new kind of non-Gaussian quantum catalyzed state is proposed via multiphoton measurements and two-mode squeezing as an input of thermal state. The characteristics of the generated multiphoton catalysis output state depends on the thermal parameter, catalyzed photon number and squeezing parameter. We then analyze the nonclassical properties by examining the photon number distribution, photocount distribution and partial negativity of the Wigner function. Our findings indicate that nonclassicality can be achieved through the implementation of multiphoton catalysis operations and modulated by the thermal parameter, catalyzed photon number and squeezing parameter.
Realistic non-Gaussian operations, which can be implemented by mixing a nonclassical Gaussian state with a Fock state at a beam splitter and then heralding on a photon-number-resolving detector, are known to improve phase estimation in a Mach-Zehnder interferometer. The existing studies have considered the single-mode squeezed vacuum for difference-intensity and parity detection, and the two-mode squeezed thermal state for parity detection alone as the initial Gaussian resources. However, a real squeezer in the lab actually produces single-mode squeezed thermal light, which has not been studied in a coherent-plus-resource interferometer. We take up this case and using the phase space Wigner picture, we obtain the heralded state produced by photon subtraction, addition and catalysis on a single-mode squeezed thermal resource, and evaluate the corresponding phase sensitivities. Single-photon catalysis, which is useless on squeezed vacuum, becomes a useful operation for any thermal occupation above $\nth\simeq0.2$, and since it heralds with a probability near one-half, it turns out to be the best success-weighted operation over the whole thermal range. In the vacuum limit our results reproduce the known hierarchy, where two-photon catalysis is the best operation. The quantum Fisher information computations confirms that thermal noise enhances the phase information encoded in the catalyzed state, demonstrating that difference-intensity detection closely approaches the ultimate precision bound across most operational regimes, and, together with a loss analysis, verifies the robustness of the effect.
We theoretically introduce a new kind of non-Gaussian state, namely, the mixture of multiphoton added thermal states, achieved through multiphoton measurements at one output port of the beam splitter (termed multiphoton catalysis) for thermal state input. We discuss the success probabilities of detection (the normalization factors). Furthermore, we investigate their nonclassical properties based on the nonclassical depth, photon number distribution, and photocount distribution. It is shown that the multiphoton catalysis presents a better nonclassical performance by controlling the thermal parameter, catalyzed photon number and the transmissivity of the beam splitter. In addition, the nonclassicality is further examined through the partial negativity of the Wigner function, which reveals that multiphoton catalysis operation can prepare highly nonclassical quantum states. These results indicate that the preparation of a non-Gaussian states may have potential applications in the realms of quantum information processing and quantum metrology.
We highlight some of our research done in the fields of quantum optical interferometry and quantum state engineering. We discuss the body of work for which our research is predicated, as well as discuss some of the fundamental tenants of the theory of phase estimation. We do this in the context of quantum optical interferometry where our primary interest lies in the calculation of the quantum Fisher information as it has been shown that the minimum phase uncertainty obtained, the quantum Cramer-Rao bound, is saturated by parity-based detection methods. We go on to show that the phase uncertainty one obtains through the quantum Fisher information is in agreement with the error propagation calculus when using parity as a detection observable. We also introduce a technique through which one can generate new non-classical single and two-mode states of light known as photon catalysis. This involves a projective measurement made at the output of a beam splitter with variable transmittance, for 'l' photons, where our initial state is a tensor product between a single-mode field state and a number state comprised of 'q' photons. We close the paper with a discussion on a proposed state-projective scheme for generating pair coherent states using existing and readily available technology.
Abstract Based on an asymmetrical beam splitter (ABS) and conditional measurement, we have investigated the nonclassical properties of non-Gaussian states in a unified form, including photon subtraction, photon addition and quantum catalysis, by deriving analytical expressions for photon number, squeezing effect, Mandel Q parameter and Wigner function. It is found that these properties not only depend on squeezing parameter and measurement, but also on the transmissivity of the ABS. Photon addition and quantum catalysis present a higher probability in the regions of low and high transmissivity, respectively. Although both single-photon subtraction and addition share a clear negative volume, the latter is considered to be a better choice for producing nonclassical states than the two others, if both success probability and negative volume in the small squeezing region are taken into consideration. Quantum catalysis is better in the large squeezing region and with low transmissivity. These results provide some reference for generating such non-Gaussian states.