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SPIE Conference on Nonlinear Optics and its Applications

Effect of temperature on the absorption of rubidium vapor cell D2 line studied by two-photon absorption spectroscopy

Prathan Buranasiri, Nut Thanaboonrungroch, Witoon Yindeesuk, Pichet Limsuwan

Published May 14, 2018• 1 citation
Publisher

Abstract

In this research, the effect of temperature on the absorption of rubidium vapor cell D2 line was studied by Two-photon absorption spectroscopy. The diameter and length of cylindrical rubidium vapor cell used in this research are 25.65 mm and 82.12 mm, respectively. The temperature of rubidium cell was varied from room temperature to approximately 80 °C using a peltier-thermoelctric module. The laser diode at 778 nm was used as a light source for two-photon absorption spectroscopy. The absorption spectra of rubidium D2 hyperfine transitions were recorded in the range of 200-1100 nm .The results show that the absorption peak at high temperature is higher than that of lower temperature.

DOI
10.1117/12.2306747

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Journal of the Physical Society of Japan•Jul 18, 2018•7 citations
In this research, the effect of temperature on the absorption of rubidium vapor cell D2 line was studied by Two-photon absorption spectroscopy. The diameter and length of cylindrical rubidium vapor cell used in this research are 25.65 mm and 82.12 mm, respectively. The temperature of rubidium cell was varied from room temperature to approximately 80 °C using a peltier-thermoelctric module. The laser diode at 778 nm was used as a light source for two-photon absorption spectroscopy. The absorption spectra of rubidium D2 hyperfine transitions were recorded in the range of 200-1100 nm .The results show that the absorption peak at high temperature is higher than that of lower temperature.
We have constructed a simplified setup for the demonstration of laser cooling and trapping of rubidium atoms. An external-cavity diode laser was swept across the F = 3 → F' = 2, 3, 4 resonances of the D 2 -line of 85 Rb at 780 nm to resolve the saturated absorption features. Subsequently, the transition F = 3 → F' = 4 was used to cool rubidium atoms in a roomtemperature vapor cell. A cold cloud of trapped atoms with a diameter of approximately 1 mm was produced. The lifetime of the trap was measured to be 1 second.
Recently we demonstrated lasing at 420 nm and 455 nm inside of rubidium and cesium vapor cells respectively, by non-resonant, two photon absorption at near infrared pump wavelengths. Two photon absorption from the ground S1/2 state to excited D3/2,5/2 or higher lying S1/2 state via virtual states and subsequent infrared stimulated emission pumps the upper laser levels, the second excited P1/2,3/2 states. To better understand the mechanism and phenomenology of this type of laser, this paper presents a method for determining the two-photon absorption (TPA) cross-section for the 5S1/2 −→ 5D5/2 transition in naturally occurring rubidium. For an incident pump intensity of 392 W cm2 and a rubidium concentration of 3.34 × 10 atoms cm3 , a peak absorbance of 0.10 is observed. The concentration of the Rb in the test cell is determined by one photon absorption spectra of the D2, indicating a vapor curve shifted by 14 C from the exterior wall temperature. The incident laser beam is focused to a waist of 75 μm. The beam quality is consistent with an M = 1.05 − 1.09. A model for the intensity as a function of propagation distance is developed to interpret the observed absorption spectrum and determine a cross-section for the two photon absorption.
Abstract Glass cells containing neutral atoms are commonly employed in spectroscopy experiments and have potential applications in metrology. The temperature of the vapor plays a vital role as it directly influences the absorption rate of rubidium atoms. In this research, we study the effect of vapor temperature on the absorption spectrum of rubidium atoms. We observed the broadening of the spectral line and increased absorption, enabling us to determine the absorbance of atoms within the cell. These results provide valuable insights for our future work to characterize absorbance of homemade vapor cells for portable quantum device applications.
Abstract We theoretically and experimentally investigate the Doppler-broadened absorption spectrum of the D2-line (52 S 1/2 → 52 P 3/2) in thermal (room-temperature) Rb vapour over a wide range of probe intensity, probe diameter, and vapour cell temperature to understand the effect of hyperfine pumping and transit-relaxation on the absorption lineshape. We present a relatively simple but comprehensive five-level rate equation model which incorporates optical pumping of the atomic population into the other ‘dark’ ground hyperfine level (leading to absorption saturation), including contributions of the three closely spaced (within one Doppler linewidth) hyperfine levels in the excited state 52 P 3/2 (allowed by the dipole transition selection rules). D2-line transmission spectra predicted by our model show excellent agreement (rms error < 5 % ) with the experimental data for a wide range of probe intensities (from ∼ 0.001 I s a t 0 all the way up to ∼ 10 I s a t 0 , where I sat0 is the usual two-level saturation intensity for the respective atomic transition), vapour cell temperatures (24.2°C–53.5 °C) and beam diameters (1/e 2 width ∼ 1 − 6 mm). Our model also takes into account the finite transit time of atoms across the probe beam cross-section, and correctly predicts the dependence of effective saturation intensity on probe diameter (up to ∼ 10 × lower saturation intensity as compared to I sat0 for few-mm beam sizes). This ab initio five-level model can thus predict accurate Doppler lineshapes for any given experimental parameter set for a linearly polarized probe without any fitting parameters, and can be easily applied to any other atomic system by an appropriate change of the atomic constants in the rate equations.
A 64.4% reduction in absorption at the rubidium D2 line is observed when a pumping field at 775.8 nm is tuned on resonance to the transition between the excited states 5P3/2{\mathit{P}}_{3/2}P3/2​ and 5D5/2{\mathit{D}}_{5/2}D5/2​. As the pumping field is tuned off resonance, an absorption peak appears at the side of the Doppler-broadened D2 line. This modification in absorption is related to pumping-induced atomic coherence in this three-level ladder-type system. This experiment is done in a Rb vapor cell at room temperature and with cw diode lasers for both pumping and probe beams in a Doppler-free configuration.
We experimentally study the high-resolution two-photon spectroscopy of rubidium using a single laser. The 5S1/2 − 5P3/2 − 5D5/2 transition is realized via 778.1 nm laser beams acting on the vapor with a counter-propagating configuration. The intensity modulation method is employed to improve the signal-to-noise ratio of the spectrum by two orders of magnitude compared with that for direct measurement. The effects of the vapor temperature, the frequency-scanning speed of the laser, the polarization combination of the laser beams, and the laser power on the spectra are investigated to obtain the optimal experimental parameters. This research is expected to be beneficial for potential applications since it can be used to realize a compact and high-precision frequency standard for optical communication.