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Physical Review A

Observation of an electromagnetically induced change of absorption in multilevel rubidium atoms

Yongqing Li, Shaozheng Jin, Min Xiao

Published Mar 1, 1995• 64 citations
Publisher

Abstract

A 64.4% reduction in absorption at the rubidium D2 line is observed when a pumping field at 775.8 nm is tuned on resonance to the transition between the excited states 5${\mathit{P}}_{3/2}$ and 5${\mathit{D}}_{5/2}$. As the pumping field is tuned off resonance, an absorption peak appears at the side of the Doppler-broadened D2 line. This modification in absorption is related to pumping-induced atomic coherence in this three-level ladder-type system. This experiment is done in a Rb vapor cell at room temperature and with cw diode lasers for both pumping and probe beams in a Doppler-free configuration.

DOI
10.1103/physreva.51.r1754

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Measurement of Dispersive Properties of Electromagnetically Induced Transparency in Rubidium Atoms

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The dispersive properties of the atomic transition in the rubidium ${D}_{2}$ line ($5{S}_{\frac{1}{2}}\ensuremath{-}5{P}_{\frac{3}{2}}$) at 780.0 nm are measured with a Mach-Zehnder interferometer when an additional coupling field at 775.8 nm is applied to an upper transition ($5{P}_{\frac{3}{2}}\ensuremath{-}5{D}_{\frac{5}{2}}$). This ladder-type system is observed to exhibit electromagnetically induced transparency together with a rapidly varying refractive index. A reduction in group velocity for the probe beam (${v}_{g}=\frac{c}{13.2}$) is inferred from the measured dispersion curve with 52.5% suppressed absorption on resonance.

Physical Review Letters•Jan 30, 1995•731 citations
A 64.4% reduction in absorption at the rubidium D2 line is observed when a pumping field at 775.8 nm is tuned on resonance to the transition between the excited states 5P3/2{\mathit{P}}_{3/2}P3/2​ and 5D5/2{\mathit{D}}_{5/2}D5/2​. As the pumping field is tuned off resonance, an absorption peak appears at the side of the Doppler-broadened D2 line. This modification in absorption is related to pumping-induced atomic coherence in this three-level ladder-type system. This experiment is done in a Rb vapor cell at room temperature and with cw diode lasers for both pumping and probe beams in a Doppler-free configuration.
An electromagnetically induced transparency is observed at one arm of a three-level \ensuremath{\Lambda}-type system in a rubidium D1 line (794.8 nm) with an 85% reduction in absorption, when a pumping field is present at the other arm. This reduction in absorption for the weak probe field is due to the atomic coherence produced by the strong pumping field. This experiment is done in a Rb vapor cell at room temperature with cw diode lasers for both pumping and probe beams in a Doppler-free configuration. A simple theoretical treatment including Doppler broadening is in good qualitative agreement with the experimental measurement.
Doppler broadening presents a major limitation for high-resolution spectroscopy and nonlinear optics in room-temperature atomic vapors. Here, we demonstrate the suppression of Doppler broadening accompanied by pronounced absorption on the upper transition of a three-level ladder system, achieved by dressing the intermediate state with a strong control field. As a concrete realization, we study a hot vapor of 87^{87}87Rb where the lower transition is driven by a strong control field resonant with the D2 line at a wavelength of 780 nm, while a weak counter-propagating probe field at the telecom C-band wavelength of 1529 nm (5P(3/2)↔4D(5/2)5P_{(3/2)}\leftrightarrow 4D_{(5/2)}5P(3/2)​↔4D(5/2)​) interrogates the dressed states. We observe absorption features with a resonant optical depth of approximately 4 and a full width at half maximum of about 17 MHz. Remarkably, this corresponds to an order-of-magnitude reduction relative to the Doppler width, while the optical depth on the upper transition of the ladder scheme exceeds that of the Doppler-broadened lower transition. The measured spectra are in good agreement with theoretical modeling. Combining high optical density with sub-Doppler-width absorption lines typically requires laser-cooled atoms, while our approach profits from the experimental simplicity of a hot-vapor platform.
Laser spectroscopy experiments are reported on rubidium atoms by using two or three external cavity diode lasers to study multiple resonance transitions in Λ- and V-type systems as well as on (Λ+V)-type system. Electromagnetically induced transparency (EIT) peaks having sub-natural line-widths are found on the Doppler broadened transmission backgrounds with velocity selective enhanced absorption dips. In the presence of a pump laser, probe spectrum shows enhancement of EIT signal by tuning the control laser frequency when the Λ- and V-type EIT signals are made to overlap. Theoretical analysis is carried out by solving the optical Bloch equations for five-level atomic model under Λ configuration. With the numerically simulated spectra, variation of EIT transmission peak with ground state decay rate and excited state spontaneous decay rate are investigated. Effect of pump Rabi frequency on the transmission peak is also shown.
A comprehensive study of three-photon electromagnetically induced transparency (EIT) and absorption (EIA) on the rubidium cascade $5{S}_{1/2}\ensuremath{\rightarrow}5{P}_{3/2}$ (laser wavelength 780 nm), $5{P}_{3/2}\ensuremath{\rightarrow}5{D}_{5/2}$ (776 nm), and $5{D}_{5/2}\ensuremath{\rightarrow}28{F}_{7/2}$ (1260 nm) is performed. The 780-nm probe and 776-nm dressing beams are counteraligned through a Rb room-temperature vapor cell, and the 1260-nm coupler beam is co- or counteraligned with the probe beam. Several cases of EIT and EIA, measured over a range of detunings of the 776-nm beam, are studied. The observed phenomena are modeled by numerically solving the Lindblad equation, and the results are interpreted in terms of the probe-beam absorption behavior of velocity- and detuning-dependent dressed states. Interaction-time effects are discussed. To explore the utility of three-photon Rydberg EIA and EIT for microwave electric-field diagnostics, a sub-THz field generated by a signal source and a frequency quadrupler is applied to the Rb cell. The 100.633-GHz field resonantly drives the $28{F}_{7/2}\ensuremath{\leftrightarrow}29{D}_{5/2}$ transition and causes Autler-Townes splittings in the Rydberg EIA and EIT spectra, which are measured and employed to characterize the performance of the microwave quadrupler.
We report on three-photon electromagnetically induced absorption (TPEIA) due to three-photon coherence in ladder-type atomic systems for the 5S1/25{S}_{1/2}5S1/2​-5P3/25{P}_{3/2}5P3/2​-5D5/25{D}_{5/2}5D5/2​ transition in Rb atoms. When a counterpropagating coupling field was added to the typical ladder-type electromagnetically induced transparency (EIT) experiment, both EIT and two-photon absorption (TPA) switched to TPEIA. Considering three-photon coherence in a Doppler-broadened three-level ladder-type atomic system, the spectrum of the switch from EIT and TPA to TPEIA was numerically calculated and could be understood by decomposing the calculated spectrum into two-photon coherence and three-photon coherence components.
The dispersive properties of the atomic transition in the rubidium D2{D}_{2}D2​ line ($5{S}_{\frac{1}{2}}\ensuremath{-}5{P}_{\frac{3}{2}}$) at 780.0 nm are measured with a Mach-Zehnder interferometer when an additional coupling field at 775.8 nm is applied to an upper transition ($5{P}_{\frac{3}{2}}\ensuremath{-}5{D}_{\frac{5}{2}}$). This ladder-type system is observed to exhibit electromagnetically induced transparency together with a rapidly varying refractive index. A reduction in group velocity for the probe beam (vg=c13.2{v}_{g}=\frac{c}{13.2}vg​=13.2c​) is inferred from the measured dispersion curve with 52.5% suppressed absorption on resonance.