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Semiconductor Lasers and Laser Dynamics

An analytical approach to collective effects in nanolasers (Conference Presentation)

Emil C. André, Игорь Евгеньевич Проценко, Alexander V. Uskov, Jesper Mørk, Martijn Wubs

Published May 23, 2018• 0 citations
Publisher

Abstract

Traditionally, the active material in a laser is modelled as independent emitters, but in recent years it has become increasingly clear that radiative coupling between emitters can significantly change the characteristics of small lasers. Collective effects in free space such as superradiance have been studied extensively [1,2], but the effects of inter-emitter correlation in micro- and nano-cavities need further examination to be put on firm theoretical ground. Several studies of collective effects in nano-cavities have been made [3-6], but the theoretical models employed are intricate, and numerical methods are needed both to generate the dynamic equations and to solve them. We propose a model where the complexity is strongly reduced, allowing analytical solutions [7]. We consider a collection of identical two-level emitters interacting with a single cavity mode. We start from Maxwell-Bloch equations, but instead of making the typical adiabatic elimination of the polarization, we allow the polarization decay rate to be of the same magnitude or smaller than other decay rates. Hence, the traditional laser rate equations for the photon number and the population inversion must be supplemented by equations for the emitter-field correlation and the emitter-emitter correlation. This gives us four generalized laser rate equations, which we solve analytically in steady state. Comparing with the steady state results obtained from the traditional laser rate equations we see that inclusion of collective effects leads to a reduction of the photon number for small pump rates, similarly to what is found in [4]. From the generalized laser rate equations, we derive a measure of the strength of collective effects in terms of laser parameters: This describes the difference between results with and without inter-emitter correlations, and it goes smoothly to zero as we approach parameter values where the traditional laser rate equations become valid. To gain insight into the photon statistics of the laser, we construct dynamic equations for higher order correlations of operators. We derive an analytical expression for the zero-delay photon auto-correlation function, and for low pump rates we find that the interaction of emitters results in super-thermal values of the auto-correlation. This feature is observed in experiments and numerical models [4-5], and with our analytical expressions, we are able to pinpoint the parameter combinations for which the collective effects have the largest impact. Considering the same model in terms of the Fourier components of the operators, we find results for the photon number that agree well with the previous approach, while allowing computation of the linewidth. Thus, we can examine how emitter-emitter correlation affects the line broadening of the laser.

DOI
10.1117/12.2307100

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Traditionally, the active material in a laser is modelled as independent emitters, but in recent years it has become increasingly clear that radiative coupling between emitters can significantly change the characteristics of small lasers. Collective effects in free space such as superradiance have been studied extensively [1,2], but the effects of inter-emitter correlation in micro- and nano-cavities need further examination to be put on firm theoretical ground. Several studies of collective effects in nano-cavities have been made [3-6], but the theoretical models employed are intricate, and numerical methods are needed both to generate the dynamic equations and to solve them. We propose a model where the complexity is strongly reduced, allowing analytical solutions [7]. We consider a collection of identical two-level emitters interacting with a single cavity mode. We start from Maxwell-Bloch equations, but instead of making the typical adiabatic elimination of the polarization, we allow the polarization decay rate to be of the same magnitude or smaller than other decay rates. Hence, the traditional laser rate equations for the photon number and the population inversion must be supplemented by equations for the emitter-field correlation and the emitter-emitter correlation. This gives us four generalized laser rate equations, which we solve analytically in steady state. Comparing with the steady state results obtained from the traditional laser rate equations we see that inclusion of collective effects leads to a reduction of the photon number for small pump rates, similarly to what is found in [4]. From the generalized laser rate equations, we derive a measure of the strength of collective effects in terms of laser parameters: This describes the difference between results with and without inter-emitter correlations, and it goes smoothly to zero as we approach parameter values where the traditional laser rate equations become valid. To gain insight into the photon statistics of the laser, we construct dynamic equations for higher order correlations of operators. We derive an analytical expression for the zero-delay photon auto-correlation function, and for low pump rates we find that the interaction of emitters results in super-thermal values of the auto-correlation. This feature is observed in experiments and numerical models [4-5], and with our analytical expressions, we are able to pinpoint the parameter combinations for which the collective effects have the largest impact. Considering the same model in terms of the Fourier components of the operators, we find results for the photon number that agree well with the previous approach, while allowing computation of the linewidth. Thus, we can examine how emitter-emitter correlation affects the line broadening of the laser.
We study the stationary photon output and statistics of small lasers. Our closed-form expressions clarify the contribution of collective effects due to the interaction between quantum emitters. We generalize laser rate equations and explain photon trapping: a decrease of the photon number output below the lasing threshold, derive an expression for the stationary cavity mode autocorrelation function g2g_2g2​, which implies that collective effects may strongly influence the photon statistics. We identify conditions for coherent, thermal and superthermal radiation, the latter being a unique fingerprint for collective emission in lasers. These generic analytical results agree with recent experiments, complement numerical results, and provide insight into and design rules for nanolasers.
The laser has evolved from table size apparatuses to truly nano sized devices, in much the same way that computer chips have been continuously minimized. The few-emitter nanolaser represents an extreme in terms of size. The emitters can be either atoms or quantum dots, and they are coupled to a high-Q optical cavity. This system has previously been studied for the one and two emitters case, see e.g. [1, 2]. The emitters and cavity are modelled as two-level systems and a harmonic oscillator, respectively. The coupled system is modelled using the Jaynes-Cummings Hamiltonian and the two-level systems are pumped incoherently by a rate P. Solutions are found using the corresponding master equation. However, with cavity populations exceeding 100 and several emitters, the dimension of the Hilbert space of the system becomes too large to handle efficiently on a conventional computer. E.g. for four emitters and 100 photon states the density matrix has more than 2.5 × 106 elements. We have been able to simplify the problem significantly by adiabatically eliminating the photon-assisted polarizations and the correlations between emitters and cavity [3]. This results in a set of rate equations for the population of the cavity, na, and the occupation of the emitters. Fig. 1a) shows na for up to 4 emitters coupled to a cavity, as a function of the pumping rate P. The figure also shows results from a full master equation solution, and the correspondence is very good for large values of P. In Fig. 1b) the second order correlation functions g(2)(0) are shown, as obtained using the full model. The second order correlation functions become 1 for sufficiently large values of P signifying the onset of lasing. However, for larger values of P the laser quenches and the emission becomes chaotic (g(2)(0) = 2). This quenching effect is well-known in two-level models [3], but might not be realistic for semiconductor quantum dots. A proposed application for these nanolasers is in on-chip optical interconnects. In this application the modulation bandwidth is important. We have calculated the modulation bandwidth using a small-signal analysis of the rate equations, which has the advantage compared the full model of yielding a semianalytical result. The results are shown in Fig. 1c). The nanolaser has a high bandwidth, which is mostly limited by the cavity lifetime (/ 1/), but shows a prominent drop during the lasing regime. The modulation bandwidth again becomes limited by as the output becomes chaotic.
Based on a rate equation model for single-mode two-level lasers, two algorithms for stochastically simulating the dynamics and steady-state behaviour of micro- and nanolasers are described in detail. Both methods lead to steady-state photon numbers and statistics characteristic of lasers, but one of the algorithms is shown to be significantly more efficient. This algorithm, known as Gillespie's first reaction method (FRM), gives up to a thousandfold reduction in computation time compared to earlier algorithms, while also circumventing numerical issues regarding time-increment size and ordering of events. The FRM is used to examine intra-cavity photon distributions, and it is found that the numerical results follow the analytics exactly. Finally, the FRM is applied to a set of slightly altered rate equations, and it is shown that both the analytical and numerical results exhibit features that are typically associated with the presence of strong inter-emitter correlations in nanolasers.
Based on a rate equation model for single-mode two-level lasers, two algorithms for stochastically simulating the dynamics and steady-state behaviour of micro- and nanolasers are described in detail. Both methods lead to steady-state photon numbers and statistics characteristic of lasers, but one of the algorithms is shown to be significantly more efficient. This algorithm, known as Gillespie's First Reaction Method (FRM), gives up to a thousandfold reduction in computation time compared to earlier algorithms, while also circumventing numerical issues regarding time-increment size and ordering of events. The FRM is used to examine intra-cavity photon distributions, and it is found that the numerical results follow the analytics exactly. Finally, the FRM is applied to a set of slightly altered rate equations, and it is shown that both the analytical and numerical results exhibit features that are typically associated with the presence of strong inter-emitter correlations in nanolasers.
Summary form only given. The interaction strength of light and matter can be greatly influenced by altering the environment of the emitters and the electric field. In a photonic cavity the emitter-field coupling strength may become sufficiently large that the emitters and the field can exchange an excitation multiple times before it decays, giving rise to Rabi oscillations. In a passive cavity with one (several) two-level emitter(s), this manifests itself as a (collective) Rabi splitting of the transmissions spectrum [1-3], and it has recently been shown that incoherently pumped single emitters in cavities may exhibit Rabi splitting of the emission spectrum at large coupling strengths [4,5]. We present a fully analytical model describing a large collection of incoherently pumped two-level emitters in a single-mode cavity (e.g. quantum dots in a nano-cavity) and show that collective Rabi splitting of the emission spectrum can occur in these systems as well [6]. We derive a condition in terms of system parameters for the splitting to occur, and show that this is different from the condition typically associated with strong emitter-field coupling. Moreover, we show that the collective Rabi splitting decreases with increasing pump rate P, giving a transition from the strong-coupling regime to the weak-coupling regime, and possibly lasing at large P (Fig. 1(a)).
We analytically calculate the optical emission spectrum of nanolasers and nano-LEDs based on a model of many incoherently pumped two-level emitters in a cavity. At low pump rates, we find two peaks in the spectrum for large coupling strengths and numbers of emitters. We interpret the double-peaked spectrum as a signature of collective Rabi splitting, and discuss the difference between the splitting of the spectrum and the existence of two eigenmodes. We show that an LED will never exhibit a split spectrum, even though it can have distinct eigenmodes. For systems where the splitting is possible, we show that the two peaks merge into a single one when the pump rate is increased. Finally, we compute the linewidth of the systems, and discuss the influence of inter-emitter correlations on the lineshape.