Can the most "classical-like" of all quantum states, namely the Schrödinger coherent state of a harmonic oscillator, exhibit nonclassical behavior? We find that for an oscillating object initially in a coherent state, merely by observing at various instants which spatial region the object is in, the Leggett-Garg inequality (LGI) can be violated through a genuine negative result measurement, thereby repudiating the everyday notion of macrorealism. This violation thus reveals an unnoticed nonclassicality of the very state which epitomizes classicality within the quantum description. It is found that for any given mass and oscillator frequency, a significant quantum violation of LGI can be obtained by suitably choosing the initial peak momentum of the coherent state wave packet. It thus opens up potentially the simplest way (without coupling with any ancillary quantum system or using nonlinearity) for testing whether various recently engineered and sought after macroscopic oscillators, such as feedback cooled thermal trapped nanocrystals of ∼10^{6}-10^{9} amu mass, are indeed bona fide nonclassical objects.
Can the most "classical-like" of all quantum states, namely the Schrödinger coherent state of a harmonic oscillator, exhibit nonclassical behavior? We find that for an oscillating object initially in a coherent state, merely by observing at various instants which spatial region the object is in, the Leggett-Garg inequality (LGI) can be violated through a genuine negative result measurement, thereby repudiating the everyday notion of macrorealism. This violation thus reveals an unnoticed nonclassicality of the very state which epitomizes classicality within the quantum description. It is found that for any given mass and oscillator frequency, a significant quantum violation of LGI can be obtained by suitably choosing the initial peak momentum of the coherent state wave packet. It thus opens up potentially the simplest way (without coupling with any ancillary quantum system or using nonlinearity) for testing whether various recently engineered and sought after macroscopic oscillators, such as feedback cooled thermal trapped nanocrystals of ∼10^{6}-10^{9} amu mass, are indeed bona fide nonclassical objects.
The Leggett-Garg inequality (LGI), based on the notions of realism and noninvasive measurability, is applied in the context of a linear harmonic oscillator. It is found that merely through observing at various instants which region of the potential well, the oscillating quantum object is in, the LGI can be violated without taking recourse to any ancillary quantum system. Strikingly, this violation reveals an unexplored nonclassicality of the state which is considered the most "classical-like" of all quantum states, namely the Schrödinger coherent state. In the macrolimit, the extent to which such nonclassicality persists for large values of mass and classical amplitudes of oscillation is quantitatively investigated. It is found that while for any given mass and oscillator frequency, a significant quantum violation of LGI can be obtained by suitably choosing the initial peak momentum of the coherent state wave packet, as the mass is sufficiently increased, actual observability of this violation becomes increasingly difficult. A feasible experimental setup for testing the predicted quantum mechanical violation of LGI is suggested using a trapped nano-object of ∼106−109 amu mass.
In an endeavor to better define the distinction between classical macroscopic and quantum microscopic regimes, the Leggett-Garg inequalities were established as a test of macroscopic-realistic theories, which are commonly thought to be a suitable class of descriptions for classical dynamics. The relationship between their violation and nonclassicality is however not obvious. We show that classical states of light, which in the quantum optical sense are any convex sums of coherent states, may not satisfy the Leggett-Garg inequalities. After introducing a simple Mach-Zehnder setup and showing how to obtain a violation with a single photon using negative measurements, we focus on classical states of light, in particular those of low average photon number. We demonstrate how one can still perform negative measurements with an appropriate assignment of variables, and show that the inequalities are violable with coherent states. Finally, we abandon the initial phase reference and demonstrate that the violation is still possible, in particular with thermal states of light, and we investigate the effect of intermediate dephasing.
Macrorealism posits that a system possesses definite properties at all times and that we can discover these properties, in principle, without disturbing the system's subsequent behavior. The Leggett-Garg inequalities are derived under these assumptions and are readily violated by standard quantum mechanics, thereby providing a scheme to test whether demonstrably macroscopic systems can exhibit quantum coherence. Unfortunately, Leggett-Garg tests suffer from the difficult to avoid clumsiness loophole: the difficulty of proving that sequential measurements have not inadvertently disturbed the system. The recently uncovered Tsirelson inequality is derived from the simple dynamical assumption of uniform precession, obeyed by many classical systems, and requires only single-time measurements. However, Tsirelson inequality violations could be explained by a macrorealistic system that merely breaks the dynamical assumption, rather than genuine quantum behavior. By carrying out a quantum-mechanical analysis of the Tsirelson inequality in the harmonic oscillator, we develop a protocol to rule out this possibility by assessing generalized conditions of uniform precession. We show that various measures of uniform precession, some of which are related to Leggett-Garg quantities, are satisfied well enough that the presence of quantum-mechanical interference terms must be implied. We derive several incidental mathematical results relating to violating states of Tsirelson's inequality, concerning dwell time, crossing number, and probability currents, and also consider a group-theoretic analysis of the Tsirelson operator.
The Leggett-Garg (LG) inequalities were introduced to test for the possible presence of macroscopic quantum coherence. Since such effects may be found in various types of macroscopic oscillators, we consider the application of the LG approach to the one-dimensional quantum harmonic oscillator and also to more general bound systems, using a single dichotomic variable Q given by the sign of the oscillator position. We present a simple method to calculate the temporal correlation functions appearing in the LG inequalities for any bound system for which the eigenspectrum is (exactly or numerically) known. We apply this result to the quantum harmonic oscillator for a variety of experimentally accessible states, namely, energy eigenstates, and superpositions thereof. For the subspace of states spanned by only the ground state and first excited state, we readily find substantial regions of parameter space in which the LG inequalities at two, three, and four times can each be independently violated or satisfied. We also find that the violations persist, although are reduced, when the sign function defining Q is smeared to reflect experimental imprecision. For higher-energy eigenstates, we find that LG violations diminish, showing the expected classicalization. With a Q defined using a more general type of position coarse graining, we find two-time LG violations even in the ground state. We also show that two-time LG violations in a Gaussian state are readily found if the dichotomic variable at one of the times is taken to be the parity operator. To demonstrate the versatility of the approach, we repeat much of the LG analysis for the Morse potential, finding qualitatively similar physical results.
While quantum theory has been tested to an incredible degree on microscopic scales, quantum effects are seldom observed in our everyday macroscopic world. The curious results of applying quantum mechanics to macroscopic objects are perhaps best illustrated by Erwin Schrödinger's famous thought experiment, where a cat can be put into a superposition state of being both dead and alive. Obviously, these quantum predictions are in stark contradiction to our common experience. Even with plenty of theoretical explanations put forward to explain this discrepancy, a large number of questions about the frontier between the quantum and the classical world remain unanswered. To distinguish between classical and quantum behavior, two fundamental concepts inherent to classical physics have been established over the years: The world view of local realism limits the power of classical experiments to establish correlations over space, while the world view of macroscopic realism (or macrorealism) restricts temporal correlations. Necessary conditions for both world views have been formulated in the form of Bell and Leggett-Garg inequalities, and Bell inequalities have been shown to be violated by quantum mechanics through increasingly conclusive experiments. Furthermore, many challenging steps towards convincing violations of macrorealism have been taken in a number of recent experiments. In the first part of this thesis, conditions for macrorealism are analyzed in detail. Two necessary conditions for macrorealism, the original Leggett-Garg inequality and the recently proposed no-signaling in time condition, are presented. It is then shown that a combination of no-signaling in time conditions is not only necessary but also sufficient for the existence of a macrorealistic description. Finally, an operational formulation of no-signaling in time, in terms of positive-operator valued measurements and Hamiltonians, is derived. In the next part, we argue that these results lead to a suitable definition of classical behavior. In particular, we provide a formalism to judge the classicality of measurements and time evolutions. We then proceed to apply it to a number of exemplary measurement operators and Hamiltonians. Finally, we argue for the importance of spontaneously realized Hamiltonians in our intuition of classical behavior. Next, differences between local realism and macrorealism are analyzed. For this purpose, the probability polytopes for spatially and temporally separated experiments are compared, and a fundamental difference in the power of quantum mechanics to build both types of correlations is discovered. This result shows that Fine's theorem, which states that a set of Bell inequalities is necessary and sufficient for local realism, is not transferable to macrorealism. Thus, (Leggett-Garg) inequalities are in principle not well-suited for tests of macrorealism, as they can never form a necessary and sufficient condition, and unnecessarily restrict the violating parameter space. No-signaling in time is both better suited and more strongly motivated from the underlying physical theory. In the final part of this thesis, a concrete experimental setup for implementing quantum experiments with macroscopic objects is proposed. It consists of a superconducting micro-sphere in the Meißner state, which is levitated by magnetic fields. Through its expelled magnetic field, the sphere's center-of-mass motion couples to a superconducting quantum circuit. Properly tuned, ground state cooling can be realized, since the sphere's motion is extremely well isolated from the surrounding environment. This setup therefore is a promising candidate for the observation of quantum effects in macroscopic systems.
This thesis investigates three aspects of nonclassicality. The first aspect is macroscopic quantumness, a field which considers the properties of macroscopic superpositions. The various measures of macroscopicity are reviewed. An optomechanical system is described which enables us to study nonclassicality in macroscopic mechanical oscillators. We analyse the impact of different measurement settings on the macroscopicity of the mirror and the Wigner functions of the mechanical state. The same system is also considered under open system dynamics. The second nonclassical concept is the violation of macrorealism. It is shown that a two-level system can violate the Leggett-Garg inequality, thereby demonstrating that the assumptions of macrorealism do not hold. Similar dynamics are then replicated in a macroscopic mechanical system through the use of a hybrid optomechanical system in which an atom interacts with the mechanical oscillator through an optical mode. Mechanical damping is then factored into the dynamics to examine its effect on the violation of the Leggett-Garg inequality for different parameter ranges. The third is nonclassical correlations. Quantum discord and quantum entanglement are defined and several measures are explained. Entanglement distribution via separable states is introduced and then built on by adding imperfections to the operations in the protocol. It is found that the protocol is still successful in spite of the errors in the operations, both when they are unitary and non-unitary. We also develop a method of generating entanglement between two bosons through mediation with two spin systems. Through this system we demonstrate the creation of both entangled coherent states and NOON states.