In an endeavor to better define the distinction between classical macroscopic and quantum microscopic regimes, the Leggett-Garg inequalities were established as a test of macroscopic-realistic theories, which are commonly thought to be a suitable class of descriptions for classical dynamics. The relationship between their violation and nonclassicality is however not obvious. We show that classical states of light, which in the quantum optical sense are any convex sums of coherent states, may not satisfy the Leggett-Garg inequalities. After introducing a simple Mach-Zehnder setup and showing how to obtain a violation with a single photon using negative measurements, we focus on classical states of light, in particular those of low average photon number. We demonstrate how one can still perform negative measurements with an appropriate assignment of variables, and show that the inequalities are violable with coherent states. Finally, we abandon the initial phase reference and demonstrate that the violation is still possible, in particular with thermal states of light, and we investigate the effect of intermediate dephasing.
In an endeavor to better define the distinction between classical macroscopic and quantum microscopic regimes, the Leggett-Garg inequalities were established as a test of macroscopic-realistic theories, which are commonly thought to be a suitable class of descriptions for classical dynamics. The relationship between their violation and nonclassicality is however not obvious. We show that classical states of light, which in the quantum optical sense are any convex sums of coherent states, may not satisfy the Leggett-Garg inequalities. After introducing a simple Mach-Zehnder setup and showing how to obtain a violation with a single photon using negative measurements, we focus on classical states of light, in particular those of low average photon number. We demonstrate how one can still perform negative measurements with an appropriate assignment of variables, and show that the inequalities are violable with coherent states. Finally, we abandon the initial phase reference and demonstrate that the violation is still possible, in particular with thermal states of light, and we investigate the effect of intermediate dephasing.
Can the most "classical-like" of all quantum states, namely the Schrödinger coherent state of a harmonic oscillator, exhibit nonclassical behavior? We find that for an oscillating object initially in a coherent state, merely by observing at various instants which spatial region the object is in, the Leggett-Garg inequality (LGI) can be violated through a genuine negative result measurement, thereby repudiating the everyday notion of macrorealism. This violation thus reveals an unnoticed nonclassicality of the very state which epitomizes classicality within the quantum description. It is found that for any given mass and oscillator frequency, a significant quantum violation of LGI can be obtained by suitably choosing the initial peak momentum of the coherent state wave packet. It thus opens up potentially the simplest way (without coupling with any ancillary quantum system or using nonlinearity) for testing whether various recently engineered and sought after macroscopic oscillators, such as feedback cooled thermal trapped nanocrystals of ∼10^{6}-10^{9} amu mass, are indeed bona fide nonclassical objects.
According to the world view of macrorealism, the properties of a given system exist prior to and independent of measurement, which is incompatible with quantum mechanics. Leggett and Garg put forward a practical criterion capable of identifying violations of macrorealism, and so far experiments performed on microscopic and mesoscopic systems have always agreed with quantum mechanics. However, a macrorealist can always assign the cause of such violations to the perturbation that measurements effect on such small systems, and hence a definitive test would require using noninvasive measurements, preferably on macroscopic objects, where such measurements seem more plausible. However, the generation of truly macroscopic quantum superposition states capable of violating macrorealism remains a big challenge. In this work we propose a setup that makes use of measurements on the polarization of light, a property that has been extensively manipulated both in classical and quantum contexts, hence establishing the perfect link between the microscopic and macroscopic worlds. In particular, we use Leggett-Garg inequalities and the criterion of no signaling in time to study the macrorealistic character of light polarization for different kinds of measurements, in particular with different degrees of coarse graining. Our proposal is noninvasive for coherent input states by construction. We show for states with well-defined photon number in two orthogonal polarization modes, that there always exists a way of making the measurement sufficiently coarse grained so that a violation of macrorealism becomes arbitrarily small, while sufficiently sharp measurements can always lead to a significant violation.
Despite the great success of quantum mechanics, questions regarding its application still exist and the boundary between quantum and classical mechanics remains unclear. Based on the philosophical assumptions of macrorealism and noninvasive measurability, Leggett and Garg devised a series of inequalities (LG inequalities) involving a single system with a set of measurements at different times. Introduced as the Bell inequalities in time, the violation of LG inequalities excludes the hidden-variable description based on the above two assumptions. We experimentally investigated the single photon LG inequalities under decoherence simulated by birefringent media. These generalized LG inequalities test the evolution trajectory of the photon and are shown to be maximally violated in a coherent evolution process. The violation of LG inequalities becomes weaker with the increase of interaction time in the environment. The ability to violate the LG inequalities can be used to set a boundary of the classical realistic description.
While quantum theory has been tested to an incredible degree on microscopic scales, quantum effects are seldom observed in our everyday macroscopic world. The curious results of applying quantum mechanics to macroscopic objects are perhaps best illustrated by Erwin Schrödinger's famous thought experiment, where a cat can be put into a superposition state of being both dead and alive. Obviously, these quantum predictions are in stark contradiction to our common experience. Even with plenty of theoretical explanations put forward to explain this discrepancy, a large number of questions about the frontier between the quantum and the classical world remain unanswered. To distinguish between classical and quantum behavior, two fundamental concepts inherent to classical physics have been established over the years: The world view of local realism limits the power of classical experiments to establish correlations over space, while the world view of macroscopic realism (or macrorealism) restricts temporal correlations. Necessary conditions for both world views have been formulated in the form of Bell and Leggett-Garg inequalities, and Bell inequalities have been shown to be violated by quantum mechanics through increasingly conclusive experiments. Furthermore, many challenging steps towards convincing violations of macrorealism have been taken in a number of recent experiments. In the first part of this thesis, conditions for macrorealism are analyzed in detail. Two necessary conditions for macrorealism, the original Leggett-Garg inequality and the recently proposed no-signaling in time condition, are presented. It is then shown that a combination of no-signaling in time conditions is not only necessary but also sufficient for the existence of a macrorealistic description. Finally, an operational formulation of no-signaling in time, in terms of positive-operator valued measurements and Hamiltonians, is derived. In the next part, we argue that these results lead to a suitable definition of classical behavior. In particular, we provide a formalism to judge the classicality of measurements and time evolutions. We then proceed to apply it to a number of exemplary measurement operators and Hamiltonians. Finally, we argue for the importance of spontaneously realized Hamiltonians in our intuition of classical behavior. Next, differences between local realism and macrorealism are analyzed. For this purpose, the probability polytopes for spatially and temporally separated experiments are compared, and a fundamental difference in the power of quantum mechanics to build both types of correlations is discovered. This result shows that Fine's theorem, which states that a set of Bell inequalities is necessary and sufficient for local realism, is not transferable to macrorealism. Thus, (Leggett-Garg) inequalities are in principle not well-suited for tests of macrorealism, as they can never form a necessary and sufficient condition, and unnecessarily restrict the violating parameter space. No-signaling in time is both better suited and more strongly motivated from the underlying physical theory. In the final part of this thesis, a concrete experimental setup for implementing quantum experiments with macroscopic objects is proposed. It consists of a superconducting micro-sphere in the Meißner state, which is levitated by magnetic fields. Through its expelled magnetic field, the sphere's center-of-mass motion couples to a superconducting quantum circuit. Properly tuned, ground state cooling can be realized, since the sphere's motion is extremely well isolated from the surrounding environment. This setup therefore is a promising candidate for the observation of quantum effects in macroscopic systems.
In contrast to the spatial Bell's inequalities which probe entanglement between spatially separated systems, the Leggett–Garg inequalities test the correlations of a single system measured at different times. Violation of a genuine Leggett–Garg test implies either the absence of a realistic description of the system or the impossibility of measuring the system without disturbing it. Quantum mechanics violates the inequalities on both accounts and the original motivation for these inequalities was as a test for quantum coherence in macroscopic systems. The last few years has seen a number of experimental tests and violations of these inequalities in a variety of microscopic systems such as superconducting qubits, nuclear spins, and photons. In this article, we provide an introduction to the Leggett–Garg inequalities and review these latest experimental developments. We discuss important topics such as the significance of the non-invasive measurability assumption, the clumsiness loophole, and the role of weak measurements. Also covered are some recent theoretical proposals for the application of Leggett–Garg inequalities in quantum transport, quantum biology and nano-mechanical systems.