By trapping a single atom in a Fabry-Perot cavity, we can realize strong coupling
between the atom and the electromagnetic field, which may in the future be utilized
to perform quantum gates in quantum computing. Previous experiments with
Cesium atoms at the Caltech Quantum Optics group achieved a trapping time of
3 seconds, and they led to a detailed study of the atom-photon interactions known as
the vacuum-Rabi splitting. It is believed that the trapping time is limited by collisions
with residual gas molecules inside the vacuum chamber. I report three designs
for the piezoelectric-controlled cavity mirror mount, bakeable to a temperature above
250 °C and hence more desirable for deployments in ultra-high vacuum (UHV). I also
present new procedures which I have helped to develop for cavity construction and
the characterization of cavities. In addition, I consider cavity birefringence, which
can present complications to our experiments because a birefringent cavity supports
two orthogonal, nondegenerate modes. I developed a simple model of cavity birefringence
and made our first attempt to actively induce birefringence by stressing the
cavity mirrors with piezoelectric materials, although we have not yet been able to
demonstrate control over cavity birefringence. Nonetheless, with expected improvements
in both mechanical stability of the cavity and base pressure of the system, it
is hoped that a longer trapping time of 30 seconds can be achieved and that the new
experiment with a single-sided cavity can lead to further studies of the dynamics of
atom-photon interactions.
By trapping a single atom in a Fabry-Perot cavity, we can realize strong coupling
between the atom and the electromagnetic field, which may in the future be utilized
to perform quantum gates in quantum computing. Previous experiments with
Cesium atoms at the Caltech Quantum Optics group achieved a trapping time of
3 seconds, and they led to a detailed study of the atom-photon interactions known as
the vacuum-Rabi splitting. It is believed that the trapping time is limited by collisions
with residual gas molecules inside the vacuum chamber. I report three designs
for the piezoelectric-controlled cavity mirror mount, bakeable to a temperature above
250 °C and hence more desirable for deployments in ultra-high vacuum (UHV). I also
present new procedures which I have helped to develop for cavity construction and
the characterization of cavities. In addition, I consider cavity birefringence, which
can present complications to our experiments because a birefringent cavity supports
two orthogonal, nondegenerate modes. I developed a simple model of cavity birefringence
and made our first attempt to actively induce birefringence by stressing the
cavity mirrors with piezoelectric materials, although we have not yet been able to
demonstrate control over cavity birefringence. Nonetheless, with expected improvements
in both mechanical stability of the cavity and base pressure of the system, it
is hoped that a longer trapping time of 30 seconds can be achieved and that the new
experiment with a single-sided cavity can lead to further studies of the dynamics of
atom-photon interactions.
Cavity quantum electrodynamic system with strongly coupled single atoms provides a good platform for studying quantum information processing, quantum simulation, quantum network, and distributed quantum computing. Cooling and trapping single atoms is a crucial technique in the quantum technology. At present, in a high-finesse cavity with finite space, cooling and trapping single atoms is a big challenge, even though it is a mature technique for free space. Great efforts have been made to cool and trap single atoms inside a cavity, and for a trapped atom its lifetime has reached as long as tens of seconds. Developing a more flexible method of cooling and trapping single atoms in a cavity is still essential for a strongly coupled cavity quantum electrodynamic system. In this work, we demonstrate experimentally that a single cesium atom in a cavity can be trapped by utilizing a single optical tweezer settled in cavity mode, and its lifetime is (2.60 ± 0.18) s. The experiment is carried out in a Fabry-Perot cavity, which is assembled by two concave mirrors each with a curvature radius of 100 mm, and cavity length of 335 μm. The concave surfaces are highly reflective, and the cavity has a finesse of 6.1 × 104. The 1080 nm optical tweezer with a waist of 2 μm is formed by an achromatic lens group with a numerical aperture of 0.4. At first, the precooled atomic assemble released from the magneto-optical trap (MOT) is transferred into cavity mode by an optical dipole trap with a waist of 36 μm. Then, one of the successfully transferred atoms is captured by the optical tweezer with the aid of cavity cooling mechanism. A blue detuned cavity locking laser is used as a standing-wave optical trap along the cavity axis. The signal of successfully trapped one atom is obtained by recording transmission of the cavity that will decrease owing to the strong coupling induced vacuum Rabi splitting. Finally, we demonstrate the precise manipulation of the atom-cavity coupling strength, which is achieved by scanning the position of the trapped atom step by step by using a high-precision translation stage. The system realized in this work can be used to study the dynamics of single atom-photon interactions with adjustable coupling strength. In addition, the mechanism adopted in this work is compatible with constructing tweezer arrays inside cavity mode, and thus possesses more flexibility and great potentials in cavity-based quantum entanglement and quantum simulation.
In recent years, remarkable advances in the science of laser cooling and trapping of atomic samples have lead to breakthroughs in quantum optics and, in particular, in cavity quantum electrodynamics (QED). The ability to optically trap an atom within the mode of a ultra-high finesse cavity of small mode volume for experimentally significant periods of time now allows for the continuous observation of fundamental quantum optical effects. This dissertation will focus on experiments conducted to fully characterize and exert quantum control over a strongly-coupled atom-cavity system consisting of single cesium atoms isolated by a dipole trapping in the mode of a Fabry-Perot optical resonator. In particular, we describe techniques developed and implemented for exerting coherent control over the internal and quantum motional state of these atoms using stimulated Raman processes. We also focus on the applications of this system to quantum networking and quantum information science, particularly within the context of coherently transferring quantum states from atom to quantum optical fields and back. Finally, we describe a series of measurements carried out to explore the characteristic dynamics of the Jaynes-Cummings Hamiltonian which governs the system. This includes spectroscopic measurement of the signature vacuum Rabi splitting for strongly-coupled cavity QED as well as evidence in the time domain for coherent Rabi nutation of excitation between atom and field on resonance.
Cavity quantum electrodynamics (cavity QED) describes electromagnetic fields in a confined space and the radiative properties of atoms in such fields. The simplest example of such system is a single atom interacting with one mode of a high-finesse resonator. Besides observation and exploration of fundamental quantum mechanical effects, this system bears a high potential for applications quantum information science such as, e.g., quantum logic gates, quantum communication and quantum teleportation. In this thesis I present an experiment on the deterministic coupling of a single neutral atom to the mode of a high-finesse optical resonator. In Chapter 1 I describe our basic techniques for trapping and observing single cesium atoms. As a source of single atoms we use a high-gradient magneto-optical trap, which captures the atoms from background gas in a vacuum chamber and cools them down to millikelvin temperatures. The atoms are then transferred without loss into a standing-wave dipole trap, which provides a conservative potential required for experiments on atomic coherence such as quantum information processing and metrology on trapped atoms. Moreover, shifting the standing-wave pattern allows us to deterministically transport the atoms (Chapter 2). In combination with non-destructive fluorescence imaging of individual trapped atoms, this enables us to control their position with submicrometer precision over several millimeters along the dipole trap. The cavity QED system can distinctly display quantum behaviour in the so-called strong coupling regime, i.e., when the coherent atom-cavity coupling rate dominates dissipation in the system. This sets the main requirements on the resonator's properties: small mode volume and high finesse. Chapter 3 is devoted to the manufacturing, assembling, and testing of an ultra-high finesse optical Fabry-Perot resonator, stabilized to the atomic transition. In Chapter 4 I present the transportation of single atoms into the cavity and their coupling to the cavity mode. The strong coupling manifests itself in a strong reduction of the cavity transmission probed by a weak external laser. The atoms remain trapped and coupled to the cavity mode for several seconds until we move them out of the cavity for final analysis of their number and position.
A single two-level emitter coupled to a single mode of an electromagnetic resonator constitutes the most fundamental instance of light--matter interaction. Realizations of this type of system are investigated in the field of cavity quantum electrodynamics (cavity QED). Particularly important are schemes in which the coupling is strong enough to exceed the spontaneous emission rate as well as cavity damping. In this case, the coherent exchange of excitation between source and photon is the dominating process, providing the unique possibility to deterministically control the quantum evolution of the system. Great progress has recently been accomplished, technologically as well as conceptually, and the focus section in this issue of Journal of Optics B: Quantum and Semiclassical Optics features five articles highlighting important recent developments in the field. Strong coupling between single atoms and the electromagnetic cavity field have been achieved in two distinct regimes, the optical and the microwave region. The latter is represented by the micromaser, a high-Q microwave cavity pumped by a beam of highly excited Rydberg atoms. It has proved to be an almost ideal system for the generation of non-classical field states. A constraint in these experiments is the fact that the field inside the cavity can only be examined indirectly, by analysing the occupation of atoms leaving the cavity. While only two atomic states were previously identified for this purpose, V A Reshetov shows in his article (pages 119--126) that more information on the field may be extracted by taking advantage of the Zeeman substructure of the atomic levels. In the optical domain of cavity QED, by contrast, the state of the resonator field may be probed directly by measuring the light leaking from the cavity using photodetectors. In order to minimize damping, high-quality cavities must be employed. In most optical experiments these are Fabry--Perot resonators with ultra-high reflectivity mirrors, with losses as low as a few parts per million being state of the art. At the same time, the coupling of atoms and photons is enhanced by reducing the length of the cavity, so that strong coupling conditions are reached. A very attractive application of this type of cavity QED setup is the possibility of exerting control over the quantum dynamics of the system. An impressive example is the implementation of quantum feedback, reported in the paper by W P Smith and L A Orozco (pages 127--134). Using information gained from detecting a single photon escaping from the cavity, active feedback is applied to halt the dynamical evolution of the system. This is the first time active feedback has been used to modify the quantum evolution of a system at the single-photon level. The authors discuss how detunings between the subsystems affect the quantum feedback, an issue particularly relevant for ensembles of atoms with a spread in detuning. Perfect quantum feedback in this case requires the use of additional parameters to control the system. The majority of optical cavity QED experiments performed so far have used as a medium atoms traversing the cavity on random trajectories, such as, for example, thermal atomic beams. In this case, the observation of quantum effects is degraded in two ways. The Doppler effect and the finite transit time lead to line broadening, while the spatial structure of the cavity mode results in atoms in different locations experiencing different coupling with the photonic field. J E Reiner et al (pages 135--142) investigate the impact of these effects on quantum fluctuations in their cavity QED system. In order to overcome line broadening, they have developed a continuous cold atomic beam, extracted from a magneto-optical trap. An even better control of broadening effects and fluctuating coupling strength is provided by trapping the atoms inside the cavity and cooling them to temperatures at which their position spread is smaller than the optical wavelength. Much recent activity has been devoted to developing such an ultimate cavity QED system. A Vukics et al (pages 143--153) present a theoretical proposal for dynamically trapping and cooling atoms inside a cavity. By driving the atoms with a standing wave injected from the side of the cavity and by weakly exciting the cavity field itself, they predict three-dimensional trapping of the atom for periods around 1 second, an extremely long time on the typical scale of cavity QED dynamics. The essential component of their scheme is the interference between the two driving fields, determining the temperature of the particle and the stable trapping positions. In the quest for better confinement of radiation, lately, an appealing alternative to the Fabry--Perot cavity has been investigated -- the optical microsphere resonator. A sphere with a diameter of a few tens of microns, it supports so-called whispering gallery modes near its circumference, for which quality factors up to 10 10 have been measured. In order to exploit the correspondingly low field damping rates for cavity QED, a method must be found to couple atomic or solid state emitters to these modes. S Göotzinger et al (pages 154--158) report the coupling of single nanocrystals on the surface of a microsphere through the evanescent field of the mode. Selective excitation of a single nano-emitter was accomplished with a scanning confocal microscope. The system is a promising candidate for cavity QED with single-quantum emitters. The ability to fully control the quantum dynamics of atoms and light is beginning to spawn early applications. The most notable example is quantum information processing. This requires the coherent manipulation of single-quantum systems, which is ideally provided by cavity QED interaction in the strong-coupling limit. The development of practical devices will be among the principal future tasks for research in the field. This will include physical systems, which have not been covered in this issue, such as semiconductors, quantum dots as emitters, or photonic crystals as resonator structures. Cavity QED is therefore guaranteed to remain a vigorous field in the years to come.
The experiments discussed in this thesis focus on the interaction of a single trapped atom with the single mode of a high-finesse optical cavity, in the regime of strong coupling. Chapter 1 gives a brief introduction, after which Chapter 2 describes our recent measurements of the transmission spectrum of the atom-cavity system. The spectrum exhibits a clearly resolved vacuum-Rabi splitting, in good quantitative agreement with theoretical predictions. A new Raman scheme for cooling atomic motion along the cavity axis enables a complete spectrum to be recorded for an individual atom trapped within the cavity mode, in contrast to all previous measurements of this type that have required averaging over 10^3-10^5 atoms. Chapter 3 discusses our observations of photon blockade for the transmitted light in the presence of one trapped atom. Excitation of the atom-cavity system by a first photon blocks the transmission of a second one, thereby converting an incident Poissonian stream of photons into a sub-Poissonian, anti-bunched stream, as confirmed by measurements of the photon statistics of the transmitted field. The intensity correlations of the cavity transmission also reveal the energy distribution for oscillatory motion of the trapped atom. Chapter 4 details a set of simple but necessary measurements of relevant experimental parameters such as cavity geometry, linewidth, mirror properties, birefringence, and detection efficiency. The thesis concludes with Appendix A, describing the efficient laser setup we use for our magneto-optical traps.
Cavity quantum electrodynamics (QED) in the strong-coupling regime provides the opportunity to monitor and control the dynamics of a simple quantum system. A single Cesium atom interacts strongly with single-photon fields in the mode of a high-finesse optical cavity. When the resulting coherent coupling rate dominates dissipation in the system, strong coupling is realized and the system displays distinctively quantum behavior. The coupling between atomic internal states and the quantized cavity field allows for diverse protocols in quantum state preparation, quantum communication, and quantum logic. However, the atom's external or motional state must also be taken into account. My research develops cavity QED in the limit where the coherent atom-field coupling dominates the atomic kinetic energy and thus significantly affects the atomic center-of-mass motion. In this regime, the interaction of the atom with the cavity field provides both a means of controlling atomic motion and a signal for detecting that motion in real time with high signal-to-noise. The sensing capability of the ``atom-cavity microscope" is exploited to trap single atoms with single-photon fields and to monitor their orbits in real time as they are bound in the cavity. Such real-time position sensing is the basis for a detailed strategy and ongoing experiment to actively stabilize select aspects of an atom's motion within the cavity. As the cavity-enabled position measurement approaches the standard quantum limit, this work begins to realize a quantum servo for atomic position and to address questions of optimal state estimation and state preparation. In combination with other progress in cavity QED, it furthers the goal of controlled atom-field interactions for quantum information science.