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Atmospheric and Oceanic Optics

Amplified Spontaneous Emission on Sodium D-lines Using Nonresonant Optical Pumping

Timofey D. Petukhov, Gennadiy S. Evtushenko, Evgeny N. Telminov

Published Jan 1, 2018• 3 citations
Publisher

Abstract

We describe experiments on the excitation of amplified spontaneous emission on the D -lines of sodium ( D 2 = 588.9 nm; D 1 = 589.6 nm) with longitudinal optical pumping with a large detuning from the D 2 line toward shorter wavelengths. The radiation spectra are measured, showing gain on both lines, at a Na concentration of (1–5) × 10 14 cm –3 , buffer gas (helium) pressure of 600 Torr at the working temperature, and pumping power density of more than 1.5 MW/cm 2 . The time characteristics show that the output radiation varies versus the concentration of sodium atoms in the active medium. The dependences of radiation absorption at the D -lines of sodium on the concentration of Na atoms and buffer gas pressure are given.

DOI
10.1134/s102485601801013x

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We describe experiments on the excitation of amplified spontaneous emission on the D -lines of sodium ( D 2 = 588.9 nm; D 1 = 589.6 nm) with longitudinal optical pumping with a large detuning from the D 2 line toward shorter wavelengths. The radiation spectra are measured, showing gain on both lines, at a Na concentration of (1–5) × 10 14 cm –3 , buffer gas (helium) pressure of 600 Torr at the working temperature, and pumping power density of more than 1.5 MW/cm 2 . The time characteristics show that the output radiation varies versus the concentration of sodium atoms in the active medium. The dependences of radiation absorption at the D -lines of sodium on the concentration of Na atoms and buffer gas pressure are given.
Coherent emission on the 3 P –3 S resonance transition ( D line) of nonresonantly excited sodium atoms in a buffer gas atmosphere is studied experimentally and theoretically. Both forward and backward coherent emission on the D lines is observed relative to the propagation direction of a pump beam whose frequency is blue-shifted from resonance. The divergence of the emitted radiation does not exceed that of the pump beam. The emission is due to the population inversion created on the “operating” transition when the pump is far detuned from resonance and the buffer gas pressure is sufficiently high. It is found that both emission intensity and the detuning range where this phenomenon is observed increase with the buffer gas pressure.
Lasing at the resonance transitions ( D 1− and D 2− lines) of sodium was observed in the superradiance mode upon nonresonance optical excitation in the presence of a buffer gas. The dependences of the lasing intensity on the exciting radiation intensity and on the detuning of its frequency from the frequencies of resonance transitions were studied. It is found that, under specific conditions of the experiment (high pressure of a buffer gas and a rather high radiation intensity), in the case of a large positive detuning of the exciting radiation frequency from the resonance (“working”) transition frequency, the population inversion is produced at the “ working” transition, which results in lasing.
Lasing on the sodium resonance transitions (D1 and D2 lines) at the superluminosity regime was observed upon the nonresonance excitation in the presence of a buffer gas. Dependences of the lasing intensity on the pump radiation intensity and its frequency detuning from the frequencies of resonance transitions were examined. It was found that under the specific experimental conditions (high buffer gas pressure, sufficiently high intensity of pump radiation) upon the large positive frequency detuning of pump radiation with respect to the frequency of resonance (working) transition, contrary to ingrained conceptions, population inversion for the working transition is raised. That results in observed phenomena.
The highly selective Na3 + Br reaction creates a continuous electronic population inversion on Na2 transitions which demonstrates optical gain through stimulated emission in regions close to 527, 492, and 460 nm ((alpha) equals 8 X 10-3 cm-1 for an individual rotational level at approximately 527 nm). With a focus to increasing amplifier gain length and amplifying medium concentration (conversion to oscillator), we extend these initial studies employing the intersection of sodium and bromine flows formed from slit source expansions to create an extended reaction-amplification zone. Initial results with this extended reaction zone provide the first example of chemically induced Raman pumping. Unique Raman signals are induced by and correlate with emission from the NaD-line components (D1, D2) formed in the chemical reaction zone primarily as a result of the Na2 + Br yields Na* (3P) + NaBr reaction. The NaD-line emitters interact with cooled sodium dimers in a resonance Raman scattering process, for which computer simulation of the experimentally observed spectra predict an unusually large scattering linewidth close to 4 cm-1. We describe initial laser based studies on a pure sodium expansion to probe the mechanism of the unusually strong Raman scattering and to understand the origin of the large scattering linewidth. These experiments demonstrate that the Raman process can be induced only upon excitation of the NaD-line components, the Raman scattering being insufficient or nonexistent for wavelength shifts (Delta) (lambda) > 1 nm from the D lines. The scattering linewidth for the reactive process is not readily correlated with the line-broadening of the NaD-line and may result from the nature of the Na- Na2 interaction in the reactive environment. Initial double pass measurements indicate the possibility of optical gain associated with the Raman process.