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Physical Review A

Single-photon superradiant beating from a Doppler-broadened ladder-type atomic ensemble

Yoon‐Seok Lee, Sang Min Lee, Heonoh Kim, Han Seb Moon

Published Dec 22, 2017• 16 citations
Publisher

Abstract

We report on heralded-single-photon superradiant beating in the spontaneous four-wave mixing process of Doppler-broadened ladder-type $^{87}\mathrm{Rb}$ atoms. When Doppler-broadened atoms contribute to two-photon coherence, the detection probability amplitudes of the heralded single photons are coherently superposed despite inhomogeneous broadened atomic media. Single-photon superradiant beating is observed, which constitutes evidence for the coherent superposition of two-photon amplitudes from different velocity classes in the Doppler-broadened atomic ensemble. We present a theoretical model in which the single-photon superradiant beating originates from the interference between wavelength-separated two-photon amplitudes via the reabsorption filtering effect.

DOI
10.1103/physreva.96.063832

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We report on heralded-single-photon superradiant beating in the spontaneous four-wave mixing process of Doppler-broadened ladder-type 87Rb^{87}\mathrm{Rb}87Rb atoms. When Doppler-broadened atoms contribute to two-photon coherence, the detection probability amplitudes of the heralded single photons are coherently superposed despite inhomogeneous broadened atomic media. Single-photon superradiant beating is observed, which constitutes evidence for the coherent superposition of two-photon amplitudes from different velocity classes in the Doppler-broadened atomic ensemble. We present a theoretical model in which the single-photon superradiant beating originates from the interference between wavelength-separated two-photon amplitudes via the reabsorption filtering effect.
With a recent rising interest of single photon superradiance due to its potential usefulness for efficient collection of single photon from an atomic ensemble, bright and narrow photon pair source is a key component in realization of quantum communication and quantum computer based on coherent interaction between light and atomic ensemble. We report the superradiant emission of ultra-bright photon pairs with a coincidence counting rate per input power of 64,600 cps/mW via spontaneous four-wave mixing in a thermal vapour cell. The photon-pair generation rate is enhanced by the contribution of two-photon coherence of almost atomic velocity groups in the Doppler-broadened ladder-type atomic system. The quadratic proportionality of the probability of detecting a heralded single photon as a function of the optical depth clarifies that the ultra-brightness results from the superradiance. In addition, a single photon superradiant beating at a high optical depth of the atomic ensemble is observed for the first time.
We experimentally demonstrate nonlocal two-photon interference of energy-time entangled photon pairs via spontaneous four-wave mixing (SFWM) process in Doppler-broadened ladder-type 87Rb^{87}\mathrm{Rb}87Rb atoms. The Doppler-broadened ladder-type atomic system offers collective two-photon coherence which results in strong temporal correlation between the entangled photons. The spacelike separated photon pairs clearly show nonlocal two-photon interference with high visibility of $97.1\ifmmode\pm\else\textpm\fi{}2.5%$, which violates the Bell-CHSH (Clauser-Horne-Shimony-Holt) inequality by 10.5 standard deviations, in which the travel time of a single-photon towards the interferometer is much longer than the coincidence window. Our work will provide an atom-based entangled photon source which is applicable for long distance atom-memory-based quantum communication.
To realize a quantum network based on quantum entanglement swapping, bright and completely autonomous sources are essentially required. Here, we experimentally demonstrate Hong-Ou-Mandel (HOM) quantum interference between two independent bright photon pairs generated via the spontaneous four-wave mixing in Doppler-broadened ladder-type 87Rb atoms. Bright autonomous heralded single photons are operated in a continuous-wave (CW) mode with no synchronization or supplemental filters. The four-fold photon coincidence counts per hour correspond to 5000 events for a temporal range of 10 ns, one order higher than those of previously reported for autonomous single photons. We observe an HOM dip with 83% visibility with the two autonomous heralded single photons for an effective measurement time of 900 s. The achievement of the HOM interference between the two bright autonomous photon-pair sources has made an important step towards a practical scalable quantum network.
We experimentally demonstrate two-photon interference of a time-energy entangled photon pair generated via collective two-photon coherence in Doppler-broadened cascade-type ^{87}Rb atoms. The two photons originally proposed by J. D. Franson are realized as a photon pair due to collective effects, which are generated from the cascade atomic system with a relatively long lifetime of the initial state and a considerably shorter lifetime of the intermediate state. The achievement of two-photon interference with photon-pair sources generated from inhomogeneous atomic ensembles constitutes an important result for time-energy entanglement based on an atom-photon interaction.
We study dressed-atom two-photon resonant nondegenerate four-wave mixing (NFWM) in a Doppler-broadened system. It is found that there exists interference between the macroscopic field polarizations from different ensembles of atoms within the atomic velocity distribution. This polarization interference can cause significant modification of the NFWM spectra. We also show that two-photon resonant NFWM in dressed atoms can be employed as a new type of Doppler-free high-resolution Autler-Townes spectroscopy for measuring transition dipole moments between two highly excited atomic states.
We report a polarization-entangled photon-pair source obtained via spontaneous four-wave mixing (SFWM) in a Doppler-broadened atomic ensemble of ^{87}Rb atoms using a Sagnac interferometer. Collective two-photon coherence occurs in the Doppler-broadened ladder-type atomic system with bidirectional counterpropagating two-photon resonant pump and coupling fields; hence, polarization-entangled photon pairs are collectively radiated in the phase-matched direction. Without phase stabilization of the interferometry for polarization entanglement, we robustly produce all four Bell states via a polarization Sagnac configuration. The brightness, stability, and temporal purity advantages provided by our polarization-entangled SFWM photon-pair source have very important applications in the context of a practical scalable quantum network.