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Physical Review A

Generation of high-dimensional energy-time-entangled photon pairs

Da Zhang, Yiqi Zhang, Xinghua Li, Dan Zhang, Lin Cheng, Changbiao Li, Yanpeng Zhang

Published Nov 22, 2017• 25 citations
Publisher

Abstract

High-dimensional entangled photon pairs have many excellent properties compared to two-dimensional entangled two-photon states, such as greater information capacity, stronger nonlocality, and higher security. Traditionally, the degree of freedom that can produce high-dimensional entanglement mainly consists of angular momentum and energy time. In this paper, we propose a type of high-dimensional energy-time-entangled qudit, which is different from the traditional model with an extended propagation path. In addition, our method mainly focuses on the generation with multiple frequency modes, while two- and three-dimensional frequency-entangled qudits are examined as examples in detail through the linear or nonlinear optical response of the medium. The generation of high-dimensional energy-time-entangled states can be verified by coincidence counts in the damped Rabi oscillation regime, where the paired Stokes--anti-Stokes wave packet is determined by the structure of resonances in the third-order nonlinearity. Finally, we extend the dimension to $N$ in the sequential-cascade mode. Our results have potential applications in quantum communication and quantum computation.

DOI
10.1103/physreva.96.053849

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High-dimensional entangled photon pairs have many excellent properties compared to two-dimensional entangled two-photon states, such as greater information capacity, stronger nonlocality, and higher security. Traditionally, the degree of freedom that can produce high-dimensional entanglement mainly consists of angular momentum and energy time. In this paper, we propose a type of high-dimensional energy-time-entangled qudit, which is different from the traditional model with an extended propagation path. In addition, our method mainly focuses on the generation with multiple frequency modes, while two- and three-dimensional frequency-entangled qudits are examined as examples in detail through the linear or nonlinear optical response of the medium. The generation of high-dimensional energy-time-entangled states can be verified by coincidence counts in the damped Rabi oscillation regime, where the paired Stokes--anti-Stokes wave packet is determined by the structure of resonances in the third-order nonlinearity. Finally, we extend the dimension to NNN in the sequential-cascade mode. Our results have potential applications in quantum communication and quantum computation.
Summary form only given. Entanglement is a fundamental resource for the quantum processing of information and to study the intrinsic nature of quantum correlations. Entangling higher dimensional bipartite systems (qudits) has been shown to give more insight on the nature of entanglement compared to the simplest entanglement system composed of two two level systems (two qubits) [1, 2]. For quantum key distribution, increasing the dimension of the alphabet by using qudits increases the effective bit rate of the protocol, still being secure [3]. Experimentally, higher dimensional entanglement in photonic systems have been demonstrated for various degrees of freedom of light, including time-bins [4,5], transverse momentum [6, 7] or orbital angular momentum modes [8].We demonstrate here a new way to encode qudits in the energy spectrum of the entangled photons by defining frequency bins within their spectra. Broadband entangled photons are generated by continuous wave spontaneous down-conversion and detected in coincidence by sum frequency generation. By means of experimental methods used for shaping fs-laser pulses, frequency bins can be addressed in the photons spectra. Furthermore, controlling each frequency component individually allows to manipulate and characterize the quantum states. The dimension of the generated states is in practice limited by the optical resolution of the setup only.
Quantum entanglement is a fundamental resource for secure information processing and communications. The canonical optical quantum information processing encodes a single qubit per photon, with remarkable demonstrations of secure quantum communications, linear optical quantum computing amongst others. Often the polarization qubit, a discrete variable with entangled Bell states, is used. Continuous variables such as energy-time modes and spatial modes, however, present a dramatically larger Hilbert space for quantum information processing. The high-dimensional entanglement capture more qubits per photon, enabling dramatically higher secure key rates over longer distances and with better error resilience. Here I will describe our results on high-dimensional entanglement in quantum frequency combs for dense quantum communications. We first demonstrate revival of the Hong-Ou-Mandel interferences, long postulated by theorists more than a decade ago, up to 19-dimensions and with visibilities up to 96.5%. The mode-locked two-photon state in high-dimensions is further witnessed through a stabilized Franson interferometer, as a generalized Bell’s inequality test and hyperentangled through multiple degrees-of-freedom. Entanglement revivals of the non-local interference at discrete time-bins are uncovered, up to 97.8% visibility, as a fundamental resource for dense secure information processing.
We propose a method for generation of entangled photonic states in high dimensions, the so-called qudits, by exploiting quantum correlations of Orbital Angular Momentum (OAM) entangled photons, produced via Spontaneous Parametric Down Conversion. Diffraction masks containing N angular slits placed in the path of twin photons define a qudit space of dimension N2, spanned by the alternative pathways of OAM-entangled photons. We quantify the high-dimensional entanglement of path-entangled photons by the Concurrence, using an analytic expression valid for pure states. We report numerical results for the Concurrence as a function of the angular aperture size for the case of high-dimensional OAM entanglement and for the case of high-dimensional path entanglement, produced by N × M angular slits. Our results provide additional means for preparation and characterization of entangled quantum states in high-dimensions, a fundamental resource for quantum simulation and quantum information protocols.
Entanglement in high-dimensional quantum systems, where one or more degrees of freedom of light are involved, offers increased information capacities and enables new quantum protocols.Here, we demonstrate a functional source of high-dimensional, noise-resilient hyperentangled states encoded in time-frequency and vector vortex structured modes, which in turn carry single-particle entanglement between polarization and orbital angular momentum.Pairing nonlinearity-engineered parametric downconversion in an interferometric scheme with spin-to-orbital-angular-momentum conversion, we generate highly entangled photon pairs at telecom wavelength that we characterize via two-photon interference and quantum state tomography, achieving near-unity visibilities and fidelities.While hyperentanglement has been demonstrated before in photonic qubits, here we present a rich entanglement structure involving spectrally and spatially structured light, where three different forms of entanglement coexist in the same biphoton state.
Abstract In this paper, we demonstrate the generation of high-performance entangled photon-pairs in different degrees of freedom from a single piece of fiber pigtailed periodically poled LiNbO 3 (PPLN) waveguide. We utilize cascaded second-order nonlinear optical processes, i.e., second-harmonic generation (SHG) and spontaneous parametric downconversion (SPDC), to generate photon-pairs. Previously, the performance of the photon-pairs is contaminated by Raman noise photons. Here by fiber-integrating the PPLN waveguide with noise-rejecting filters, we obtain a coincidence-to-accidental ratio (CAR) higher than 52,600 with photon-pair generation and detection rate of 52.36 kHz and 3.51 kHz, respectively. Energy-time, frequency-bin, and time-bin entanglement is prepared by coherently superposing correlated two-photon states in these degrees of freedom, respectively. The energy-time entangled two-photon states achieve the maximum value of CHSH-Bell inequality of S = 2.71 ± 0.02 with two-photon interference visibility of 95.74 ± 0.86%. The frequency-bin entangled two-photon states achieve fidelity of 97.56 ± 1.79% with a spatial quantum beating visibility of 96.85 ± 2.46%. The time-bin entangled two-photon states achieve the maximum value of CHSH-Bell inequality of S = 2.60 ± 0.04 and quantum tomographic fidelity of 89.07 ± 4.35%. Our results provide a potential candidate for the quantum light source in quantum photonics.
Photonic quantum technologies rely on the deterministic preparation of quantum states encoded in single-photons degrees of freedom. While polarisation, orbital angular momentum and path have been routinely used since the early days of photonic quantum information, the last few years have seen an increasing interest in the frequency-time encoding [1, 2]. Indeed, the possibility of generating high-dimensional states, together with the compatibility of frequency modes and standard optical components, makes the spectral degree of freedom suitable for enhancing the efficiency of quantum protocols, spanning from quantum communication to optical quantum computation.