Photonic quantum technologies rely on the deterministic preparation of quantum states encoded in single-photons degrees of freedom. While polarisation, orbital angular momentum and path have been routinely used since the early days of photonic quantum information, the last few years have seen an increasing interest in the frequency-time encoding [1, 2]. Indeed, the possibility of generating high-dimensional states, together with the compatibility of frequency modes and standard optical components, makes the spectral degree of freedom suitable for enhancing the efficiency of quantum protocols, spanning from quantum communication to optical quantum computation.
Photonic quantum technologies rely on the deterministic preparation of quantum states encoded in single-photons degrees of freedom. While polarisation, orbital angular momentum and path have been routinely used since the early days of photonic quantum information, the last few years have seen an increasing interest in the frequency-time encoding [1, 2]. Indeed, the possibility of generating high-dimensional states, together with the compatibility of frequency modes and standard optical components, makes the spectral degree of freedom suitable for enhancing the efficiency of quantum protocols, spanning from quantum communication to optical quantum computation.
The field of high-dimensional quantum photonics involves the use of multimode photonic degrees-of-freedom such as the spatial, temporal, or spectral structure of light to encode multi-level quantum states. Recent years have seen rapid progress in the development of methods to generate, manipulate, and distribute such quantum states of light and their use in a range of quantum technology applications that offer practical advantages over conventional qubit-based approaches. High-dimensional quantum states of light encoded in photonic time-bins, frequency-bins, transverse-spatial modes, waveguide paths, and temporal modes have enabled noise-robust fundamental tests of quantum mechanics, error-resilient and high-capacity quantum communication protocols, andas well as efficient approaches for quantum information processing, to name just a few examples. However, research in this field has progressed fairly independently, with little exchange across different photonic degrees-of-freedom or between experiment and theory and no comprehensive comparison between degrees-of-freedom. This roadmap aims to bridge this gap by surveying progress in each area and identifying shared challenges and opportunities that cut across two or more photonic degrees-of-freedoms. We review early work and state-of-the-art experimental techniques under development for high-dimensional quantum states encoded in single and entangled photons, as well as theoretical tools for their measurement and certification. We outline the main outstanding challenges for theory and each experimental degree-of-freedom, identifying promising future directions of research that may enable these to be overcome. We end by discussing interconnections and shared challenges centered around their distribution, measurement, and manipulation, with a view towards their integration into next-generation quantum technology platforms and applications.
Quantum photonics is increasingly making use of the energy-time degree of freedom (DoF) to encode information. Its inherently high-dimensionality offers higher information capacity and robustness against noise. Most frequently, the energy-time DoF is exploited in the form of time bins and frequency bins, with direct applications in both quantum information processing tasks and quantum communication protocols. More recently, it has been used also in its pulse modes (or temporal modes) form, sets of states overlapping in time and frequency but kept orthogonal considering their temporal and spectral phase, whose difficult manipulation and characterisation made it less appealing for experimental applications. The production of states encoded in pulse modes has been demonstrated through sum frequency generation in waveguides [1] and parametric down conversion in bulk crystals [2], as well as the demonstration of schemes for creating hyper-entanglement among energy-time DoF and other high-dimensional DoFs [3], [4]. However, their implementation is still an area of continuous development and evolution, given the complexity of manipulating and characterising them.
The exploitation of quantum mechanics has the potential to solve important challenges and \nintroduce novel technologies enabling, among others, powerful computation (which can solve \ncertain problems exponentially faster than classical computers), perfectly secure communications, \nas well as sensing and imaging with precision and resolutions not achievable by classical means. \nIn order to make use of the unique properties of quantum physics, experimental platforms \nthat provide access to, and allow the control of quantum states, need to be developed. In \nparticular, quantum systems composed of multiple parties are required, where each party is in a \ncoherent superposition of states, and where multiples of such parties are in a coherent \nsuperposition with each other (e.g. being entangled). Additionally, in order to make use of such \nentangled quantum systems, it is required that each individual party can be coherently controlled \nand measured. The usability and available quantum resources of the entangled system is related \nto its size, which is proportional to the number of entangled parties, as well as the dimensionality \nof the superposition each party is in. For this reason, there is a imminent demand to achieve, \ninvestigate, and improve the generation and control of large quantum systems, comprised of as \nmany entangled parties as possible, where each party is in an ideally high-dimensional \nsuperposition. \nMany quantum platforms are currently subject to extensive research, such as trapped ions, \nsuperconducting circuits, defect centers in solid-state crystals, mechanical oscillators, and optical \nquantum states (i.e. photons). While all platforms provide distinct advantages (as well as \nchallenges), optical photon states are of particular interest, because they can interact with other \nquantum systems, and can be transmitted over long distances while preserving their quantum \ncoherence without the need for extensive shielding. A large variety of sources for optical \nquantum states has been demonstrated, however most such implementations suffer from high \ncomplexity, ultimately limiting their scalability. Integrated photonics has recently become a \nleading platform for the compact, cost-efficient, and stable generation and processing of optical \nquantum states. However, to date, integrated quantum sources have only been able to generate \nphoton pairs, which operated on single channels, and single polarization modes. Furthermore, in \nthe few realizations of on-chip entanglement, they were limited to two entangled parties, where \neach party was in a two-dimensional superposition. These limitations of current integrated photon sources arise in large part from the concepts currently exploited to generate and control these \nstates. In particular, path-entangled sources are the most commonly used, but increasing the \nquantum state complexity requires a significant, and very challenging, increase in device \ncomplexity. There is therefore an urgent need to develop new concepts that can achieve the onchip \ngeneration of large and complex photon states without increasing source complexity, while \nstill enabling coherent quantum state control and detection. \nIn this work, we aim to address these limitations by making use of multiple frequency and \ntemporal modes within a single spatial waveguide mode (therefore readily compatible with \nstandard optical fibers) of an on-chip microring resonator. This approach is in contrast to more \ncommonly used techniques relying on path entanglement, which exploits multiple spatial modes \nand generates entanglement by means of complex waveguide structures. Working within a single \nspatial mode, we achieve the first demonstration of pure heralded single photons and entangled \nphoton pairs, which are emitted on multiple frequency modes from a single source. We then \ndemonstrate the first generation of multi-photon entangled quantum states on a photonic chip. \nFinally, by making use of the spectral multi-mode nature of optical frequency combs, we achieve \nthe generation of photon pairs in a coherent superposition of multiple frequency modes, \nrepresenting the first generation of high-dimensional entangled states on a photonic chip. \nOur work represents a significant step forward in the generation of complex quantum \nstates on a photonic chip and in a single spatial mode compatible with standard optical fibers. In \naddition, we demonstrated coherent quantum state control and manipulation for all generated \nstates by means of standard telecommunications components, which could in the future be also \nintegrated on single, monolithic chip. Our results indicate that the exploitation of integrated \noptical frequency comb sources for the generation of optical quantum states can provide a \nscalable and practical platform for quantum technologies.
High-dimensional degrees of photons – such as orbital angular momentum, spatial modes of frequency – provide a powerful mean to increase the density and security of quantum communication, and to enhance flexibility in quantum computing. In particular, the spatial degree of freedom is particularly suited to on-chip integration. Rapid progress has been made in recent years to develop integrated circuits achieving on-chip quantum interference, entanglement and gate operations on spatially encoded states, culminating in the demonstration of the Boson Sampling task on-chip [1]. While many of these demonstrations have relied on external sources to generate quantum states of light, which were then fed into a passive circuitry, a next step has been taken recently with the demonstration of active chips combining the generation and manipulation of spatially encoded states [2].
Encoding information in high-dimensional degrees of freedom of photons has led to new avenues in various quantum protocols such as communication and information processing. Yet to fully benefit from the increase in dimension requires a deterministic detection system, e.g., to reduce dimension dependent photon loss in quantum key distribution. Recently, there has been a growing interest in using vector vortex modes, spatial modes of light with entangled degrees of freedom, as a basis for encoding information. However, there is at present no method to detect these non-separable states in a deterministic manner, negating the benefit of the larger state space. Here we present a method to deterministically detect single photon states in a four dimensional space spanned by vector vortex modes with entangled polarisation and orbital angular momentum degrees of freedom. We demonstrate our detection system with vector vortex modes from the |[Formula: see text]| = 1 and |[Formula: see text]| = 10 subspaces using classical and weak coherent states and find excellent detection fidelities for both pure and superposition vector states. This work opens the possibility to increase the dimensionality of the state-space used for encoding information while maintaining deterministic detection and will be invaluable for long distance classical and quantum communication.