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Physical Review A

Hyperfine interaction in the Autler-Townes effect: The formation of bright, dark, and chameleon states

Teodora Kirova, A. Cinins, Dmitry K. Efimov, Martins Bruvelis, K. Miculis, Nikolai N. Bezuglov, Marcis P. Auzinsh, I. I. Ryabtsev, Aigars Ekers

Published Oct 26, 2017• 11 citations
Publisher

Abstract

This paper is devoted to clarifying the implications of hyperfine (HF) interaction in the formation of adiabatic (i.e., ``laser-dressed'') states and their expression in the Autler-Townes (AT) spectra. We first use the Morris-Shore model [J. R. Morris and B. W. Shore, Phys. Rev. A 27, 906 (1983)] to illustrate how bright and dark states are formed in a simple reference system where closely spaced energy levels are coupled to a single state with a strong laser field with the respective Rabi frequency ${\mathrm{\ensuremath{\Omega}}}_{S}$. We then expand the simulations to realistic hyperfine level systems in Na atoms for a more general case when non-negligible HF interaction can be treated as a perturbation in the total system Hamiltonian. A numerical analysis of the adiabatic states that are formed by coupling of the $3{p}_{3/2}$ and $4{d}_{5/2}$ states by the strong laser field and probed by a weak laser field on the $3{s}_{1/2}\ensuremath{-}3{p}_{3/2}$ transition yielded two important conclusions. Firstly, the perturbation introduced by the HF interaction leads to the observation of what we term ``chameleon'' states---states that change their appearance in the AT spectrum, behaving as bright states at small to moderate ${\mathrm{\ensuremath{\Omega}}}_{S}$, and fading from the spectrum similarly to dark states when ${\mathrm{\ensuremath{\Omega}}}_{S}$ is much larger than the HF splitting of the $3{p}_{3/2}$ state. Secondly, excitation by the probe field from two different HF levels of the ground state allows one to address orthogonal sets of adiabatic states; this enables, with appropriate choice of ${\mathrm{\ensuremath{\Omega}}}_{S}$ and the involved quantum states, a selective excitation of otherwise unresolved hyperfine levels in excited electronic states.

DOI
10.1103/physreva.96.043421

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This paper is devoted to clarifying the implications of hyperfine (HF) interaction in the formation of adiabatic (i.e., laser-dressed'') states and their expression in the Autler-Townes (AT) spectra. We first use the Morris-Shore model [J. R. Morris and B. W. Shore, Phys. Rev. A 27, 906 (1983)] to illustrate how bright and dark states are formed in a simple reference system where closely spaced energy levels are coupled to a single state with a strong laser field with the respective Rabi frequency ${\mathrm{\ensuremath{\Omega}}}_{S}$. We then expand the simulations to realistic hyperfine level systems in Na atoms for a more general case when non-negligible HF interaction can be treated as a perturbation in the total system Hamiltonian. A numerical analysis of the adiabatic states that are formed by coupling of the $3{p}_{3/2}$ and $4{d}_{5/2}$ states by the strong laser field and probed by a weak laser field on the $3{s}_{1/2}\ensuremath{-}3{p}_{3/2}$ transition yielded two important conclusions. Firstly, the perturbation introduced by the HF interaction leads to the observation of what we term chameleon'' states---states that change their appearance in the AT spectrum, behaving as bright states at small to moderate \ensuremathΩS{\mathrm{\ensuremath{\Omega}}}_{S}\ensuremathΩS​, and fading from the spectrum similarly to dark states when \ensuremathΩS{\mathrm{\ensuremath{\Omega}}}_{S}\ensuremathΩS​ is much larger than the HF splitting of the 3p3/23{p}_{3/2}3p3/2​ state. Secondly, excitation by the probe field from two different HF levels of the ground state allows one to address orthogonal sets of adiabatic states; this enables, with appropriate choice of \ensuremathΩS{\mathrm{\ensuremath{\Omega}}}_{S}\ensuremathΩS​ and the involved quantum states, a selective excitation of otherwise unresolved hyperfine levels in excited electronic states.
Earlier research highlighted the absence of certain bright peaks in Autler-Townes laser excitation spectra of alkali-metal atoms and attributed this phenomenon to a specific architecture of adiabatic (or ``laser-dressed'') states in hyperfine (HF) components. Here we have studied the dressed states' properties in several two-photon excitation schemes where constructive and destructive interferences between HF excitation pathways limit the available two-photon transitions. The analysis reveals a mechanism by which this interference reduces the conventional two-photon selection rule for the total angular momentum FFF, from $\mathrm{\ensuremath{\Delta}}F=0,\ifmmode\pm\else\textpm\fi{}1$ to $\mathrm{\ensuremath{\Delta}}F\ensuremath{\equiv}0$. Our discovery presents a practical method for selectively controlling the populations of unresolvable HF FFF components of ns1/2n{s}_{1/2}ns1/2​ Rydberg states in alkali-metal atoms. Using numerical simulations with sodium and rubidium atoms, we demonstrate that by blocking the effects of HF interaction with a specially tuned auxiliary control-laser field, the deviations from the ideal selectivity of the HF components population can be lower than 0.010.01%0.01 for Na and 0.0010.001%0.001 for Rb atoms.
Abstract We have investigated the formation of laser‐dressed states in HF components of sodium atoms and their manifestations in Autler–Townes spectra. An explicit procedure is proposed for constructing a specific Morris–Shore wave function basis, within which two‐photon excitation schemes are reduced to sets of mutually orthogonal 3‐ and 2‐level excitation sequences, and single uncoupled states. It has been demonstrated that the Morris–Shore basis states correspond to bright and dark states, along with chameleon states introduced in our recent work. Numerical simulations of the Autler–Townes spectra reveal that chameleon states can be further categorized as “fast” or “slow.” Our extended classification of dressed states enables more accurate reconstruction of excited state properties in optical methods for atomic media diagnostics.
We investigated the absence of certain bright peaks in Autler-Townes laser excitation spectra of alkali metal atoms. Our research revealed that these dips in the spectra are caused by a specific architecture of adiabatic (or ``laser-dressed'') states in hyperfine (HF) components. The dressed states' analysis pinpointed several cases where constructive and destructive interference between HF excitation pathways in a two-photon excitation scheme limits the available two-photon transitions. This results in a reduction of the conventional two-photon selection rule for the total angular momentum FFF, from ΔF=0,±1ΔF= 0,\pm 1ΔF=0,±1 to ΔF≡0ΔF\equiv 0ΔF≡0. Our discovery presents practical methods for selectively controlling the populations of unresolvable HF FFF-components of ns1/2ns_{1/2}ns1/2​ Rydberg states in alkali metal atoms. Using numerical simulations with sodium and rubidium atoms, we demonstrate that by blocking the effects of HF interaction with a specially tuned auxiliary control laser field, the deviations from the ideal selectivity of the HF components population can be lower than 0.01%0.01\%0.01% for Na and 0.001%0.001\%0.001% for Rb atoms.
Abstract We investigated the Autler–Townes (AT) splitting produced by microwave (mw) transitions between atomic Rydberg states explored by optical spectroscopy from the ground electronic state. The laser-atom Hamiltonian describing the double irradiation of such a multilevel system is analysed on the basis of the Morris–Shore transformation. The application of this transformation to the mw-dressed atomic system allows the identification of bright, dark, and spectator states associated with different configurations of atomic states and mw polarisations. We derived synthetic spectra that show the main features of Rydberg spectroscopy. Complex AT spectra are obtained in a regime of strong mw dressing, where a hybridisation of the Rydberg fine structure states is produced by the driving.
This work focuses on visualization of dark states arising in systems of hyperfine states upon two-photon excitation.In our experiment, levels 3S 1/2 and 3P 1/2 of sodium atoms are coupled by a strong S-laser field forming the laser-dressed adiabatic states, which are then monitored by scanning a weak probe P-field across the 3P 1/2 → 7D 3/2 transition.The excitation spectrum of the 7D 3/2 state exhibits one main peak and several side peaks.The latter shift farther apart with increasing S-laser intensity, while the position of the main peak is hardly affected, which associates its origin with a class of dark states decoupled from laser interactions.The results of numerical simulation of the observed spectra based on the solution of the optical Bloch equations are in good agreement with the experimental data.The results are of interest for atomic and laser physics.
The Autler—Townes effect is considered for the case where a strong control field acts in the frequency profile of a hyperfine transition taking into account the hyperfine interaction. An exact expression is derived for the susceptibility of the medium with respect to a probe field that acts in the frequency profile of a coupled transition of the alkaliatom D 1 line. It is shown that the hyperfine interaction in the excited state may substantially modify the susceptibility of the medium. In particular, it is shown that, when the control field is tuned to wings of atomic transitions, the structure of the Autler—Townes resonances appears to be noticeably differing from what is predicted by the Λ-scheme approximation. It is found that tuning of the control field frequency to between hyperfine components of the excited state enhances the resonant structure in this region. The results are discussed in terms of the quantum memory protocols based on the effects of Raman scattering and electromagnetically induced transparency.