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Light storage for 150 milliseconds at room temperature

Or Katz, Ofer Firstenberg

Published Oct 18, 2017• 0 citations
OpenAlex

Abstract

Light storage is the controlled and reversible mapping of light fields onto long-lived states of matter [1], forming the basis for quantum memories in optical quantum networks [2-6]. Prominent storage media are warm alkali gases due to their strong optical coupling and long-lived spin states [7-8]. In a dense gas, the random atomic collisions dominate the lifetime of the spin coherence, limiting the storage time to a few milliseconds [9-10]. Here we present and experimentally demonstrate a storage scheme that is insensitive to spin-exchange collisions, thus enabling long storage times at high atomic densities. This unique property is achieved by mapping the light field onto spin orientation, rather than onto higher spin moments. We report on a record storage lifetime for a warm system of 150 milliseconds (1/e) in cesium vapor. Furthermore, our scheme lays the foundations for hour-long quantum memories using rare-gas nuclear spins.

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Light storage is the controlled and reversible mapping of light fields onto long-lived states of matter [1], forming the basis for quantum memories in optical quantum networks [2-6]. Prominent storage media are warm alkali gases due to their strong optical coupling and long-lived spin states [7-8]. In a dense gas, the random atomic collisions dominate the lifetime of the spin coherence, limiting the storage time to a few milliseconds [9-10]. Here we present and experimentally demonstrate a storage scheme that is insensitive to spin-exchange collisions, thus enabling long storage times at high atomic densities. This unique property is achieved by mapping the light field onto spin orientation, rather than onto higher spin moments. We report on a record storage lifetime for a warm system of 150 milliseconds (1/e) in cesium vapor. Furthermore, our scheme lays the foundations for hour-long quantum memories using rare-gas nuclear spins.
Light storage, the controlled and reversible mapping of photons onto long-lived states of matter, enables memory capability in optical quantum networks. Prominent storage media are warm alkali vapors due to their strong optical coupling and long-lived spin states. In a dense gas, the random atomic collisions dominate the lifetime of the spin coherence, limiting the storage time to a few milliseconds. Here we present and experimentally demonstrate a storage scheme that is insensitive to spin-exchange collisions, thus enabling long storage times at high atomic densities. This unique property is achieved by mapping the light field onto spin orientation within a decoherence-free subspace of spin states. We report on a record storage time of 1 s in room-temperature cesium vapor, a 100-fold improvement over existing storage schemes. Furthermore, our scheme lays the foundations for hour-long quantum memories using rare-gas nuclear spins.
Nuclear spins of noble gases exhibit exceptionally long coherence times and can potentially serve as a long-lived storage medium for quantum information. We analyze and compare the performance of two mechanisms for mapping the quantum state of light onto the collective spin state of noble gases. The first mechanism utilizes collisional exchange with the electronic spin state of metastable noble-gas atoms, while the second relies on spin-exchange collisions with ground-state alkali-metal atoms. We describe the operation of an optical quantum memory relying on these two mechanisms using a compact model and study strategies that optimize the memory storage efficiency. Through numerical simulations, we identify optimal sequences for storing optical signals with different signal bandwidths and electronic spin relaxation rates. This work highlights the qualitative difference between the two approaches for using noble gases as long-lived quantum memories at noncryogenic conditions and outlines the regimes in which they are expected to be efficient.
Optical quantum memories, which store and preserve the quantum state of photons, rely on a coherent mapping of the photonic state onto matter states that are optically accessible. Here we outline and characterize schemes to map the state of photons onto long-lived but optically inaccessible collective states of noble-gas spins. The mapping employs coherent spin-exchange interaction arising from random collisions with alkali vapor. We propose efficient storage strategies in two operating regimes and analyze their performance for several proposed experimental configurations.
Summary form only given. The spin polarized ground state of a cesium gas in a paraffin coated glass cell at room temperature has been recently used for generation of a long lived entangled state of atoms. In this paper we report on the first results towards using this medium as a quantum memory for polarization states of a light beam. The possibility of a reversible transfer of polarization states between light and atoms via interspecies teleportation protocols has been previously proposed. A narrowband tunable source of entangled light needed for such a transfer has been constructed before. We demonstrate that our set-up allows detection of the quantum state of light propagating through an atomic sample by means of observing the state of the long lived collective spin of the sample. For this purpose a polarization squeezed optical probe is prepared by mixing orthogonally polarized squeezed vacuum and coherent light with a variable phase on a polarizing beamsplitter.
The long-lived, efficient storage and retrieval of a qubit encoded on a photon is an important ingredient for future quantum networks. Although systems with intrinsically long coherence times have been demonstrated, the combination with an efficient light-matter interface remains an outstanding challenge. In fact, the coherence times of memories for photonic qubits are currently limited to a few milliseconds. Here we report on a qubit memory based on a single atom coupled to a high-finesse optical resonator. By mapping and remapping the qubit between a basis used for light-matter interfacing and a basis which is less susceptible to decoherence, a coherence time exceeding 100 ms has been measured with a time-independant storage-and-retrieval efficiency of 22%. This demonstrates the first photonic qubit memory with a coherence time that exceeds the lower bound needed for teleporting qubits in a global quantum internet.