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arXiv:quant-ph/0504152 · Physical Review Letters

Long-Lived Quantum Memory with Nuclear Atomic Spins

Aurélien Dantan, Gael Reinaudi, Alice Sinatra, Franck Laloë, E. Giacobino, M. Pinard

Published Sep 15, 2005• 35 citations
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Abstract

We propose to store nonclassical states of light into the macroscopic collective nuclear spin (10(18) atoms) of a 3He vapor, using metastability exchange collisions. These collisions, commonly used to transfer orientation from the metastable state 2 3S1 to the ground state of 3He, can also transfer quantum correlations. This gives a possible experimental scheme to map a squeezed vacuum field state onto a nuclear spin state with very long storage times (hours).

DOI
10.1103/physrevlett.95.123002

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We propose to store nonclassical states of light into the macroscopic collective nuclear spin (10(18) atoms) of a 3He vapor, using metastability exchange collisions. These collisions, commonly used to transfer orientation from the metastable state 2 3S1 to the ground state of 3He, can also transfer quantum correlations. This gives a possible experimental scheme to map a squeezed vacuum field state onto a nuclear spin state with very long storage times (hours).
Nuclear spins of noble gases exhibit exceptionally long coherence times and can potentially serve as a long-lived storage medium for quantum information. We analyze and compare the performance of two mechanisms for mapping the quantum state of light onto the collective spin state of noble gases. The first mechanism utilizes collisional exchange with the electronic spin state of metastable noble-gas atoms, while the second relies on spin-exchange collisions with ground-state alkali-metal atoms. We describe the operation of an optical quantum memory relying on these two mechanisms using a compact model and study strategies that optimize the memory storage efficiency. Through numerical simulations, we identify optimal sequences for storing optical signals with different signal bandwidths and electronic spin relaxation rates. This work highlights the qualitative difference between the two approaches for using noble gases as long-lived quantum memories at noncryogenic conditions and outlines the regimes in which they are expected to be efficient.
Light storage is the controlled and reversible mapping of light fields onto long-lived states of matter [1], forming the basis for quantum memories in optical quantum networks [2-6]. Prominent storage media are warm alkali gases due to their strong optical coupling and long-lived spin states [7-8]. In a dense gas, the random atomic collisions dominate the lifetime of the spin coherence, limiting the storage time to a few milliseconds [9-10]. Here we present and experimentally demonstrate a storage scheme that is insensitive to spin-exchange collisions, thus enabling long storage times at high atomic densities. This unique property is achieved by mapping the light field onto spin orientation, rather than onto higher spin moments. We report on a record storage lifetime for a warm system of 150 milliseconds (1/e) in cesium vapor. Furthermore, our scheme lays the foundations for hour-long quantum memories using rare-gas nuclear spins.
We propose a technique to control the macroscopic collective nuclear spin of a helium-3 gas in the quantum regime using light. The scheme relies on metastability exchange collisions to mediate interactions between optically accessible metastable states and the ground-state nuclear spin, giving rise to an effective nuclear spin-light quantum nondemolition interaction of the Faraday form. Our technique enables measurement-based quantum control of nuclear spins, such as the preparation of spin-squeezed states. This, combined with the day-long coherence time of nuclear spin states in helium-3, opens the possibility for a number of applications in quantum technology.
Light storage, the controlled and reversible mapping of photons onto long-lived states of matter, enables memory capability in optical quantum networks. Prominent storage media are warm alkali vapors due to their strong optical coupling and long-lived spin states. In a dense gas, the random atomic collisions dominate the lifetime of the spin coherence, limiting the storage time to a few milliseconds. Here we present and experimentally demonstrate a storage scheme that is insensitive to spin-exchange collisions, thus enabling long storage times at high atomic densities. This unique property is achieved by mapping the light field onto spin orientation within a decoherence-free subspace of spin states. We report on a record storage time of 1 s in room-temperature cesium vapor, a 100-fold improvement over existing storage schemes. Furthermore, our scheme lays the foundations for hour-long quantum memories using rare-gas nuclear spins.
Optical quantum memories, which store and preserve the quantum state of photons, rely on a coherent mapping of the photonic state onto matter states that are optically accessible. Here we outline and characterize schemes to map the state of photons onto long-lived but optically inaccessible collective states of noble-gas spins. The mapping employs coherent spin-exchange interaction arising from random collisions with alkali vapor. We propose efficient storage strategies in two operating regimes and analyze their performance for several proposed experimental configurations.