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Physical review. B./Physical review. B

Magnon-magnon interactions in a room-temperature magnonic Bose-Einstein condensate

Oleksandr Dzyapko, Ivan Lisenkov, Patrik Nowik-Boltyk, V. E. Demidov, S. O. Demokritov, Benny Koene, Andrei I. Kirilyuk, Th. Rasing, V. S. Tiberkevich, Andrei N. Slavin

Published Aug 30, 2017• 40 citations
Publisher

Abstract

The Bose-Einstein condensate of magnons (mBEC) that is formed at room temperature in parametrically pumped magnetic films is doubly degenerate: it is formed simultaneously in two spectral minima corresponding to the lowest-energy magnons propagating in opposite directions along the in-plane bias magnetic field. In this work the interactions of magnons in the mBEC are studied both theoretically and experimentally. It is shown by direct calculation that the magnons residing in each of the degenerate spectral minima of mBEC form a practically ideal magnon gas, as the attractive self-interaction between these magnons is very weak. At the same time, the interaction between the magnons residing in different spectral minima, corresponding to opposite directions of the magnon wave vector, is relatively strong and repulsive, leading to a repulsive total intermagnon interaction. By measuring the spectral characteristics of the mBEC it is shown that with increased magnon density the energy per magnon in the mBECs increases, thus confirming experimentally that the net intermagnon interaction in a doubly degenerate mBEC is repulsive.

DOI
10.1103/physrevb.96.064438

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The Bose-Einstein condensate of magnons (mBEC) that is formed at room temperature in parametrically pumped magnetic films is doubly degenerate: it is formed simultaneously in two spectral minima corresponding to the lowest-energy magnons propagating in opposite directions along the in-plane bias magnetic field. In this work the interactions of magnons in the mBEC are studied both theoretically and experimentally. It is shown by direct calculation that the magnons residing in each of the degenerate spectral minima of mBEC form a practically ideal magnon gas, as the attractive self-interaction between these magnons is very weak. At the same time, the interaction between the magnons residing in different spectral minima, corresponding to opposite directions of the magnon wave vector, is relatively strong and repulsive, leading to a repulsive total intermagnon interaction. By measuring the spectral characteristics of the mBEC it is shown that with increased magnon density the energy per magnon in the mBECs increases, thus confirming experimentally that the net intermagnon interaction in a doubly degenerate mBEC is repulsive.
A quantised spin wave – magnon – in magnetic films can undergo Bose-Einstein condensation (BEC) into two energetically degenerate lowest-energy quantum states with nonzero wave vectors ±k BEC . This corresponds to two interfering condensates forming spontaneously in momentum space. Brillouin Light Scattering studies for a microwavepumped film with submicrometer spatial resolution experimentally confirm the existence of the two wavefunctions and show that their interference results in a nonuniform ground state of the condensate with the density oscillating in space. Moreover, fork dislocations in the density fringes provide direct experimental evidence for the formation of pinned half-quantum vortices in the magnon condensate. The measured amplitude of the density oscillation implies the formation of a nonsymmetric state that corresponds to nonequal occupation of two energy minima. We discuss the experimental findings and consider the theory of magnon condensates, which includes, to leading order, the contribution from the noncondensed magnons. The effect of the noncondensed magnon cloud is to increase the contrast of the asymmetric state and to bring about the experimental measurements. Introduction Magnons are quasiparticles corresponding to quantised spin waves that describe the collective motion of spins [1]. In recent years, it has become possible to realise a BEC of magnons in two remarkably different systems: in superfluid phases of an isotope of helium – Helium-3 at ultralow temperatures [2, 3] and in ferrimagnetic insulators [4, 5, 6, 7]. In the normal, noncondensed state, these magnetic materials exhibit a magnetically ordered state with a gas of magnons whose phases are not correlated. However, once condensation occurs, spins develop phase coherence resulting in a common global frequency and phase of precession. At room temperature, ferrimagnetic insulators, such as yttrium-iron garnet (YIG) films, together with a combination of an in-plane magnetic field and microwave radiation, are required for the magnon condensation [4, 5, 6, 7]. Therefore, in analogy with exciton– polariton condensates, this provides yet another example of a BEC of quasiparticle excitations in a solid-state system. Experimental Realisation of a Bose-Einstein Condensate of Magnons in an Epitaxial YIG-film A room-temperature Bose-Einstein condensate of magnons was created in an epitaxial YIG-film using an experimental setup shown in Fig. 25.1a, which, in general, is similar to that used in our previous studies [4, 5]. Given that magnons are quasiparticle excitations, their number is not conserved and, therefore, the chemical potential is zero.
Abstract Bose–Einstein condensation (BEC) of magnons is one of the few macroscopic quantum phenomena observable at room temperature. Due to the competition of the exchange and the magnetic dipole interactions, the minimum-energy magnon state is doubly degenerate and corresponds to two antiparallel non-zero wavevectors. Correspondingly, the room-temperature magnon BEC differs essentially from other condensates, since it takes place simultaneously at ± kmin. The degeneracy of BEC and interaction between its two components have significant impact on condensate properties. Phase locking of the two condensates causes formation of a standing wave of the condensate density and quantized vortices. Additionally, interaction between the two components is believed to be important for stabilization of the condensate with respect to a real-space collapse. Thus, the possibility to create a non-degenerate, single-component condensate is decisive for understanding of underlying physics of magnon BEC. Here, we experimentally demonstrate an approach, which allows one to accomplish this challenging task. We show that this can be achieved by using a separation of the two components of the degenerate condensate in the real space by applying a local pulsed magnetic field, which causes their motion in the opposite directions. Thus, after a certain delay, the two clouds corresponding to different components become well separated in the real space. We find that motion of the clouds can be described well based on the peculiarities of magnon dispersion characteristics. Additionally, we show that, during the motion, the condensate cloud harvests non-condensed magnons, which results in a partial compensation of condensate depletion.
Bose-Einstein condensation (BEC) of magnons is one of few macroscopic quantum phenomena observable at room temperature. Due to competition of the exchange and the magnetic dipole interactions the minimum-energy magnon state is doubly degenerate and corresponds to two antiparallel non-zero wavevectors. Correspondingly, magnon BEC differs essentially from other condensates, since it takes place simultaneously at +/-k_min. The degeneracy of BEC and interaction between its two components have significant impact on the condensate properties. Phase locking of the two condensates causes formation of a standing wave of the condensate density and quantized vortices. Additionally, interaction between the two components is believed to be important for stabilization of the condensate with respect to the real-space collapse. Thus, the possibility to create a non-degenerate, single-component condensate is decisive for understanding of underlying physics of magnon BEC. Here, we experimentally demonstrate an approach, which allows one to accomplish this challenging task. We show that this can be achieved by using a separation of the two components of the degenerate condensate in the real space by applying a local pulsed magnetic field, which causes their motion in the opposite directions. Thus, after a certain delay, the two clouds corresponding to different components become well separated in the real space. We find that the motion of the clouds can be described well based on the peculiarities of the magnon dispersion characteristics. Additionally, we show that, during the motion, the condensate cloud harvests non-condensed magnons, which results in a partial compensation of the condensate depletion.
We report evidence for the existence of a supercurrent of magnons in a magnon Bose-Einstein condensate (BEC) prepared in a room temperature yttrium-iron-garnet (YIG) magnetic film. The magnon BEC is formed in a parametrically populated magnon gas, and its temporal evolution is studied by time-resolved Brillouin light scattering (BLS) spectroscopy in the area of the BLS laser focus. It has been found that local laser heating in the center of the condensate decreases the density of the magnon BEC in the steady-state pump regime and it enhances the temporal decrease of the freely evolving magnon condensate after the termination of the pumping pulse, but it does not alter the relaxation dynamics of the gaseous magnon phase. This phenomenon is understood as the appearance of a magnon supercurrent within the condensate due to a temperature-gradient induced phase gradient in the condensate. Bose-Einstein condensation [1] can be achieved either by decreasing the temperature of a boson gas [2] or by increasing its density. The latter method is especially applicable to g ases of weakly interacting quasi-particles such as excitons [3] , polaritons [4, 5], photons [6], and magnons [7, 8]. When a spin system is pumped, and when the injected magnons thermalize through scattering processes conserving both their number and the total energy, a Bose-Einstein condensate (BEC) may be formed at the lowest energy state of the energy-momentum spectrum even at room temperature conditions of the magnetic film carrying the magnons [8, 9]. As the condensed magnon phase is localized in the global energy minimum, its group velocity is exactly zero and no energy transport can be associated with the magnon BEC. The situation can change, when a magnon supercurrent driven by a gradient in the phase of the wavefunction of a magnon condensate can be excited. Such a phase gradient can be induced by, e.g., a potential gradient or a temperature gradient. However, the dynamics of magnon condensates in such a gradient is still terra incognita. Here we provide experimental insight into the evolution of a magnon BEC in a thermal gradient generated by local laser heating. We show that such a heating influences both the steady-state characteristics and the transitional behavior of the magno n BEC, which can be understood using the concept of a magnon supercurrent. We study the temporal evolution of a magnon BEC in a single-crystal yttrium iron garnet (YIG, Y3Fe5O12) film by
In this paper, we theoretically investigate the stability of spin-wave solitons in Bose-Einstein condensates of repulsive magnons, confined by an inhomogeneous external magnetic field described by a Gaussian well. For this purpose, we use the quasi-one-dimensional Gross-Pitaevskii equation to describe the behavior of the condensate. In order to solve the Gross-Pitaevskii equation, we used two different approaches: one analytical (variational method) and another numerical (split-step Crank-Nicolson method). The stability of the solutions and the validation of the numerical results were confirmed, respectively, through the anti-VK criterion and the virial theorem. Furthermore, the simulations described the behavior of physical quantities of interest such as chemical potential, energy per magnon and central density as a function of the nonlinearity of the model (magnon-magnon interactions). The theoretical results provide subsidies for a better understanding of the nonlinear phenomena related to the Bose-Einstein condensates of magnons in ferromagnetic films.
Two recent articles of the Munster University experimental team led by S.O. Demokritov displayed several important facts related to the Bose-Einstein condensation of magnons (BECM) under permanent pumping first discovered in 2006. They contradicted existing theories of this phenomenon, which predict the attractive interaction between magnons and strong spontaneous violation of the reflection symmetry. In this article, we show that these theories implicitly assumed all relaxation processes to be fast compared with the lifetime of the magnons, whereas one of them -- relaxation between two minima of energy -- is slow. We classify processes responsible for the inter-minima relaxation and present their analytic theory. We analyze how the slow inter-minima relaxation modifies the anticipated properties of a ferromagnet with the magnon condensate.