In this thesis, we present new tools for the study of quantum systems and propose several novel schemes for practical applications in quantum information science. We explore two main topics, engineered dissipation and light-matter quantum interfaces, and investigate both with a focus on collective effects that arise if a large number of particles interact coherently with an optical quantum field. To this end, we study atomic vapor at room temperature interacting with light. We also consider ultracold atoms in optical lattices, Bose-Einstein condensates and single atoms in optical cavities for the implementation of the ideas and schemes put forward here.
In this thesis, we present new tools for the study of quantum systems and propose several novel schemes for practical applications in quantum information science. We explore two main topics, engineered dissipation and light-matter quantum interfaces, and investigate both with a focus on collective effects that arise if a large number of particles interact coherently with an optical quantum field. To this end, we study atomic vapor at room temperature interacting with light. We also consider ultracold atoms in optical lattices, Bose-Einstein condensates and single atoms in optical cavities for the implementation of the ideas and schemes put forward here.
Atoms in optical lattices are promising candidates to implement quantum information processing. Their behaviour is well understood on a microscopic level, they exhibit excellent coherence properties, and they can be easily manipulated using external fields. In very deep optical lattices, each atom is restricted to a single lattice site and can be used as a qubit. If the lattice is shallow enough such that the atoms can move, their properties can be used to simulate certain condensed matter phenomena such as superconductivity. In this thesis, we show how technical problems of optical lattices such as restricted decoherence times, or fundamental shortcomings such as the lack of phonons or strong spin interactions, can be overcome by using current or near-future experimental techniques. We introduce a scheme that makes it possible to simulate model Hamiltonians known from high-temperature superconductivity. For this purpose, previous simulation schemes to realise the spin interaction terms are extended. We especially overcome the condition of a filling factor of exactly one, which otherwise would restrict the phase of the simulated system to a Mott-insulator. This scheme makes a large range of parameters accessible, which is difficult to cover with a condensed matter setup. We also investigate the properties of optical lattices submerged into a Bose-Einstein condensate (BEC). A weak-coupling expansion in the BEC-impurity interaction strength is used to derive a model that describes the lattice atoms in terms of polarons, i.e.~atoms dressed by Bogoliubov phonons. This is analogous to the description of electrons in solids, and we observe similar effects such as a crossover from coherent to incoherent transport for increasing temperatures. Moreover, the condensate mediates an attractive off-site interaction, which leads to macroscopic clusters at experimentally realistic parameters. Since the atoms in the lattice can also be used as a quantum register with the BEC mediating a two-qubit gate, we derive a quantum master equation to examine the coherence properties of the atomic qubits. We show that the system exhibits sub- and superdecoherence and that a fast implementation of the two-qubit gate competes with dephasing. Finally, we show how to realise the encoding of qubits in a decoherence-free subspace (DFS) using optical lattices. We develop methods for implementing robust gate operations on qubits encoded in a DFS exploiting collisional interactions between the atoms. We also give a detailed analysis of the performance and stability of the gate operations and show that a robust implementation of quantum repeaters can be achieved using our setup. We compare the robust repeater scheme to one that makes use of conventional qubits only, and show the conditions under which one outperforms the other.
In the present thesis we study several schemes where the detection of the emitted light from an atomic ensemble gives information about the state of the atoms. In chapter 1 we review the basic theory for the light matter interaction in second quantized form. In chapter 2 we show how conservative potentials for the atoms, such as dispersive optical lattices, can be realized experimentally due to the dispersive interaction with a far detuned laser We then review some basic properties of the physics of a particle in a periodic potential. We show that the ground state and the lowest lying excitations of a Bose-Einstein condensate in a dispersive optical lattice can be described by the Bose-Hubbard Hamiltonian. In chapter 3 we study the photonic bandstructure of a chain of fixed pointlike atoms in a biperiodic configuration. We calculate the photonic spectra and the probe transmission if the atoms are in free space and inside a standing wave optical resonator. In chapter 4 we consider light scattering from ultracold atoms in an optical lattice where we calculate the photonic scattering cross section as a function of energy and direction of emission along the Mott-insulator-superfluid phase transition. We take into account the finite tunneling rate for the atoms, when evaluating the scattering cross section of the photons and the effect of photon recoil onto the atoms. In chapter 5 we consider a gas of ultracold atoms trapped at two spatially separated regions in space. Using a two Raman lasers to couple atoms out of the systems we show that it is possible to measure the mean value of the atomic field operator of the two systems by measuring the scattered light intensity of one of the Raman lasers. We show how this setup might be used to measure the temperature of a Bose-Einstein condensate and to monitor the superfluid to Mott-insulator phase transition for a gas of ultracold atoms in an optical lattice.
During the last decades the development of laser cooling and trapping has revolutionized the field of quantum optics. Now we master techniques to control the quantum properties of atoms and light, even at a single atom and single photon level. Understanding and controlling interactions of atoms and light both on the microscopic single particle and on the macroscopic collective levels, are two of the very active directions of the current research in this field. The goal is to engineer quantum systems with tailored properties designed for specific applications. One of the ambitious applications on this way is interfacing quantum information for quantum communication and quantum computing. We summarize here theoretical ideas and experimental methods for interfacing atom-based quantum memories with single flying photons.
Quantum optics, the study of light at the level of its building blocks, \nhas been one of the frontiers of science. The arena of quantum optics \nhas been fruitful for investigations of a wide range of interesting questions, \nfrom those on the fundamental structures in driven dissipative \nsystems to those on applications of quantum information processing \nand quantum communication. \nThe first part of this thesis is concerned with one of the holy grails \nof quantum optics: an efficient transfer of energy (coupling) between \nsingle photons and matter degrees of freedom. From a certain point \nof view, the problem of efficient coupling is purely geometrical. The \nefficiency of coupling between an atom and light is difficult because \nit is difficult to shape the wavefunction of a single photon such \nthat it overlaps perfectly with the matter degree of freedom (emitter). \nThe first contribution of this thesis is addressing this issue by considering \nan emitter which perfectly matches the single photon plane-wave. \nMoreover, luckily, such an emitter is already realized in nature in the \nform of a two-dimensional crystal. We show that a new generation \nof two-dimensional semiconductors, transition metal dichalcogenide \n(TMD) monolayers, have especially favorable characteristics for allowing \nhighly efficient coupling between photons and matter degrees \nof freedom. \nOne of the most important goals in realizing an efficient coupling \nbetween photons and matter degrees of freedom is that unlike photons, \nmatter excitations interact with each other. Hence, if we would \nlike to have photons which act as if they interact, one possible way \nis to first convert them into matter excitations, and then transfer the \ncorrelations due matter interactions back to photons. As the second \ncontribution of this thesis, we demonstrate that TMD monolayers placed \nwithin a cavity can help us create photons which avoid each other \nas if they interact. The effect can be simply understood as the TMD \nmonolayer acting as a filter for photons, such that it only allows the \npassage of one photon at a time. \nBesides being the fundamental building block of light, photons also \nserve as mediators of interactions between charged particles. In a \nsense, two positive charges repel each other because there is always \na photon which lets them know that they are close to one another. \nOn the other hand, systems of many interacting particles behave in \na completely different way then when they are alone. It may even be \nargued that all physical phenomena at some level emerge from the \nbehavior of many interacting constituents. Given this point of view, \nit is crucial to find ways to control photons in order to control the \ninteractions that they mediate between matter degrees of freedom. \nAs the third contribution of this thesis, we analyze an experimental \nscheme where the control of photonic degrees of freedom can allow \nan experimentalist to modify the strength and range of interactions \nbetween matter. In particular, we propose squeezed photon states as \na resource to control such interactions. \nThe second part of this thesis is concerned with the emergent phenomena \narising in a system of many interacting particles. In particular, \nthe fourth contribution of this thesis considers the combination \nof two fascinating phenomena which emerges such condensed matter \nsystems: superconductivity and geometric effects in lattice band \nstructures. Separately, both superconductivity and the non-trivial geometrical \neffects in lattice systems are well-established subfields of condensed \nmatter physics. Yet only more recently, the combination of \nthese two phenomena were investigated in the context of topological \nsuperconductors, as well as other superconducting states which emerge \non top of band structures with non-trivial geometry. In our study, \nwe attempt at clarifying one of the ways that the non-trivial geometry \nassociated with the lattice band structure may affect the dynamics of \nan emergent superconducting state. Surprisingly, our analysis shows \nthat one of the most robust characteristics of the superconductor, vortices \nenclosing a quantum of magnetic flux, can be modified due to \ngeometrical effects.
This thesis summarizes the research work we did in the past years, which focuses on the theoretical study of quantum effects of ordered atomic structures interacting with the quantum electric field of an optical resonator. Within this work we investigated the quantum properties of the light at the cavity output, emitted by this kind of system, and the quantum state of the atoms confined by the light fields of the cavity mode. Following one possible partition, we have organized the thesis in two parts. The first part of the thesis is devoted to the quantum properties of the light at the output of optical cavities, in which atoms are confined. After a brief introduction on the basics of atom-photon interactions, we show theoretically, that two atomic dipoles in a resonator can behave as a quantum non-linear medium, whose response can be controlled through the interactomic distance of the atoms inside the resonator. We identify the parameter regime, for which the system operates as a parametric amplifier, based on the atoms' collective dipole cascade emission. Moreover we also determine the corresponding field squeezing spectrum at the cavity output. These dynamics could be observed as a result of self-organization processes of laser-cooled atoms in resonators. The second part of the thesis studies the quantum ground state of an ultracold atomic gas trapped inside an optical resonator by the mechanical effects of atom-photon interactions. Due to the strong coupling regime, the ultracold atomic gas feels a quantum potential, where the fluctuations at the single photon level may be relevant in determining the trapping conditions. This potential depends on the atomic distribution, which at the same time determines the intracavity field amplitude. Here, after a brief introduction on ultracold atoms in optical lattices, we study the low temperature physics of an ultracold atomic gas in the quantum potential formed inside a pumped cavity, by mapping the dynamics to an effective Bose-Hubbard model. We predict the existence of non-compressible states of the atomic gas, and determine a phase diagram as a function of the cavity parameters. Novel effects are encountered, such as the existence of overlapping stability regions corresponding to competing insulator-like states when the laser pumps the cavity, to provide one example out of many. At the end of the thesis a concluding chapter presents some general outlooks to this thesis work.
Quantum trapping potentials for ultracold gases change the landscape of classical properties of scattered light and matter. The atoms in a quantum many-body correlated phase of matter change the properties of light and vice versa. The properties of both light and matter can be tuned by design and depend on the interplay between long-range (nonlocal) interactions mediated by an optical cavity and short-range processes of the atoms. Moreover, the quantum properties of light get significantly altered by this interplay, leading the light to have nonclassical features. Further, these nonclassical features can be designed and optimised. Introduction and background. Under some of the most extreme experimental conditions of temperature and vacuum, atoms can be controlled by lasers in optical lattices. Beyond controlling the spatial distribution of atoms by light, one can selectively pump at a particular wavelength optimising the interaction with light by several orders of magnitude with additional mirrors. As this occurs, the light in the cavity mediates a true quantum potential that couples all the atoms along the optical lattice, leading to the formation of a quantum optical lattice. The structural arrangement of the atoms can be modified by the light, as photons interact with atoms and vice versa. Main results. In this paper, we concentrate on understanding and showing how the light scattered by the atoms acquires features that are inherently quantum mechanical and originated due to the atomic condensation into a many-body state. The atoms have strong correlations among them as they locally interact and move in the optical lattice in addition to the cavity mediated long-range interaction. We show how one can design and optimise the quantum properties of the scattered light by the atoms, and how it contains information regarding the correlated phases of matter that emerge. Wider Implications. Our results will allow to consider the design of quantum properties of light and the interplay between different energy scales in the system towards the implementation of new quantum simulators, the possibility to optimise these properties for technological applications and ultimately innovate towards possible implementations of quantum system engineering of states.