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Cavity-Modified Super- and Subradiant Rayleigh Scattering of Two Atoms

René Reimann, Wolfgang Alt, Tobias Kampschulte, Tobias Macha, Lothar Ratschbacher, Natalie Thau, Seokchan Yoon, Dieter Meschede

Published Aug 25, 2014• 0 citations
OpenAlex

Abstract

We report on the observation of cooperative radiation of exactly two neutral atoms strongly coupled to the single mode field of an optical cavity, which is close to the lossless-cavity limit. Monitoring the cavity output power, we observe constructive and destructive interference of collective Rayleigh scattering for certain relative distances between the two atoms. Because of cavity backaction onto the atoms, the cavity output power for the constructive two-atom case ($N=2$) is almost equal to the single-emitter case ($N=1$), which is in contrast to free-space where one would expect an $N^2$ scaling of the power. These effects are quantitatively explained by a classical model as well as by a quantum mechanical model based on Dicke states. We extract information on the relative phases of the light fields at the atom positions and employ advanced cooling to reduce the jump rate between the constructive and destructive atom configurations. Thereby we improve the control over the system to a level where the implementation of two-atom entanglement schemes involving optical cavities becomes realistic.

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We report on the observation of cooperative radiation of exactly two neutral atoms strongly coupled to the single mode field of an optical cavity, which is close to the lossless-cavity limit. Monitoring the cavity output power, we observe constructive and destructive interference of collective Rayleigh scattering for certain relative distances between the two atoms. Because of cavity backaction onto the atoms, the cavity output power for the constructive two-atom case (N=2N=2N=2) is almost equal to the single-emitter case (N=1N=1N=1), which is in contrast to free-space where one would expect an N2N^2N2 scaling of the power. These effects are quantitatively explained by a classical model as well as by a quantum mechanical model based on Dicke states. We extract information on the relative phases of the light fields at the atom positions and employ advanced cooling to reduce the jump rate between the constructive and destructive atom configurations. Thereby we improve the control over the system to a level where the implementation of two-atom entanglement schemes involving optical cavities becomes realistic.
We report on the observation of cooperative radiation of exactly two neutral atoms strongly coupled to the single mode field of an optical cavity, which is close to the lossless-cavity limit. Monitoring the cavity output power, we observe constructive and destructive interference of collective Rayleigh scattering for certain relative distances between the two atoms. Because of cavity backaction onto the atoms, the cavity output power for the constructive two-atom case (N=2) is almost equal to the single-emitter case (N=1), which is in contrast to free-space where one would expect an N^{2} scaling of the power. These effects are quantitatively explained by a classical model as well as by a quantum mechanical model based on Dicke states. We extract information on the relative phases of the light fields at the atom positions and employ advanced cooling to reduce the jump rate between the constructive and destructive atom configurations. Thereby we improve the control over the system to a level where the implementation of two-atom entanglement schemes involving optical cavities becomes realistic.
Integrating Rydberg-state control of atom-atom interactions with cavity control of atom-light interactions enables the combination of local entangling operations with photon-mediated long-range coupling, measurement, and communication. Such integration is challenging because electric fields generated by charges on cavity optics and by cavity-stabilizing actuators may disturb Rydberg-state coherence. Here, we couple a Rydberg tweezer array to a high-cooperativity optical cavity, suppressing the electric fields produced by cavity length actuation so that the residual field variation of about 3 mV/cm3~\mathrm{mV/cm}3 mV/cm rms does not limit Rydberg coherence. We demonstrate two capabilities that neither system provides alone. First, we use Purcell-enhanced fluorescence to read out atoms directly in the ground-Rydberg basis within 7.5 μs7.5~μ\mathrm{s}7.5 μs, well within the Rydberg-state lifetime, with ground- and Rydberg-state detection infidelities of 3%3\%3% and 5%5\%5%, respectively, and with low atom loss. Second, we use Rydberg-Rydberg interactions to control collective light-atom scattering into the cavity mode. Specifically, we drive blockaded Rabi oscillations between a state with two ground-state atoms, which scatter collectively with a superradiant or subradiant rate controlled by the atomic positions, and an entangled state with a single Rydberg excitation, which scatters like a single atom. These capabilities open routes toward networked Rydberg processors, mid-circuit measurements in analog quantum simulators, and many-body quantum optics with entangled emitters coupled collectively to light.
We realize collective enhancement and suppression of light scattered by an array of tweezer-trapped ^{87}Rb atoms positioned within a strongly coupled Fabry-Pérot optical cavity. We illuminate the array with light directed transverse to the cavity axis, in the low saturation regime, and detect photons scattered into the cavity. For an array with integer-optical-wavelength spacing each atom scatters light into the cavity with nearly identical scattering amplitude, leading to an observed N^{2} scaling of cavity photon number as the atom number increases stepwise from N=1 to N=8. By contrast, for an array with half-integer-wavelength spacing, destructive interference of scattering amplitudes yields a nonmonotonic, subradiant cavity intensity versus N. By analyzing the polarization of light emitted from the cavity, we find that Rayleigh scattering can be collectively enhanced or suppressed with respect to Raman scattering. We observe also that atom-induced shifts and broadenings of the cavity resonance are precisely tuned by varying the atom number and positions. Altogether, tweezer arrays provide exquisite control of atomic cavity QED spanning from the single- to the many-body regime.
The collective behavior of ensembles of atoms has been studied in-depth since the seminal paper of Dicke [R. H. Dicke, Phys. Rev. 93, 99 (1954)], where he demonstrated that a group of emitters in collective states is able to radiate with increased intensity and modified decay rates in particular directions, a phenomenon which he called superradiance. Here, we show that the fundamental setup of two atoms coupled to a single-mode cavity can be distinctly exceeding the free-space superradiant behavior, a phenomenon which we call hyperradiance. The effect is accompanied by strong quantum fluctuations and surprisingly arises for atoms radiating out-of-phase, an alleged non-ideal condition, where one expects subradiance. We are able to explain the onset of hyperradiance in a transparent way by a photon cascade taking place among manifolds of Dicke states with different photon numbers under particular out-of-phase coupling conditions. The theoretical results can be realized with current technology and thus should stimulate future experiments.
Collective coupling between dipoles can dramatically modify the optical response of a medium. Such effects depend strongly on the geometry of the medium and the polarization of the light. Using a classical coupled dipole model, here we investigate the simplest case of one-dimensional arrays of interacting atomic dipoles driven by a weak laser field. Changing the polarization and direction of the driving field allows us to separately address superradiant, subradiant, redshifted, and blueshifted eigenmodes, as well as observe strong Fano-like interferences between different modes. The cooperative eigenvectors can be characterized by the phase difference between nearest-neighbor dipoles, ranging from all oscillating in phase to all oscillating out of phase with their nearest neighbors. Investigating the eigenvalue behavior as a function of atom number and lattice spacing, we find that certain eigenmodes of an infinite atomic chain have the same decay rate as a single atom between two mirrors. The effects we observe provide a framework for collective control of the optical response of a medium, giving insight into the behavior of more complicated geometries, as well as providing further evidence for the dipolar analog of cavity QED.