Excited state degenerate four-wave mixing in a four-level saturable system is treated theoretically and experimentally. The results show that the external pump feild influences intensely the intensities of the PC signals.
A theoretical description for a forward degenerate four-wave mixing process in homogeneously broadened two-level absorbers with arbitrary intensities of all four beams is presented. Assuming no pump absorption and depletion, we obtain an analytical solution of forward degenerate four-wave mixing signal intensity in the limit of the strong pumps and weak probe and signal. In the case of low absorption or large detuning, this solution is shown to become equivalent to that of the phase-conjugate degenerate four-wave mixing derived by Abrams and Lind [Opt. Lett.2, 94 (1978)]. For arbitrary beam intensities and absorption parameters, the signal intensity is numerically calculated by solution of the coupled equations of complex wave amplitudes. Comparing the results of the numerical calculation with those of the analytical solution, we discuss the validity of using the analytical solution in practical experiments and show the saturation behavior that is due to the strong probe beam. The line shapes under the various ratios among the input beams and absorption parameters are also obtained and discussed.
Transient phase conjugation by degenerate four-wave mixing in saturable dyes is investigated theoretically and experimentally. Two special cases are examined: (1) the case in which two pump waves and a probe wave are simultaneously turned on and (2) the case in which the pump waves are turned on well before the incidence of the probe wave. For case (1) a peak appears in the transient reflectivity for high pump intensity, while for case (2) the reflectivity increases monotonically with time up to the steady-state value irrespective of the value of the pump intensity.