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Journal of the Optical Society of America B

Theory of forward degenerate four-wave mixing in two-level saturable absorbers

Dai‐Hyuk Yu, Jai-Hyung Lee, Joon-Sung Chang, Jae Won HAHN

Published Aug 1, 1999• 11 citations
Publisher

Abstract

A theoretical description for a forward degenerate four-wave mixing process in homogeneously broadened two-level absorbers with arbitrary intensities of all four beams is presented. Assuming no pump absorption and depletion, we obtain an analytical solution of forward degenerate four-wave mixing signal intensity in the limit of the strong pumps and weak probe and signal. In the case of low absorption or large detuning, this solution is shown to become equivalent to that of the phase-conjugate degenerate four-wave mixing derived by Abrams and Lind [Opt. Lett.2, 94 (1978)]. For arbitrary beam intensities and absorption parameters, the signal intensity is numerically calculated by solution of the coupled equations of complex wave amplitudes. Comparing the results of the numerical calculation with those of the analytical solution, we discuss the validity of using the analytical solution in practical experiments and show the saturation behavior that is due to the strong probe beam. The line shapes under the various ratios among the input beams and absorption parameters are also obtained and discussed.

DOI
10.1364/josab.16.001261

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Conference on Lasers and Electro-Optics Pacific Rim (CLEO-PR)•Jan 20, 2003•0 citations
A theoretical description for a forward degenerate four-wave mixing process in homogeneously broadened two-level absorbers with arbitrary intensities of all four beams is presented. Assuming no pump absorption and depletion, we obtain an analytical solution of forward degenerate four-wave mixing signal intensity in the limit of the strong pumps and weak probe and signal. In the case of low absorption or large detuning, this solution is shown to become equivalent to that of the phase-conjugate degenerate four-wave mixing derived by Abrams and Lind [Opt. Lett.2, 94 (1978)]. For arbitrary beam intensities and absorption parameters, the signal intensity is numerically calculated by solution of the coupled equations of complex wave amplitudes. Comparing the results of the numerical calculation with those of the analytical solution, we discuss the validity of using the analytical solution in practical experiments and show the saturation behavior that is due to the strong probe beam. The line shapes under the various ratios among the input beams and absorption parameters are also obtained and discussed.
An analytical expression for the degenerate four-wave mixing signal produced in a medium composed of two-level atoms by pump and probe lasers of arbitrary intensities and parallel linear polarization, suffering negligible absorption and depletion, has been derived. The Abrams–Lind approach [Opt. Lett.2, 94 and 3, 205 (1978)] for deriving the phase-matched polarization has been extended to find all the other higher-order polarization terms contributing to the signal. The signal field amplitude is expressed as an infinite series whose convergence rate depends on the intensity of the input fields and their detuning from resonance. The solution is successfully verified by comparison with a full numerical nonperturbative calculation and is found to be equivalent to the Abrams–Lind result in the limit of weak probe intensity. The result is used to calculate the saturation effects on spectral line shape that are relevant to simulation of molecular spectra obtained by degenerate four-wave mixing with saturating pump and probe fields. The result is extended to treat atomic motion in the case of forward geometry of the input beams.
The coupled equations satisfied by the pump, probe, and signal waves in a four-wave interaction in a two-level saturable absorber are derived, taking into account the effects of absorption and depletion. Numerical solutions of these equations are presented in two limits; one in which the probe-wave amplitude is small compared with that of the pump waves and another in which the probe- and pump-wave amplitudes are comparable. The results indicate that absorption effects are important when the wave amplitudes are less than the saturation amplitude of the absorption process. The importance of the depletion effects depends on the type of four-wave interaction. The most significant effects occur when the undepleted theory predicts probe-wave reflectivities exceeding unity.
We have derived an analytic expression for the intensity distribution of two counterpropagating waves of arbitrary input intensity in a saturable absorber. We use this distribution to extend the theory of degenerate four-wave mixing to include the effects of pump wave absorption. In particular, the spatial variation of the nonlinear absorption and coupling constants that appear in the coupled-amplitude equations for the probe and the signal (i.e., conjugate) waves are determined. These coupled-amplitude equations are solved numerically in a noniterative manner, leading to a prediction for the phase-conjugate reflectivity. The nature of the predictions differs qualitatively from those1,2 derived from theories that ignore pumpwave absorption, especially for the case of off-line-center excitation. At large values of the input pump intensities, the phase conjugate reflectivity can be larger than that predicted by theories that ignore pump-wave absorption.
There is presently a considerable amount of interest in wave conjugation via four-wave mixing in saturable absorbing media. Typically, the four-wave process in volves the interaction, of two counter-propagating pump waves and an Input probe wave via a third-order nonlinearity in the polarization of the medium. Introduction of the probe wave produces a reflected signal wave in the retrodirection. Abrams and Lind have determined the magnitude of the reflected wave obtained from a two-level saturable absorber by solving a set of coupled equations for the probe and signal waves. To obtain this solution, they assumed that the probe and signal waves are weak compared with the pump waves and that the amplitudes of the pumps are constant. In this paper we shall consider the effect of pump attenuation caused by absorption and pump depletion caused by the transfer of energy to the probe and signal waves.
A calculation of degenerate four-wave mixing in a homogeneously broadened two-level saturable absorber is presented. An analytical formula for the local electric dipole polarization responsible for degenerate four-wave mixing is derived for arbitrary electric-field strengths. The overall efficiency of the medium is calculated by numerically solving the coupled wave equations with the use of the phase-matching electric dipole polarization. Solutions are presented when the laser is tuned on and off resonance for various input laser intensities and linear absorption coefficients. Optimal conditions for maximum efficiency are discussed.
Nowadays degenerate four wave mixing (DFWM) with forward geometry (FDFWM) has found increasing usage, for example, in the gas phase detection. In the fields of theoretical development of DFWM, most of the studies have been concentrated on the understanding of phase-conjugated DFWM. However, few theories have dealt with FDFWM. These models calculated the signal directly from the off-diagonal element of the density matrix by assuming optically thin medium. In the paper we obtain a theoretical model for FDFWM in Doppler broadened two-level absorbers including propagation effect and discuss the Doppler effect on the signal intensity and lineshape. Assuming that probe and signal field amplitudes are small compared with those of the pump fields and pump field amplitudes are constant in the interaction volume, we obtain the following coupled equations from the Maxwell equation using the slowly varying envelope approximation and the paraxial approximation.