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Bulletin of the American Physical Society

Phase Diagram of the Spatially Anisotropic Heisenberg Model on a Triangular Lattice

Sedigh Ghamari, Catherine Kallin, Sung-Sik Lee, Erik Schwartz Sørensen

Published Feb 27, 2012• 0 citations
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Ground- and excited-state quantum fidelities in combination with generalized quantum fidelity susceptibilites, obtained from exact diagonalizations, are used to explore the phase diagram of the anisotropic next-nearest-neighbour triangular Heisenberg model. Specifically, the J'-J2 plane of this model, which connects the J1-J2 chain and the anisotropic triangular lattice Heisenberg model, is explored using these quantities. Through the use of a quantum fidelity associated with the first excited-state, in addition to the conventional ground-state fidelity, the BKT-type transition and Majumdar-Ghosh point of the J1-J2 chain (J'=0) are found to extend into the J'-J2 plane and connect with points on the J2=0 axis thereby forming bounded regions in the phase diagram. These bounded regions are then explored through the generalized quantum fidelity susceptibilities χρ, χ₁₂₀°, χD and χCAF which are associated with the spin stiffness, 120° spiral order parameter, dimer order parameter and collinear antiferromagnetic order parameter respectively. These quantities are believed to be extremely sensitive to the underlying phase and are thus well suited for finite-size studies. Analysis of the fidelity susceptibilities suggests that the J', J2≪J phase of the anisotropic triangular model is either a collinear antiferromagnet or possibly a gapless disordered phase that is directly connected to the Luttinger phase of the J1-J2 chain. Furthermore, the outer region is dominated by incommensurate spiral physics as well as dimer order.
Motivated by experiments on nonmagnetic triangular-lattice Mott insulators, we study one candidate paramagnetic phase, namely the columnar dimer (or valence-bond) phase. We apply variants of the bond-operator theory to a dimerized and spatially anisotropic spin-1/2 Heisenberg model and determine its zero-temperature phase diagram and the spectrum of elementary triplet excitations (triplons). Depending on model parameters, we find that the minimum of the triplon energy is located at either a commensurate or an incommensurate wave vector. Condensation of triplons at this commensurate-incommensurate transition defines a quantum Lifshitz point, with effective dimensional reduction that possibly leads to nontrivial paramagnetic (e.g., spin-liquid) states near the closing of the triplet gap. We also discuss the two-particle decay of high-energy triplons, and we comment on the relevance of our results for the organic Mott insulator EtMe3{}_{3}3​P[Pd(dmit)2{}_{2}2​]2{}_{2}2​.