We investigate the anisotropic triangular lattice that interpolates from decoupled one-dimensional chains to the isotropic triangular lattice and has been suggested to be relevant for various quasi-two-dimensional materials such as
Cs2CuCl4 or $\ensuremath{\kappa}\text{\ensuremath{-}}{(ET)}_{2}{\text{Cu}}_{2}{(\text{CN})}_{3}$. We obtain an excellent accuracy by means of a representation for the resonating valence-bond wave function with both singlet and triplet pairings. This approach allows us to establish that the magnetic order is rapidly destroyed away from the pure triangular lattice and incommensurate spin correlations are short range. A nonmagnetic spin liquid naturally emerges in a wide range of the phase diagram with strong one-dimensional character.
We study a system of
N interacting triplons (the elementary excitations of a valence-bond solid) described by an effective interacting boson model derived within the bond operator formalism in order to determine the stability and the properties of many-triplon states. In particular, we consider the square lattice spin-$1/2\phantom{\rule{4pt}{0ex}}{J}_{1}\ensuremath{-}{J}_{2}$ antiferromagnetic Heisenberg model, focus on the intermediate parameter region where a quantum paramagnetic phase sets in, and consider the columnar valence-bond solid as a reference state. Within the bond operator theory, the Heisenberg model is mapped into an effective boson model in terms of triplet operators
t. The effective boson model is studied at the harmonic approximation and the energy of the triplons and the expansion of the triplon operators
b in terms of the triplet operators
t are determined. Such an expansion allows us to perform a second mapping and, therefore, determine an effective interacting boson model in terms of the triplon operators
b. We then consider systems with a fixed number
N of triplons and study the stability of many-triplon states within a mean-field approximation. We show that many-triplon states are stable, the lowest-energy ones are constituted by a small number of triplons, and the excitation gaps are finite. For
J2=0.48J1 and
0.52J1, we also calculate spin-spin and dimer-dimer correlation functions, dimer order parameters, and the bipartite von Neumann entanglement entropy within our mean-field formalism in order to determine the properties of the many-triplon state as a function of the triplon number
N. We find that the spin and the dimer correlations decay exponentially and that the entanglement entropy obeys an area law, regardless of the triplon number
N. Moreover, only for
J2=0.48J1, the spin correlations indicate that the many-triplon states with large triplon number
N might display a more homogeneous singlet pattern than the columnar valence-bond solid. We also comment on possible relations between the many-triplon states with large triplon number
N and gapped spin-liquid states.
We use a combination of numerical density matrix renormalization group calculations and several analytical approaches to comprehensively study a simplified model for a spatially anisotropic spin-
21 triangular lattice Heisenberg antiferromagnet: the three-leg triangular spin tube (TST). The model is described by three Heisenberg chains, with exchange constant
J, coupled antiferromagnetically with exchange constant ${J}^{\ensuremath{'}}$ along the diagonals of the ladder system, with periodic boundary conditions in the shorter direction. Here, we determine the full phase diagram of this model as a function of both spatial anisotropy (between the isotropic and decoupled chain limits) and magnetic field. We find a rich phase diagram, which is remarkably dominated by quantum states: the phase corresponding to the classical ground state appears only in an exceedingly small region. Among the dominant phases generated by quantum effects are commensurate and incommensurate coplanar quasiordered states, which appear in the vicinity of the isotropic region for most fields, and in the high-field region for most anisotropies. The coplanar states, while not classical ground states, can at least be understood semiclassically. Even more strikingly, the largest region of phase space is occupied by a spin density wave phase, which has incommensurate collinear correlations along the field. This phase has no semiclassical analog, and may be ascribed to enhanced one-dimensional fluctuations due to frustration. Cutting across the phase diagram is a magnetization plateau, with a gap to all excitations and ``up-up-down'' spin order, with a quantized magnetization equal to
31 of the saturation value. In the TST, this plateau extends almost but not quite to the decoupled chains limit. Most of the above features are expected to carry over to the two-dimensional system, which we also discuss. At low field, a dimerized phase appears, which is particular to the one-dimensional nature of the TST, and which can be understood from quantum Berry phase arguments.
The nature of quantum spin liquids is studied for the spin-
1/2 antiferromagnetic Heisenberg model on a square lattice containing exchange interactions between nearest-neighbor sites,
J1, and those between next-nearest-neighbor sites,
J2. We perform variational Monte Carlo simulations together with the quantum-number-projection technique and clarify the phase diagram in the ground state together with its excitation spectra. We obtain the nonmagnetic phase in the region
0.4<J2/J1≤0.6 sandwiched by the staggered and stripe antiferromagnetic (AF) phases. Our direct calculations of the spin gap support the notion that the triplet excitation from the singlet ground state is gapless in the range of
0.4<J2/J1≤0.5, while the gapped valence-bond-crystal (VBC) phase is stabilized for
0.5<J2/J1≤0.6. The VBC order is likely to have the columnar symmetry with a spontaneous symmetry breaking of the
C4v symmetry. The power-law behaviors of the spin-spin and dimer-dimer correlation functions in the gapless region are consistent with the emergence of the algebraic quantum-spin-liquid phase (critical phase). The exponent of the spin correlation
⟨S(0)S(r)⟩∝1/rz+η at a long distance
r appears to increase from
z+η∼1 at
J2/J1∼0.4 toward the continuous transition to the VBC phase at
J1/J1∼0.5. Our results, however, do not fully exclude the possibility of a direct quantum transition between the staggered AF and VBC phases with a wide critical region and deconfined criticality.
We extend to magnetically ordered phases a recently developed expansion in
1/d for coupled-dimer Heisenberg magnets, where
d is the number of space dimensions. This extension utilizes generalized bond operators describing spin excitations on top of a reference state involving triplet condensates. We explicitly consider a model of dimers on a hypercubic lattice which displays, in addition to the paramagnetic singlet phase, a collinear antiferromagnetic phase for which we calculate static and dynamic observables at zero temperature. In particular, we show that the
1/d expansion smoothly connects the paramagnetic and antiferromagnetic phases and produces sensible results at and near the quantum phase transition point. Among others, we determine the dispersion and spectral-weight distribution of the amplitude (i.e., Higgs) mode of the ordered phase. In the limit of vanishing intradimer coupling, we connect our approach to spin-wave theory.
We study quantum phase transitions of Mott insulators between spin-glass and featureless paramagnetic phases. Specifically, we consider a triangular-lattice bilayer Heisenberg model with bond disorder. The clean system has two phases, a dimer quantum paramagnet and a non-collinear antiferromagnet, separated by a quantum critical point. Bond disorder destroys the antiferromagnetic phase via the interference of dipolar textures and results in spin-glass order, such that the system features a quantum phase transition between spin-glass and dimer phases. We study the vicinity of this transition using a variant of bond-operator theory and calculate thermodynamic observables as well as excitation spectra. Bond disorder leads to strong inhomogeneities near the transition which suppresses non-collinearities and leads to anomalously weak glassiness in the near-critical quantum spin glass. We characterize the low-energy excitations which have a strong tendency towards spatial localization, and we track the behavior of the amplitude (i.e. Higgs) mode across the glass phase whose spectral weight we find to be strongly suppressed due to interference effects.