Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Excitonic Bell States with Entangled Angular Momenta

Mark T. Lusk

Published Jun 22, 2017• 0 citations
OpenAlex

Abstract

A class of centrosymmetric molecules support excitons with a well-defined quasi-angular momentum. Cofacial arrangements of these molecules can be engineered so that quantum cutting produces a pair of excitons on sandwiching acceptors with angular momenta that are maximally entangled. These Bell state constituents can subsequently travel in opposite directions down molecular chains as ballistic wave packets. This is a direct excitonic analog to the entangled polarization states produced by the spontaneous parametric downconversion of light. As in optical settings, the ability to produce Bell states should enable experiments and technologies based on non-local excitonic quantum correlation. The idea is elucidated with a combination of quantum electrodynamics theory and numerical simulations.

Related papers

Entangled Excitons via Spontaneous Downconversion

Ariel Shlosberg, Mark T. Lusk

molecules support excitons with a well-defined quasi-angular momentum. Cofacial arrangements of these molecules can be engineered so that quantum cutting produces a pair of excitons with angular momenta that are maximally entangled. The Bell state constituents can subsequently travel in opposite directions down molecular chains as ballistic wave packets. This is a direct excitonic analog to the entangled polarization states produced by the spontaneous parametric down-conversion of light. As in optical settings, the ability to produce Bell states should enable foundational experiments and technologies based on non-local excitonic quantum correlation. The idea is elucidated with a combination of quantum electrodynamics theory and numerical simulation.

arXiv:1706.07420•Jun 22, 2017•0 citations

Twisted molecular excitons as mediators for changing the angular momentum of light

Xiaoning Zang, Mark T. Lusk

Molecules with ${C}_{N}$ or ${C}_{Nh}$ symmetry can absorb quanta of optical angular momentum to generate twisted excitons with well-defined quasiangular momenta of their own. Angular momentum is conserved in such interactions at the level of a paraxial approximation for the light beam. A sequence of absorption events can thus be used to create a range of excitonic angular momenta. Subsequent decay can produce radiation with a single angular momentum equal to that accumulated. Such molecules can thus be viewed as mediators for changing the angular momentum of light. This sidesteps the need to exploit nonlinear light-matter interactions based on higher-order susceptibilities. A tight-binding paradigm is used to verify angular momentum conservation and demonstrate how it can be exploited to change the angular momentum of light. The approach is then extended to a time-dependent density functional theory setting where the key results are shown to hold in a many-body, multilevel setting.

arXiv:1703.01844•Physical Review A•Jul 11, 2017•12 citations

High-dimensional angular two-photon interference and angular qudit states

Graciana Puentes

Using angular position–orbital angular momentum entangled photons, we propose an experiment to generate maximally entangled states in D-dimensional quantum systems, the so called qudits, by exploiting correlations of parametric down-converted photons. Angular diffraction masks containing N angular slits in the arms of each twin photon define a qudit space of dimension N2, spanned by the alternative pathways of the photons. Numerical results for N angular slits with N = 2, 4, 5, 10 are reported. We discuss relevant experimental parameters for an experimental implementation of the proposed scheme using Spatial Light Modulators (SLMs), and twin-photons produced by Spontaneous Parametric Down Conversion (SPDC). The entanglement of the qudit state can be quantified in terms of the Concurrence, which can be expressed in terms of the visibility of the interference fringes, or by using Entanglement Witnesses. These results provide an additional means for preparing entangled quantum states in high-dimensions, a fundamental resource for quantum simulation and quantum information protocols.

arXiv:2002.10513•OSA Continuum•May 8, 2020•5 citations

Entanglement of angular momenta of atoms and molecules

Kenji Mishima, Koichi Yamashita

Abstract In this article, we investigate the entanglement degrees of angular momenta of atoms and molecules. We demonstrate theoretically and numerically the guidelines, how to prepare maximally entangled states and how the entanglement of the angular momenta changes by changing the quantum numbers of atoms and molecules. We show that the entanglement degree reduces to the Clebsch–Gordan coefficients frequently encountered in angular momentum theory. The maximally entangled states found in this manner are useful for quantum computers and quantum information science. © 2008 Wiley Periodicals, Inc. Int J Quantum Chem, 2008

International Journal of Quantum Chemistry•Jan 1, 2008•3 citations

Orbital angular momentum of entangled counterpropagating photons

Juan P. Torres, Clara I. Osorio, Lluís Torner

We elucidate the paraxial orbital angular momentum of entangled photon pairs generated by spontaneous parametric downconversion in different noncollinear geometries in which the entangled photons counterpropagate. We find, in particular, the orbital angular momentum of entangled pairs generated in transverse-emitting configurations, in which none of the known rules for selecting orbital angular momentum holds.

Optics Letters•Aug 13, 2004•39 citations

Entanglement of very high orbital angular momentum

Robert Fickler, Peizhe Li, Radek Łapkiewicz +5 more

Orbital angular momentum (OAM) of single photons represents a new optical degree of freedom for the entanglement of photons [1,2]. One physical realization of OAM carrying light beams are the so called Laguerre-Gaussian modes of light with the required helical phase structure. One big advantage over the well known polarization degree of freedom is the possibility of realizing entanglement between two photons with very high quantum numbers. However, the creation of photonic OAM entanglement using the widely used spontaneous parametric downconversion process is limited by the strongly reduced efficiency for higher momenta [3]. We have realized a novel method to create entanglement between two photons with a very high difference in their OAM quantum number and momentum respectively. Furthermore we have explored hybrid entanglement of photons in the OAM and polarization degree of freedom.

Frontiers in Optics•Jan 1, 2011•1 citation
A class of centrosymmetric molecules support excitons with a well-defined quasi-angular momentum. Cofacial arrangements of these molecules can be engineered so that quantum cutting produces a pair of excitons on sandwiching acceptors with angular momenta that are maximally entangled. These Bell state constituents can subsequently travel in opposite directions down molecular chains as ballistic wave packets. This is a direct excitonic analog to the entangled polarization states produced by the spontaneous parametric downconversion of light. As in optical settings, the ability to produce Bell states should enable experiments and technologies based on non-local excitonic quantum correlation. The idea is elucidated with a combination of quantum electrodynamics theory and numerical simulations.
molecules support excitons with a well-defined quasi-angular momentum. Cofacial arrangements of these molecules can be engineered so that quantum cutting produces a pair of excitons with angular momenta that are maximally entangled. The Bell state constituents can subsequently travel in opposite directions down molecular chains as ballistic wave packets. This is a direct excitonic analog to the entangled polarization states produced by the spontaneous parametric down-conversion of light. As in optical settings, the ability to produce Bell states should enable foundational experiments and technologies based on non-local excitonic quantum correlation. The idea is elucidated with a combination of quantum electrodynamics theory and numerical simulation.
Molecules with CN{C}_{N}CN​ or CNh{C}_{Nh}CNh​ symmetry can absorb quanta of optical angular momentum to generate twisted excitons with well-defined quasiangular momenta of their own. Angular momentum is conserved in such interactions at the level of a paraxial approximation for the light beam. A sequence of absorption events can thus be used to create a range of excitonic angular momenta. Subsequent decay can produce radiation with a single angular momentum equal to that accumulated. Such molecules can thus be viewed as mediators for changing the angular momentum of light. This sidesteps the need to exploit nonlinear light-matter interactions based on higher-order susceptibilities. A tight-binding paradigm is used to verify angular momentum conservation and demonstrate how it can be exploited to change the angular momentum of light. The approach is then extended to a time-dependent density functional theory setting where the key results are shown to hold in a many-body, multilevel setting.
Using angular position–orbital angular momentum entangled photons, we propose an experiment to generate maximally entangled states in D-dimensional quantum systems, the so called qudits, by exploiting correlations of parametric down-converted photons. Angular diffraction masks containing N angular slits in the arms of each twin photon define a qudit space of dimension N2, spanned by the alternative pathways of the photons. Numerical results for N angular slits with N = 2, 4, 5, 10 are reported. We discuss relevant experimental parameters for an experimental implementation of the proposed scheme using Spatial Light Modulators (SLMs), and twin-photons produced by Spontaneous Parametric Down Conversion (SPDC). The entanglement of the qudit state can be quantified in terms of the Concurrence, which can be expressed in terms of the visibility of the interference fringes, or by using Entanglement Witnesses. These results provide an additional means for preparing entangled quantum states in high-dimensions, a fundamental resource for quantum simulation and quantum information protocols.
Abstract In this article, we investigate the entanglement degrees of angular momenta of atoms and molecules. We demonstrate theoretically and numerically the guidelines, how to prepare maximally entangled states and how the entanglement of the angular momenta changes by changing the quantum numbers of atoms and molecules. We show that the entanglement degree reduces to the Clebsch–Gordan coefficients frequently encountered in angular momentum theory. The maximally entangled states found in this manner are useful for quantum computers and quantum information science. © 2008 Wiley Periodicals, Inc. Int J Quantum Chem, 2008
Orbital angular momentum (OAM) of single photons represents a new optical degree of freedom for the entanglement of photons [1,2]. One physical realization of OAM carrying light beams are the so called Laguerre-Gaussian modes of light with the required helical phase structure. One big advantage over the well known polarization degree of freedom is the possibility of realizing entanglement between two photons with very high quantum numbers. However, the creation of photonic OAM entanglement using the widely used spontaneous parametric downconversion process is limited by the strongly reduced efficiency for higher momenta [3]. We have realized a novel method to create entanglement between two photons with a very high difference in their OAM quantum number and momentum respectively. Furthermore we have explored hybrid entanglement of photons in the OAM and polarization degree of freedom.