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Single-photon cesium Rydberg excitation spectroscopy by using of 318.6-nm UV laser and room-temperature cesium vapor cell

Jieying Wang, Jiandong Bai, Jun He, Junmin Wang

Published Jun 20, 2017• 0 citations
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Abstract

We demonstrate a single-photon Rydberg excitation spectroscopy of cesium (Cs) atoms in a room-temperature vapor cell. Cs atoms are excited directly from 6S1/2 ground state to nP3/2 (n = 70 - 100) Rydberg states with a 318.6 nm ultraviolet (UV) laser,and Rydberg excitation spectra are obtained by transmission enhancement of a probe beam resonant to Cs 6S1/2, F = 4 - 6P3/2, F' = 5 transition as partial population on F = 4 ground state are transferred to Rydberg state .Analysis reveals that the observed spectra are velocity-selective spectroscopy of Rydberg state, from which the amplitude and linewidth influenced by lasers'Rabi frequency have been investigated. Fitting to energies of Cs nP3/2 (n = 70 -100) states, the determined quantum defect is 3.56671(42). The demodulated spectra can also be employed as frequency references to stabilize the UV laser frequency to specific Cs Rydberg transition.

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(n = 70 -100) states, the determined quantum defect is 3.56671(42). The demodulated spectra can also be employed as frequency references to stabilize the UV laser frequency to specific Cs Rydberg transition.

arXiv:1706.06237•Optics Express•Sep 7, 2017•26 citations

Realization of a watt-level narrow-linewidth 318-nm UV laser and single-photon Rydberg excitation of cesium atoms (Conference Presentation)

Junmin Wang, Jieying Wang, Jiandong Bai +1 more

Nowadays the long-range dipole-dipole interaction between highly-excited Rydberg atoms at micrometer distance become promising way to establish the atom-atom quantum entanglement and to implement the two-qubit logic gate. For alkali metal atoms, single-photon excitation from the ground state to the desired Rydberg state demands powerful narrow-linewidth ultra-violet (UV) laser, which is very challenging. Maybe just because of this, the studies of single-photon Rydberg excitation of alkali metal atoms are rare. Alternatively people have employed the two-photon or three-photon Rydberg excitation scheme. However, comparing with the single-photon Rydberg excitation, the two-photon or three-photon scheme has following drawbacks: atomic decoherence due to the photon scattering from the lower and upper transitions, and light shift of the involved ground state and Rydberg state due to the lower and upper transition laser beams. Thanks to the efficient laser frequency conversion technology with PPXX material and the well-developed commercial fiber laser as well as fiber amplifier, we have implemented a tunable 318.6-nm UV laser system based on the cavity-enhanced second-harmonic generation following the single-pass sum-frequency generation of 1560.5-nm and 1076.9-nm fiber-amplified lasers. More than 2-Watt output of the 318.6-nm UV laser has been achieved with a typical linewidth of smaller than 10 kHz. Employing the UV laser system we have demonstrated a single-photon Rydberg excitation spectroscopy of cesium (Cs) atoms. Partial Cs atoms can be directly excited from 6S_1/2 ground state to nP_3/2 (n = 70 - 100) Rydberg states, and Rydberg excitation spectra are obtained with transmission enhancement of a probe beam locked to Cs 6S_1/2 (F = 4) - 6P_3/2 (F’ = 5) cycling transition because partial population on the ground state (F = 4) are transferred to Rydberg state. The quantum defect for Cs nP_3/2 (n = 70 -100) Rydberg states is determined experimentally. Further more, the demodulated single-photon Rydberg excitation spectrum is employed to stabilize the UV laser to specific Cs Rydberg transition to improve the laser frequency stability. References: [1] Opt. Express 25 (2017) p.22510; [2] J. Opt. 19 (2017) 045501; [3] J. Opt. Soc. Am. B 33 (2016) p.2020; [4] Opt. Commun. 370 (2016) p.150. Funding: the National Natural Science Foundation of China (61475091).

SPIE Conference on Nonlinear Optics and its Applications•May 23, 2018•0 citations

Measurement of quantum defect of cesium nP3/2 (n = 70—94) Rydberg states by using ultraviolet single-photon Rydberg excitation

Shuo Liu, Jiandong Bai, Jieying Wang +2 more

A narrow-linewidth continuous-wave single-frequency tunable 318.6-nm ultraviolet laser system with watt-level output power is developed in our experiment based on well-developed fiber lasers, fiber amplifiers, and efficient laser frequency conversion technique. Cesium 6S1/2—nP3/2 (n = 70—94) single-photon Rydberg excitation in a room-temperature cesium atomic vapor cell is realized by using our ultraviolet laser system. The single-photon Rydberg excitation signal is obtained via the V-type three-level atomic system which contains 6S1/2 (F = 4) ground state, 6P3/2 (F = 5) excited state and one of nP3/2 (n = 70—94) Rydberg states. When cesium atoms populated on the ground state are partially excited to Rydberg state by the ultraviolet laser, absorption of 852.3-nm probe beam which is locked to 6S1/2 (F = 4)—6P3/2 (F ′ = 5) hyperfine transition will decrease. In this way, the cesium Rydberg states are detected. The quantum defects for cesium nP3/2 (n = 70—94) Rydberg states are experimentally measured with a high-precision wavemeter. The variation trend of experimentally measured data deviates from that of calculated values. Due to the fact that the cesium vapor cell is positioned in a magnetic shielding tank, the Zeeman effect can be ignored. Considering that the polarizability of Rydberg atoms is proportional to (n*)7, in which n* is the effective principal quantum number, the Rydberg screen effect of cesium atomic vapor cell cannot completely protect cesium atoms from being perturbed by an external DC electric field. Therefore the residual DC electric field existing inside the cesium vapor cell will have a significant influence on quantum defect measurement of Rydberg atoms. Using the theoretical model of Stark effect and the relationship between polarizability of Rydberg atoms and the effective principal quantum number n*, the corrected experimental value of quantum defect for cesium nP3/2 (n = 70—94) Rydberg states is found to be ~(3.5591 ± 0.0007). The corrected experimental value of quantum defect is consistent with the calculation.

Acta Physica Sinica•Jan 1, 2019•1 citation

Single-photon Rydberg excitation spectra of cesium atomic vapor with a 319nm ultra-violet laser

iandong Bai, Jieying Wang, Shuo Liu +2 more

We demonstrate the single-photon excitation spectra of cesium Rydberg atoms by means of a Doppler-free purely all-optical detection with a room-temperature vapor cell and a 319 nm ultra-violet (UV) laser. We excite atoms directly from 6S1/2 ground state to 71P3/2 Rydberg state with a narrow-linewidth 319 nm UV laser. The detection of Rydberg states is performed by monitoring the absorption of an 852 nm probe beam in a V-type three-level system. With a strong coupling light, we observe the Autler-Townes (AT) doublet, and the dependences of the separation and linewidths on the coupling intensity are experimentally investigated, which is consistent with the prediction based on the dressed state theory. Moreover, the AT splitting can be used to measure the Rabi frequency. In an external magnetic field, the Rydberg spectra of nondegenerate Zeeman sublevels are demonstrated. The splitting of the spectrum is of great significance for studying the characteristics of Rydberg atoms.

•Jun 1, 2018•0 citations

Measurement of the fine structure of cesium Rydberg state

Dong-Liang Pei, Jun He, Jieying Wang +2 more

The spectra of Rydberg atoms are of great significance for studying the energy levels of Rydberg atoms and the interaction between neutral atoms, especially, the high-precision spectra of Rydberg atoms can be used to measure the energy level shifts of Rydberg atoms resulting from the dipole-dipole interactions in room-temperature vapor cells. In this paper we report the preparation of cesium Rydberg states based on the cascaded two-photon excitation of 509 nm laser and 852 nm laser in opposite, and the measurements of the fine structure of cesium Rydberg states. In this experiment, the 509 nm laser is generated by the cavity-enhanced second-harmonic generation from 1018 nm laser with a periodically-poled KTP crystal and has a maximum power of about 1 W, and the 852 nm probe laser is provided by an external-cavity diode laser with a maximum output power of 5 mW and a typical linewidth of 1 MHz. By scanning the frequency of 509 nm coupling laser, it is presented that the Doppler-free spectra based on electromagnetically-induced transparency (EIT) of 509 nm coupling laser and 852 nm probe laser. The velocity-selective EIT spectra are used to study the spectral splitting of 6S1/26P3/257S(D) ladder-type system of cesium Rydberg atoms in a room-temperature vapor cell. The powers of 852 nm probe laser and 509 nm coupling laser are 0.3 upW and 200 mW, respectively. Their waist radii are both approximately 50 m. The intervals of hyperfine splitting of the intermediate state 6P3/2(F'=3, 4, 5) and fine splitting of 57D3/2 and 57D5/2 Rydberg states are measured by a frequency calibrating. Concretely, the velocity-selective spectrum with a radio frequency (RF) modulation of 30 MHz is used as a reference to calibrate the Rydberg fine-structure states in the hot vapor cell, where the RF frequency precision is smaller than a hertz on long time scales and the EIT linewidth is smaller than 13 MHz. The experimental value of the fine structure splitting of 57D3/2 and 57D5/2 Rydberg states is (354.72.5) MHz, that is in consistence with the value of 346.8 MHz calculated by Rydberg-Ritz equation and quantum defects of 57D3/2 and 57D5/2 Rydberg states. The experimental values of hyperfine splitting of intermediate state 6P3/2(F'=3, 4, 5) are also coincident with the theoretical calculated values. The dominant discrepancy existing between the experimental and calculated results may arise from the nonlinear correspondence of the PZT while the 509 nm wavelength cavity is scanned, and the measurement accuracy influenced by the spectral linewidth. The velocity-selective spectroscopy technique can also be used to measure the energy level shifts caused by the interactions of Rydberg atoms.

Acta Physica Sinica•Jan 1, 2017•6 citations

Nonlinear spectroscopy of three-photon excitation of cesium Rydberg atoms in vapor cell*

Jiabei Fan, Yunhui He, Yuechun Jiao +3 more

We present nonlinear spectra of four-level ladder cesium atoms employing 6S 1/2 → 6P 3/2→ 7S 1/2 → 30P 3/2 scheme of a room temperature vapor cell. A coupling laser drives Rydberg transition, a dressing laser couples two intermediate levels, and a probe laser optically probes the nonlinear spectra via electromagnetically induced transparency (EIT). Nonlinear spectra are detected as a function of coupling laser frequency. The observed spectra exhibit an enhanced absorption (EA) signal at coupling laser resonance to Rydberg transition and enhanced transmission (ET) signals at detunings to the transition. We define the enhanced absorption (transmission) strength, H EA (H ET), and distance between two ET peaks, γ ET, to describe the spectral feature of the four-level atoms. The enhanced absorption signal H EA is found to have a maximum value when we vary the dressing laser Rabi frequency Ω d, corresponding Rabi frequency is defined as a separatrix point, Ω dSe . The values of Ω dSe and further η = Ω dSe /Ω c are found to depend on the probe and coupling Rabi frequency but not the atomic density. Based on Ω dSe , the spectra can be separated into two regimes, weak and strong dressing ranges, Ω d ≲ Ω dSe and Ω d ≳ Ω dSe , respectively. The spectroscopies display different features at these two regimes. A four-level theoretical model is developed that agrees well with the experimental results in terms of the probe-beam absorption behavior of Rabi frequency-dependent dressed states.

Chinese Physics B•Nov 13, 2020•10 citations
We demonstrate a single-photon Rydberg excitation spectroscopy of cesium (Cs) atoms in a room-temperature vapor cell. Cs atoms are excited directly from 6S1/2 ground state to nP3/2 (n = 70 - 100) Rydberg states with a 318.6 nm ultraviolet (UV) laser,and Rydberg excitation spectra are obtained by transmission enhancement of a probe beam resonant to Cs 6S1/2, F = 4 - 6P3/2, F' = 5 transition as partial population on F = 4 ground state are transferred to Rydberg state .Analysis reveals that the observed spectra are velocity-selective spectroscopy of Rydberg state, from which the amplitude and linewidth influenced by lasers'Rabi frequency have been investigated. Fitting to energies of Cs nP3/2 (n = 70 -100) states, the determined quantum defect is 3.56671(42). The demodulated spectra can also be employed as frequency references to stabilize the UV laser frequency to specific Cs Rydberg transition.
Nowadays the long-range dipole-dipole interaction between highly-excited Rydberg atoms at micrometer distance become promising way to establish the atom-atom quantum entanglement and to implement the two-qubit logic gate. For alkali metal atoms, single-photon excitation from the ground state to the desired Rydberg state demands powerful narrow-linewidth ultra-violet (UV) laser, which is very challenging. Maybe just because of this, the studies of single-photon Rydberg excitation of alkali metal atoms are rare. Alternatively people have employed the two-photon or three-photon Rydberg excitation scheme. However, comparing with the single-photon Rydberg excitation, the two-photon or three-photon scheme has following drawbacks: atomic decoherence due to the photon scattering from the lower and upper transitions, and light shift of the involved ground state and Rydberg state due to the lower and upper transition laser beams. Thanks to the efficient laser frequency conversion technology with PPXX material and the well-developed commercial fiber laser as well as fiber amplifier, we have implemented a tunable 318.6-nm UV laser system based on the cavity-enhanced second-harmonic generation following the single-pass sum-frequency generation of 1560.5-nm and 1076.9-nm fiber-amplified lasers. More than 2-Watt output of the 318.6-nm UV laser has been achieved with a typical linewidth of smaller than 10 kHz. Employing the UV laser system we have demonstrated a single-photon Rydberg excitation spectroscopy of cesium (Cs) atoms. Partial Cs atoms can be directly excited from 6S_1/2 ground state to nP_3/2 (n = 70 - 100) Rydberg states, and Rydberg excitation spectra are obtained with transmission enhancement of a probe beam locked to Cs 6S_1/2 (F = 4) - 6P_3/2 (F’ = 5) cycling transition because partial population on the ground state (F = 4) are transferred to Rydberg state. The quantum defect for Cs nP_3/2 (n = 70 -100) Rydberg states is determined experimentally. Further more, the demodulated single-photon Rydberg excitation spectrum is employed to stabilize the UV laser to specific Cs Rydberg transition to improve the laser frequency stability. References: [1] Opt. Express 25 (2017) p.22510; [2] J. Opt. 19 (2017) 045501; [3] J. Opt. Soc. Am. B 33 (2016) p.2020; [4] Opt. Commun. 370 (2016) p.150. Funding: the National Natural Science Foundation of China (61475091).
A narrow-linewidth continuous-wave single-frequency tunable 318.6-nm ultraviolet laser system with watt-level output power is developed in our experiment based on well-developed fiber lasers, fiber amplifiers, and efficient laser frequency conversion technique. Cesium 6S1/2—nP3/2 (n = 70—94) single-photon Rydberg excitation in a room-temperature cesium atomic vapor cell is realized by using our ultraviolet laser system. The single-photon Rydberg excitation signal is obtained via the V-type three-level atomic system which contains 6S1/2 (F = 4) ground state, 6P3/2 (F = 5) excited state and one of nP3/2 (n = 70—94) Rydberg states. When cesium atoms populated on the ground state are partially excited to Rydberg state by the ultraviolet laser, absorption of 852.3-nm probe beam which is locked to 6S1/2 (F = 4)—6P3/2 (F ′ = 5) hyperfine transition will decrease. In this way, the cesium Rydberg states are detected. The quantum defects for cesium nP3/2 (n = 70—94) Rydberg states are experimentally measured with a high-precision wavemeter. The variation trend of experimentally measured data deviates from that of calculated values. Due to the fact that the cesium vapor cell is positioned in a magnetic shielding tank, the Zeeman effect can be ignored. Considering that the polarizability of Rydberg atoms is proportional to (n*)7, in which n* is the effective principal quantum number, the Rydberg screen effect of cesium atomic vapor cell cannot completely protect cesium atoms from being perturbed by an external DC electric field. Therefore the residual DC electric field existing inside the cesium vapor cell will have a significant influence on quantum defect measurement of Rydberg atoms. Using the theoretical model of Stark effect and the relationship between polarizability of Rydberg atoms and the effective principal quantum number n*, the corrected experimental value of quantum defect for cesium nP3/2 (n = 70—94) Rydberg states is found to be ~(3.5591 ± 0.0007). The corrected experimental value of quantum defect is consistent with the calculation.
We demonstrate the single-photon excitation spectra of cesium Rydberg atoms by means of a Doppler-free purely all-optical detection with a room-temperature vapor cell and a 319 nm ultra-violet (UV) laser. We excite atoms directly from 6S1/2 ground state to 71P3/2 Rydberg state with a narrow-linewidth 319 nm UV laser. The detection of Rydberg states is performed by monitoring the absorption of an 852 nm probe beam in a V-type three-level system. With a strong coupling light, we observe the Autler-Townes (AT) doublet, and the dependences of the separation and linewidths on the coupling intensity are experimentally investigated, which is consistent with the prediction based on the dressed state theory. Moreover, the AT splitting can be used to measure the Rabi frequency. In an external magnetic field, the Rydberg spectra of nondegenerate Zeeman sublevels are demonstrated. The splitting of the spectrum is of great significance for studying the characteristics of Rydberg atoms.
The spectra of Rydberg atoms are of great significance for studying the energy levels of Rydberg atoms and the interaction between neutral atoms, especially, the high-precision spectra of Rydberg atoms can be used to measure the energy level shifts of Rydberg atoms resulting from the dipole-dipole interactions in room-temperature vapor cells. In this paper we report the preparation of cesium Rydberg states based on the cascaded two-photon excitation of 509 nm laser and 852 nm laser in opposite, and the measurements of the fine structure of cesium Rydberg states. In this experiment, the 509 nm laser is generated by the cavity-enhanced second-harmonic generation from 1018 nm laser with a periodically-poled KTP crystal and has a maximum power of about 1 W, and the 852 nm probe laser is provided by an external-cavity diode laser with a maximum output power of 5 mW and a typical linewidth of 1 MHz. By scanning the frequency of 509 nm coupling laser, it is presented that the Doppler-free spectra based on electromagnetically-induced transparency (EIT) of 509 nm coupling laser and 852 nm probe laser. The velocity-selective EIT spectra are used to study the spectral splitting of 6S1/26P3/257S(D) ladder-type system of cesium Rydberg atoms in a room-temperature vapor cell. The powers of 852 nm probe laser and 509 nm coupling laser are 0.3 upW and 200 mW, respectively. Their waist radii are both approximately 50 m. The intervals of hyperfine splitting of the intermediate state 6P3/2(F'=3, 4, 5) and fine splitting of 57D3/2 and 57D5/2 Rydberg states are measured by a frequency calibrating. Concretely, the velocity-selective spectrum with a radio frequency (RF) modulation of 30 MHz is used as a reference to calibrate the Rydberg fine-structure states in the hot vapor cell, where the RF frequency precision is smaller than a hertz on long time scales and the EIT linewidth is smaller than 13 MHz. The experimental value of the fine structure splitting of 57D3/2 and 57D5/2 Rydberg states is (354.72.5) MHz, that is in consistence with the value of 346.8 MHz calculated by Rydberg-Ritz equation and quantum defects of 57D3/2 and 57D5/2 Rydberg states. The experimental values of hyperfine splitting of intermediate state 6P3/2(F'=3, 4, 5) are also coincident with the theoretical calculated values. The dominant discrepancy existing between the experimental and calculated results may arise from the nonlinear correspondence of the PZT while the 509 nm wavelength cavity is scanned, and the measurement accuracy influenced by the spectral linewidth. The velocity-selective spectroscopy technique can also be used to measure the energy level shifts caused by the interactions of Rydberg atoms.
We present nonlinear spectra of four-level ladder cesium atoms employing 6S 1/2 → 6P 3/2→ 7S 1/2 → 30P 3/2 scheme of a room temperature vapor cell. A coupling laser drives Rydberg transition, a dressing laser couples two intermediate levels, and a probe laser optically probes the nonlinear spectra via electromagnetically induced transparency (EIT). Nonlinear spectra are detected as a function of coupling laser frequency. The observed spectra exhibit an enhanced absorption (EA) signal at coupling laser resonance to Rydberg transition and enhanced transmission (ET) signals at detunings to the transition. We define the enhanced absorption (transmission) strength, H EA (H ET), and distance between two ET peaks, γ ET, to describe the spectral feature of the four-level atoms. The enhanced absorption signal H EA is found to have a maximum value when we vary the dressing laser Rabi frequency Ω d, corresponding Rabi frequency is defined as a separatrix point, Ω dSe . The values of Ω dSe and further η = Ω dSe /Ω c are found to depend on the probe and coupling Rabi frequency but not the atomic density. Based on Ω dSe , the spectra can be separated into two regimes, weak and strong dressing ranges, Ω d ≲ Ω dSe and Ω d ≳ Ω dSe , respectively. The spectroscopies display different features at these two regimes. A four-level theoretical model is developed that agrees well with the experimental results in terms of the probe-beam absorption behavior of Rabi frequency-dependent dressed states.