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Bulletin of the American Physical Society

Ultracold and ultrafast: Probing quantum gases with femtosecond laser pulses

Philipp Wessels, Bernhard Ruff, Tobias Kroker, Steffen Pehm oller, Juliette Simonet, Markus Drescher, K. Sengstock

Published Jun 8, 2017• 0 citations
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Abstract Understanding Coulomb driven many-body dynamics in ultracold atomic systems far from equilibrium remains an open challenge, particularly when ultrafast excitation channels create competing pathways toward Rydberg gases or ultracold plasmas. Here, we investigate the many-body dynamics in a 87 Rb Bose-Einstein condensate after exposure to a single femtosecond laser pulse. By tuning the laser wavelength across the two-photon ionization threshold, we can control the initial state that is either dominated by free electrons and leads to an ultracold plasma or dominated by electrons in excited states which leads to a dense Rydberg gas. The large bandwidth enables overcoming the Rydberg blockade that limits the excitation density for narrow-linewidth lasers. We directly measure the kinetic energy of the released electrons and compare the final distribution of free, bound and plasma electrons to molecular dynamics simulations where the electrons are modeled as individual particles including collisional ionization and recombination processes. We find very good agreement between the simulated electron distribution and the experimental observation. We identify charge imbalance as main driver for the decay of a dense Rydberg gas into an ultracold plasma.
We have studied the effects of chirped femtosecond laser pulses on the formation of ultracold molecules in a Rb magneto-optical trap. We have found that application of chirped femtosecond pulses suppressed the formation of (85)Rb and (87)Rb(2) a(3)sigma(+)(u) molecules in contrast to comparable nonchirped pulses, cw illumination, and background formation rates. Variation of the amount of chirp indicated that this suppression is coherent in nature, suggesting that coherent control is likely to be useful for manipulating the dynamics of ultracold quantum molecular gases.