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Bulletin of the American Physical Society

Two-Photon Polarization Spectroscopy of atomic Cs over the $6s^{2}S_{1/2}\rightarrow6p^{2}P_{3/2}\rightarrow9d^{2}D_{5/2}$ transition

M. J. Welsh, Seda Kin, Jacob D Hinkle, Servet Bayram

Published Apr 9, 2005• 0 citations
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An experimental investigation of the Cs $6s\phantom{\rule{0.2em}{0ex}}^{2}S_{1∕2}\ensuremath{\rightarrow}6p\phantom{\rule{0.2em}{0ex}}^{2}P_{3∕2}\ensuremath{\rightarrow}10s\phantom{\rule{0.2em}{0ex}}^{2}S_{1∕2}$ double-resonance two-photon polarization spectrum has been made. In the investigation, a linear polarization degree was measured to extract the alignment depolarization cross section in the cesium $6p\phantom{\rule{0.2em}{0ex}}^{2}P_{3∕2}$ level due to collisions between ground-level argon and excited $6p\phantom{\rule{0.2em}{0ex}}^{2}P_{3∕2}$ cesium atoms over the Zeeman coherences. The spectra show strong depolarization of the Cs $6p\phantom{\rule{0.2em}{0ex}}^{2}P_{3∕2}$ level. The measured alignment depolarization cross section value of 186 $(58)\phantom{\rule{0.3em}{0ex}}{\mathrm{\AA{}}}^{2}$ is in good agreement with the experiment and theoretical predictions.

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Power dependence of multi-photon processes in the 5S1/2−5P3/2−5D5/25S_{1/2}-5P_{3/2}-5D_{5/2}5S1/2​−5P3/2​−5D5/2​ transition of 87^{87}87Rb atoms
The polarization dependence of double-resonance optical pumping (DROP) in the ladder-type electromagnetically induced transparency (EIT) of the $5{S}_{1/2}\ensuremath{-}5{P}_{3/2}\ensuremath{-}5{D}_{5/2}$ transition of 87{}^{87}87Rb atoms is studied. The transmittance spectra in the $5{S}_{1/2}(F=2)\ensuremath{-}5{P}_{3/2}({F}^{\ensuremath{'}}=3)\ensuremath{-}5{D}_{5/2}({F}^{\ensuremath{'}\ensuremath{'}}=2,3,4)$ transition were observed as caused by EIT, DROP, and saturation effects in the various polarization combinations between the probe and coupling lasers. The features of the double-structure transmittance spectra in the $5{S}_{1/2}(F=2)\ensuremath{-}5{P}_{3/2}({F}^{\ensuremath{'}}=3)\ensuremath{-}5{D}_{5/2}({F}^{\ensuremath{'}\ensuremath{'}}=4)$ cycling transition were attributed to the difference in saturation effect according to the transition routes between the Zeeman sublevels and the EIT according to the two-photon transition probability.
An experimental investigation of the Cs $6s\phantom{\rule{0.2em}{0ex}}^{2}S_{1∕2}\ensuremath{\rightarrow}6p\phantom{\rule{0.2em}{0ex}}^{2}P_{3∕2}\ensuremath{\rightarrow}10s\phantom{\rule{0.2em}{0ex}}^{2}S_{1∕2}$ double-resonance two-photon polarization spectrum has been made. In the investigation, a linear polarization degree was measured to extract the alignment depolarization cross section in the cesium 6p2P3∕26p\phantom{\rule{0.2em}{0ex}}^{2}P_{3∕2}6p2P3∕2​ level due to collisions between ground-level argon and excited 6p2P3∕26p\phantom{\rule{0.2em}{0ex}}^{2}P_{3∕2}6p2P3∕2​ cesium atoms over the Zeeman coherences. The spectra show strong depolarization of the Cs 6p2P3∕26p\phantom{\rule{0.2em}{0ex}}^{2}P_{3∕2}6p2P3∕2​ level. The measured alignment depolarization cross section value of 186 (58)A˚2(58)\phantom{\rule{0.3em}{0ex}}{\mathrm{\AA{}}}^{2}(58)A˚2 is in good agreement with the experiment and theoretical predictions.