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What are zero energy excitations in high-$T_{c}$ superconductors?

Yu. G. Pogorelov, M. C. Santos, В. М. Локтев

Published May 16, 2006• 0 citations
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Abstract

The long disputed issue of the limiting value of quasiparticle density of states $\r(0) = \r (\e \to 0)$ in a \emph{d-}wave superconductor with impurities (\emph{vs} its linear vanishing, $\r_0(\e) \propto |\e|/\D$, near the nodal point $\e = 0$ in a pure system with the gap parameter $\D$) is discussed. Using the technique of group expansions of Green functions in complexes of interacting impurities, it is shown that finite $\r(0)$ value is possible if the (finite) impurity perturbation $V$ is spin-dependent (magnetic). The found value has a power law dependence on the impurity concentration $c$: $\r(0) \propto \r_N c^{n}$, where $\r_N$ is the normal metal density of states and $n \geq 2$ is the least number of impurities in a complex that can localize nodal quasiparticle. This result essentially differs from the known predictions of self-consistent approximation: $\r(0) \propto \r_N \sqrt {c/\r_N\D}$ (for the unitary limit $V \to \infty$) or $\r(0) \propto (\D/cV^2)\exp(-\D/cV^2\r_N)$ (for the Born limit $|V|\r_N \ll 1$). We predict also existence of a narrow interval (mobility gap) around the Fermi energy, where all the states are localized on proper impurity clusters, leading to exponential suppression of low-temperature kinetics.

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Impurity clusters and localization of nodal quasiparticles in \emph{d}-wave superconductors

Yu. G. Pogorelov, M. C. Santos, В. М. Локтев

The long disputed issue of the limiting value of quasiparticle density of states $\r(0) = \r (\e \to 0)$ in a \emph{d-}wave superconductor with impurities (\emph{vs} its linear vanishing, $\r_0(\e) \propto |\e|/\D$, near the nodal point $\e = 0$ in a pure system with the gap parameter $\D$) is discussed. Using the technique of group expansions of Green functions in complexes of interacting impurities, it is shown that finite $\r(0)$ value is possible if the (finite) impurity perturbation $V$ is spin-dependent (magnetic). The found value has a power law dependence on the impurity concentration $c$: $\r(0) \propto \r_N c^{n}$, where $\r_N$ is the normal metal density of states and $n \geq 2$ is the least number of impurities in a complex that can localize nodal quasiparticle. This result essentially differs from the known predictions of self-consistent approximation: $\r(0) \propto \r_N \sqrt {c/\r_N\D}$ (for the unitary limit $V \to \infty$) or $\r(0) \propto (\D/cV^2)\exp(-\D/cV^2\r_N)$ (for the Born limit $|V|\r_N \ll 1$). We predict also existence of a narrow interval (mobility gap) around the Fermi energy, where all the states are localized on proper impurity clusters, leading to exponential suppression of low-temperature kinetics.

arXiv:cond-mat/0605424•May 16, 2006•0 citations

Impurity States and the Absence of Quasiparticle Localization in Disorderedd-Wave Superconductors

Alexander V. Balatsky, M. I. Salkola

The absence of localization of impurity-induced low-energy quasiparticle states in a 2D d-wave superconductor is shown for any amount of disorder in the limit of unitary scatterers. This result follows from the fact that a unitary impurity produces a marginally bound state at zero energy which decays as a power law along the nodes of the d-wave energy gap. Consequently, for finite density of impurities, the impurity-induced states are coupled by long-range overlaps yielding extended quasiparticle states below a characteristic energy scale ${\ensuremath{\omega}}_{c}$. Simple scaling arguments suggest that ${\ensuremath{\omega}}_{c}\ensuremath{\propto}{e}^{{\ensuremath{-}c/n}_{\mathrm{imp}}}$, with ${n}_{\mathrm{imp}}$ the impurity density and c a positive constant.

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Nodal quasiparticles in doped d-wave superconductors: self-consistent T-matrix approach

В. М. Локтев, Yu. G. Pogorelov

A comparative analysis has been done of the formerly established two self-consistent solutions for the density of quasiparticle states in doped d-wave superconductors, having strikingly different and disputed behavior near the Fermi energy. One of them (1) remains finite in this limit, while the other (2) tends to zero. To resolve this discrepancy, the known Ioffe-Regel criterion for band states, widely used for doped semiconductors, was applied to these solutions. It is shown that both them are valid in limited and different energy regions, where the corresponding quasiparticles are weakly damped. In particular, density of states of nodal quasiparticles near the Fermi level is provided by the (2) solution, while the (1) only applies far enough from this level.

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Superconductor-insulator transition and energy localization

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We develop an analytical theory for generic disorder-driven quantum phase transitions. We apply this formalism to the superconductor-insulator transition and we briefly discuss the applications to the order-disorder transition in quantum magnets. The effective spin-$\frac{1}{2}$ models for these transitions are solved in the cavity approximation which becomes exact on a Bethe lattice with large branching number $K⪢1$ and weak dimensionless coupling $g⪡1$. The characteristic feature of the low-temperature phase is a large self-formed inhomogeneity of the order-parameter distribution near the critical point $K\ensuremath{\ge}{K}_{c}(g)$, where the critical temperature ${T}_{c}$ of the ordering transition vanishes. We find that the local probability distribution $P(B)$ of the order parameter $B$ has a long power-law tail in the region where $B$ is much larger than its typical value ${B}_{0}$. Near the quantum-critical point, at $K\ensuremath{\rightarrow}{K}_{c}(g)$, the typical value of the order parameter vanishes exponentially, ${B}_{0}\ensuremath{\propto}{e}^{\ensuremath{-}C/[K\ensuremath{-}{K}_{c}(g)]}$ while the spatial scale ${N}_{inh}$ of the order parameter inhomogeneities diverges as ${[K\ensuremath{-}{K}_{c}(g)]}^{\ensuremath{-}2}$. In the disordered regime, realized at $K<{K}_{c}(g)$ we find actually two distinct phases characterized by different behavior of relaxation rates. The first phase exists in an intermediate range of ${K}^{\ensuremath{\ast}}(g)<K<{K}_{c}(g)$. It has two regimes of energies: at low excitation energies, $\ensuremath{\omega}<{\ensuremath{\omega}}_{d}(K,g)$, the many-body spectrum of the model is discrete, with zero-level widths, while at $\ensuremath{\omega}>{\ensuremath{\omega}}_{d}$ the level acquire a nonzero width which is self-generated by the many-body interactions. In this phase the spin model provides by itself an intrinsic thermal bath. Another phase is obtained at smaller $K<{K}^{\ensuremath{\ast}}(g)$, where all the eigenstates are discrete, corresponding to full many-body localization. These results provide an explanation for the activated behavior of the resistivity in amorphous materials on the insulating side near the superconductor-insulator transition and a semiquantitative description of the scanning tunneling data on its superconductive side.

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Impurity scattering and localization in d -wave superconductors

Marcel Franz, Catherine Kallin, A. J. Berlinsky

Strong evidence is presented for the localization of low-energy quasiparticle states in disordered $d$-wave superconductors. Within the framework of the Bogoliubov-de Gennes (BdG) theory applied to the extended Hubbard model with a finite concentration of nonmagnetic impurities, we carry out a fully self-consistent numerical diagonalization of the BdG equations on finite clusters containing up to 50\ifmmode\times\else\texttimes\fi{}50 sites. Localized states are identified by probing their sensitivity to the boundary conditions and by analyzing the finite-size dependence of inverse participation ratios.

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Modeling the dynamics of quasiparticles in superconducting devices at low temperatures

Fischer, Paul Benedikt

Superconducting materials are useful for a wide range of applications, ranging from particle detectors to quantum computing. The presence of excitations (quasiparticles) in the superconductor can be a resource in some devices and a disturbance in others - in kinetic inductance detectors, the generation of quasiparticles by an incoming photon can be read out and used to calculate the energy of the photon, while the tunnelling of quasiparticles is a cause of decoherence in quantum computing. While early research mostly focused on superconductors close to the critical temperature, temperatures that are far below the critical temperatures are often used for current applications. At these low temperatures, the energy exchange between quasiparticles and phonons becomes slow, and even small disturbances may drive the energy distribution of the quasiparticles out of thermal equilibrium. In fact, experiments usually show a residual number of quasiparticles even at milikelvin temperatures, for which the thermal density of quasiparticles would be negligible. This thesis consists of two parts: In the first part, I model the energy distribution of quasiparticles in superconducting resonators: Quasiparticles absorb energy by absorbing photons and release it as phonons, which drives the superconductor out of thermal equilibrium. I solve a set of rate equations, both numerical and analytical, to calculate the energy distribution of the quasiparticles. For parameters typically used in kinetic inductance detectors made of aluminum, the microwave signal used to read out the resonator dominates the energy distribution of the quasiparticles, while their density is determined by other processes. At not too low temperatures, quasiparticles are mainly produced by thermal phonons, and my calculations reproduce recently measured quality factors of resonators at temperatures above 250 mK without free parameters. I show that even a very small number of photons of higher energy, which I ascribe to noise from the microwave generator, would dominate the quasiparticle density at lower temperatures. Under this assumption, my calculations also reproduce the quality factors at lower temperatures. In the second part of this thesis, I investigate the effects of spatial fluctuations of the superconducting energy gap on the dynamics of quasiparticles. Recently, it has been proposed that such fluctuations may lead to the localization of quasiparticles in states below the energy gap, which could cause a finite quasiparticle density even at very low temperatures. Using the Keldysh-Usadel formalism, I derive rates for the different processes (recombination/(de-) localization/generation) of quasiparticles in such systems. Using these rate equations I derive new upper limits for the quasiparticle density that could result from these localized states. These upper limits show that localization caused by weak magnetic impurities in typical aluminum systems does not lead to a relevant quasiparticle density. This contradicts previous theories, which only consider the recombination between two localized quasiparticles without examining their dynamics in detail.

•Jan 1, 2025•0 citations
What are zero energy excitations in high-TcT_{c}Tc​ superconductors?
The long disputed issue of the limiting value of quasiparticle density of states (˚0)=(˚\e→0)\r(0) = \r (\e \to 0)(˚​0)=(˚​\e→0) in a \emph{d-}wave superconductor with impurities (\emph{vs} its linear vanishing, \r_0(\e) \propto |\e|/\D, near the nodal point \e=0\e = 0\e=0 in a pure system with the gap parameter \D\D\D) is discussed. Using the technique of group expansions of Green functions in complexes of interacting impurities, it is shown that finite (˚0)\r(0)(˚​0) value is possible if the (finite) impurity perturbation VVV is spin-dependent (magnetic). The found value has a power law dependence on the impurity concentration ccc: \r(0) \propto \r_N c^{n}, where \r_N is the normal metal density of states and n≥2n \geq 2n≥2 is the least number of impurities in a complex that can localize nodal quasiparticle. This result essentially differs from the known predictions of self-consistent approximation: \r(0) \propto \r_N \sqrt {c/\r_N\D} (for the unitary limit V→∞V \to \inftyV→∞) or \r(0) \propto (\D/cV^2)\exp(-\D/cV^2\r_N) (for the Born limit |V|\r_N \ll 1). We predict also existence of a narrow interval (mobility gap) around the Fermi energy, where all the states are localized on proper impurity clusters, leading to exponential suppression of low-temperature kinetics.
The long disputed issue of the limiting value of quasiparticle density of states $\r(0) = \r (\e \to 0)$ in a \emph{d-}wave superconductor with impurities (\emph{vs} its linear vanishing, $\r_0(\e) \propto |\e|/\D$, near the nodal point $\e = 0$ in a pure system with the gap parameter $\D$) is discussed. Using the technique of group expansions of Green functions in complexes of interacting impurities, it is shown that finite (˚0)\r(0)(˚​0) value is possible if the (finite) impurity perturbation VVV is spin-dependent (magnetic). The found value has a power law dependence on the impurity concentration ccc: $\r(0) \propto \r_N c^{n}$, where $\r_N$ is the normal metal density of states and n≥2n \geq 2n≥2 is the least number of impurities in a complex that can localize nodal quasiparticle. This result essentially differs from the known predictions of self-consistent approximation: $\r(0) \propto \r_N \sqrt {c/\r_N\D}$ (for the unitary limit V→∞V \to \inftyV→∞) or $\r(0) \propto (\D/cV^2)\exp(-\D/cV^2\r_N)$ (for the Born limit $|V|\r_N \ll 1$). We predict also existence of a narrow interval (mobility gap) around the Fermi energy, where all the states are localized on proper impurity clusters, leading to exponential suppression of low-temperature kinetics.
The absence of localization of impurity-induced low-energy quasiparticle states in a 2D d-wave superconductor is shown for any amount of disorder in the limit of unitary scatterers. This result follows from the fact that a unitary impurity produces a marginally bound state at zero energy which decays as a power law along the nodes of the d-wave energy gap. Consequently, for finite density of impurities, the impurity-induced states are coupled by long-range overlaps yielding extended quasiparticle states below a characteristic energy scale ${\ensuremath{\omega}}_{c}$. Simple scaling arguments suggest that ${\ensuremath{\omega}}_{c}\ensuremath{\propto}{e}^{{\ensuremath{-}c/n}_{\mathrm{imp}}}$, with nimp{n}_{\mathrm{imp}}nimp​ the impurity density and c a positive constant.
A comparative analysis has been done of the formerly established two self-consistent solutions for the density of quasiparticle states in doped d-wave superconductors, having strikingly different and disputed behavior near the Fermi energy. One of them (1) remains finite in this limit, while the other (2) tends to zero. To resolve this discrepancy, the known Ioffe-Regel criterion for band states, widely used for doped semiconductors, was applied to these solutions. It is shown that both them are valid in limited and different energy regions, where the corresponding quasiparticles are weakly damped. In particular, density of states of nodal quasiparticles near the Fermi level is provided by the (2) solution, while the (1) only applies far enough from this level.
We develop an analytical theory for generic disorder-driven quantum phase transitions. We apply this formalism to the superconductor-insulator transition and we briefly discuss the applications to the order-disorder transition in quantum magnets. The effective spin-12\frac{1}{2}21​ models for these transitions are solved in the cavity approximation which becomes exact on a Bethe lattice with large branching number K⪢1K⪢1K⪢1 and weak dimensionless coupling g⪡1g⪡1g⪡1. The characteristic feature of the low-temperature phase is a large self-formed inhomogeneity of the order-parameter distribution near the critical point $K\ensuremath{\ge}{K}_{c}(g)$, where the critical temperature Tc{T}_{c}Tc​ of the ordering transition vanishes. We find that the local probability distribution P(B)P(B)P(B) of the order parameter BBB has a long power-law tail in the region where BBB is much larger than its typical value B0{B}_{0}B0​. Near the quantum-critical point, at $K\ensuremath{\rightarrow}{K}_{c}(g)$, the typical value of the order parameter vanishes exponentially, ${B}_{0}\ensuremath{\propto}{e}^{\ensuremath{-}C/[K\ensuremath{-}{K}_{c}(g)]}$ while the spatial scale Ninh{N}_{inh}Ninh​ of the order parameter inhomogeneities diverges as ${[K\ensuremath{-}{K}_{c}(g)]}^{\ensuremath{-}2}$. In the disordered regime, realized at K<Kc(g)K<{K}_{c}(g)K<Kc​(g) we find actually two distinct phases characterized by different behavior of relaxation rates. The first phase exists in an intermediate range of ${K}^{\ensuremath{\ast}}(g)<K<{K}_{c}(g)$. It has two regimes of energies: at low excitation energies, $\ensuremath{\omega}<{\ensuremath{\omega}}_{d}(K,g)$, the many-body spectrum of the model is discrete, with zero-level widths, while at $\ensuremath{\omega}>{\ensuremath{\omega}}_{d}$ the level acquire a nonzero width which is self-generated by the many-body interactions. In this phase the spin model provides by itself an intrinsic thermal bath. Another phase is obtained at smaller $K<{K}^{\ensuremath{\ast}}(g)$, where all the eigenstates are discrete, corresponding to full many-body localization. These results provide an explanation for the activated behavior of the resistivity in amorphous materials on the insulating side near the superconductor-insulator transition and a semiquantitative description of the scanning tunneling data on its superconductive side.
Strong evidence is presented for the localization of low-energy quasiparticle states in disordered ddd-wave superconductors. Within the framework of the Bogoliubov-de Gennes (BdG) theory applied to the extended Hubbard model with a finite concentration of nonmagnetic impurities, we carry out a fully self-consistent numerical diagonalization of the BdG equations on finite clusters containing up to 50\ifmmode\times\else\texttimes\fi{}50 sites. Localized states are identified by probing their sensitivity to the boundary conditions and by analyzing the finite-size dependence of inverse participation ratios.
Superconducting materials are useful for a wide range of applications, ranging from particle detectors to quantum computing. The presence of excitations (quasiparticles) in the superconductor can be a resource in some devices and a disturbance in others - in kinetic inductance detectors, the generation of quasiparticles by an incoming photon can be read out and used to calculate the energy of the photon, while the tunnelling of quasiparticles is a cause of decoherence in quantum computing. While early research mostly focused on superconductors close to the critical temperature, temperatures that are far below the critical temperatures are often used for current applications. At these low temperatures, the energy exchange between quasiparticles and phonons becomes slow, and even small disturbances may drive the energy distribution of the quasiparticles out of thermal equilibrium. In fact, experiments usually show a residual number of quasiparticles even at milikelvin temperatures, for which the thermal density of quasiparticles would be negligible. This thesis consists of two parts: In the first part, I model the energy distribution of quasiparticles in superconducting resonators: Quasiparticles absorb energy by absorbing photons and release it as phonons, which drives the superconductor out of thermal equilibrium. I solve a set of rate equations, both numerical and analytical, to calculate the energy distribution of the quasiparticles. For parameters typically used in kinetic inductance detectors made of aluminum, the microwave signal used to read out the resonator dominates the energy distribution of the quasiparticles, while their density is determined by other processes. At not too low temperatures, quasiparticles are mainly produced by thermal phonons, and my calculations reproduce recently measured quality factors of resonators at temperatures above 250 mK without free parameters. I show that even a very small number of photons of higher energy, which I ascribe to noise from the microwave generator, would dominate the quasiparticle density at lower temperatures. Under this assumption, my calculations also reproduce the quality factors at lower temperatures. In the second part of this thesis, I investigate the effects of spatial fluctuations of the superconducting energy gap on the dynamics of quasiparticles. Recently, it has been proposed that such fluctuations may lead to the localization of quasiparticles in states below the energy gap, which could cause a finite quasiparticle density even at very low temperatures. Using the Keldysh-Usadel formalism, I derive rates for the different processes (recombination/(de-) localization/generation) of quasiparticles in such systems. Using these rate equations I derive new upper limits for the quasiparticle density that could result from these localized states. These upper limits show that localization caused by weak magnetic impurities in typical aluminum systems does not lead to a relevant quasiparticle density. This contradicts previous theories, which only consider the recombination between two localized quasiparticles without examining their dynamics in detail.