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arXiv:1006.5767 · Physical Review B

Superconductor-insulator transition and energy localization

M. V. Feigel’man, L. B. Ioffe, Marc Mézard

Published Nov 29, 2010• 100 citations
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Abstract

We develop an analytical theory for generic disorder-driven quantum phase transitions. We apply this formalism to the superconductor-insulator transition and we briefly discuss the applications to the order-disorder transition in quantum magnets. The effective spin-$\frac{1}{2}$ models for these transitions are solved in the cavity approximation which becomes exact on a Bethe lattice with large branching number $K⪢1$ and weak dimensionless coupling $g⪡1$. The characteristic feature of the low-temperature phase is a large self-formed inhomogeneity of the order-parameter distribution near the critical point $K\ensuremath{\ge}{K}_{c}(g)$, where the critical temperature ${T}_{c}$ of the ordering transition vanishes. We find that the local probability distribution $P(B)$ of the order parameter $B$ has a long power-law tail in the region where $B$ is much larger than its typical value ${B}_{0}$. Near the quantum-critical point, at $K\ensuremath{\rightarrow}{K}_{c}(g)$, the typical value of the order parameter vanishes exponentially, ${B}_{0}\ensuremath{\propto}{e}^{\ensuremath{-}C/[K\ensuremath{-}{K}_{c}(g)]}$ while the spatial scale ${N}_{inh}$ of the order parameter inhomogeneities diverges as ${[K\ensuremath{-}{K}_{c}(g)]}^{\ensuremath{-}2}$. In the disordered regime, realized at $K<{K}_{c}(g)$ we find actually two distinct phases characterized by different behavior of relaxation rates. The first phase exists in an intermediate range of ${K}^{\ensuremath{\ast}}(g)<K<{K}_{c}(g)$. It has two regimes of energies: at low excitation energies, $\ensuremath{\omega}<{\ensuremath{\omega}}_{d}(K,g)$, the many-body spectrum of the model is discrete, with zero-level widths, while at $\ensuremath{\omega}>{\ensuremath{\omega}}_{d}$ the level acquire a nonzero width which is self-generated by the many-body interactions. In this phase the spin model provides by itself an intrinsic thermal bath. Another phase is obtained at smaller $K<{K}^{\ensuremath{\ast}}(g)$, where all the eigenstates are discrete, corresponding to full many-body localization. These results provide an explanation for the activated behavior of the resistivity in amorphous materials on the insulating side near the superconductor-insulator transition and a semiquantitative description of the scanning tunneling data on its superconductive side.

DOI
10.1103/physrevb.82.184534

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We numerically study the superconductor-insulator phase transition in a model disordered two-dimensional (2D) superconductor as a function of applied magnetic field. The calculation involves quantum Monte Carlo calculations of the (2+1)D(2+1)\text{D}(2+1)D XYXYXY model in the presence of both disorder and magnetic field. The XYXYXY coupling is assumed to have the form $\ensuremath{-}J\text{ }\text{cos}({\ensuremath{\theta}}_{i}\ensuremath{-}{\ensuremath{\theta}}_{j}\ensuremath{-}{A}_{ij})$, where Aij{A}_{ij}Aij​ has a mean of zero and a standard deviation $\ensuremath{\Delta}{A}_{ij}$. In a real system, such a model would be approximately realized by a 2D array of small Josephson-coupled grains with slight spatial disorder and a uniform applied magnetic field. The different values $\ensuremath{\Delta}{A}_{ij}$ then correspond to an applied field such that the average number of flux quanta per plaquette has various integer values NNN: larger NNN corresponds to larger $\ensuremath{\Delta}{A}_{ij}$. For any value of $\ensuremath{\Delta}{A}_{ij}$, there appears to be a critical coupling constant ${K}_{c}(\ensuremath{\Delta}{A}_{ij})=\sqrt{{[J/(2U)]}_{c}}$, where UUU is the charging energy, below which the system is a Mott insulator; there is also a corresponding critical conductivity ${\ensuremath{\sigma}}^{\ensuremath{\ast}}(\ensuremath{\Delta}{A}_{ij})$ at the transition. For $\ensuremath{\Delta}{A}_{ij}=\ensuremath{\infty}$, the order parameter of the transition is a renormalized coupling constant ggg. Using a numerical technique appropriate for disordered systems, we show that the transition at this value of $\ensuremath{\Delta}{A}_{ij}$ takes place from an insulating (I) phase to a Bose glass (BG) phase, and that the dynamical critical exponent characterizing this transition is $z\ensuremath{\sim}1.3$. By contrast, z=1z=1z=1 for this model at $\ensuremath{\Delta}{A}_{ij}=0$. We suggest that the superconductor-to-insulator transition is actually of this I to BG class at all nonzero $\ensuremath{\Delta}{A}_{ij}$'s, and we support this interpretation by both numerical evidence and an analytical argument based on the Harris criterion [A. B. Harris, J. Phys. C 7, 1671 (1974)]. Kc{K}_{c}Kc​ is found to be a monotonically increasing function of $\ensuremath{\Delta}{A}_{ij}$. For certain values of KKK, a disordered Josephson array may undergo a transition from an ordered, Bose glass phase to an insulator with increasing $\ensuremath{\Delta}{A}_{ij}$.
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We develop an analytical theory, based on the quantum cavity method, describing the quantum phase transitions in low-temperature, strongly disordered ferromagnets and superconductors. At variance with the usual quantum critical points, we find a phase diagram with two critical points separating three phases. When the disorder increases, the systems goes from the ordered phase to an intermediate disordered phase characterized by activated transport and then to a second disordered phase where no transport is possible. Both the ordered and disordered phases exhibit strong inhomogeneity of their basic properties typical of glassy physics.
Bosonic excitations within long-range ordered, but strongly inhomogeneous phases have been studied in quite some detail. My thesis focuses instead on understanding the insulating, localized phase of disordered bosonic systems. In particular I study localization properties of strongly interacting bosons and spin systems in a disorder potential at zero temperature. I focus on simple, prototypical spin models (Ising model and XY model) in random fields on a Cayley tree with large connectivity. Regarding the nature of the quantum phase transition in strong disorder I find the following results: i) With a uniformly distributed disorder non-extensive excitations in the disordered phase are all localized. ii)Moreover, I find that the order arises due to a collective condensation, which is qualitatively distinct from a Bose Einstein condensation of single particle excitations into a delocalized state. In particular, in non-frustrated Bose glasses, I do not find evidence for a boson mobility edge in the Bose glass. These results are qualitatively different from claims in the recent literatures . Considering that (many body) localization of bosons is a kind of quantum glass transition, it is an interesting question to ask what phenomena occur, if the ingredients for more conventional (classical) glassy physics are added to a disordered bosons system, namely: random, frustrated interactions between the bosons. One can still think about such a system as bosons in a disordered potential, where the disordered potential is, at least partly, self-generated by random frustrated interactions between the bosons. This question takes us to the study of another type of disordered systems: glassy systems. Those are typically characterized by low temperature phases with an inhomogeneous density or magnetization pattern, which is extremely long-lived due to the occurrence of non-trivial ergodicity breaking. I study a solvable model of hard core bosons (pseudospins) subject to disorder and frustrating interactions. This solvable model provides insight into the possibility of coexistence of super uidity and glassy density order, as well as into the nature of the coexistence phase (the superglass). In particular, for the considered mean field model I prove the existence of a superglass phase. This complements the numerical evidence for such phases provided by quantum Monte Carlo investigations in finite dimensions and on random graphs. Those were, however, limited to finite temperature, and could thus not fully elucidate the structure of the phases at T = 0. In contrast, my analytical approach allows one to understand the quantum phase transition between glassy superfluid and insulator, and the non-trivial role played by glassy correlations. When the frustrated interactions are strong enough, the superfluid order may be destroyed. As I will show in a mean field model, this happens within the glass phase of the system, where a disorder induced superfluid-insulator phase transition takes place to give way to a frustrated Bose glass. The glassy background on top of which this happens leads to many interesting phenomena which seem not to have been noticed before. To understand the nature of the glassy superfluid-insulator quantum phase transition at zero temperature and the transport properties on the insulating, Bose glass side of the transition is the goal of the third part of my thesis. To address the above questions, I studied an exactly solvable model of a glassy superfluid-insulator quantum phase transition on a Bethe lattice geometry with high connectivity. My main results can be summarized as follows: i) I found that the superfluid-insulator transition is shifted to stronger hopping. This is a result of the pseudo gap in the density of states of the glass state, which tends to strongly disfavor the onset of superfluidity. ii) In the glassy insulator, the discrete local energy levels become broadened due to the quantum fluctuations.The level-broadening process appears as a phase transition which has strong similarities with an Anderson localization transition, and has implications on many body localization. By using the locator expansion for bosons I found that, the glassy insulator has a finite mobility edge for the bosonic excitations, which, however, does not close upon approaching the SI quantum phase transition point. This finding helps to understand the nature of the superfluid-to-frustrated Bose glass transition: the superfluid emerges as a collective phase ordering phenomenon at zero temperature, and not as a condensation in to a single particle delocalized state, in contrast to opposite predictions in the recent literatures. The existence of a mobility edge in the insulator suggests the possibility of phononless, activated transport in the bosonic insulator, which might be a candidate explanation for the experimentally seen activated transport, which has remained a mystery for a long time.
Zero-temperature or quantum phase transitions in itinerant electronic systems both with and without quenched disordered are discussed. Phase transitions considered include, the ferromagnetic transition, the antiferromagnetic transition, the superconductor-metal transition, and various metal-insulator transitions. Emphasis is placed on how to determine the universal properties that characterize these quantum phase transitions. For the first three of the phase transitions listed above, one of the main physical ideas established is that in zero-temperature systems there are soft or slow modes that exist in addition to the soft order parameter fluctuations, and that these modes can couple to the critical modes. These extra soft modes are shown to have a profound effect on the quantum critical properties. For quantum phase transitions involving zero wavenumber order parameters, i.e., the ferromagnetic and superconductor-metal transitions, these extra modes effectively lead to long-ranged effective interactions between order parameter fluctuations, which in turn lead to exactly soluble critical behaviors. For the antiferromagnetic case, we argue that while in low enough dimensions disorder fluctuation effects tend to destroy long-range order, quantum fluctuations counteract this effect and in some parameter regions manage to re-establish antiferromagnetic long-range order. For the metal-insulator transition, some recent new ideas are reviewed. In particular, it is pointed out that for interacting disordered electrons, one expects that in high dimensions the metal-insulator transition is related to the phase transition that occurs in random-field magnets in high dimensions. If the analogy also holds in three dimensions this suggests that the metal-insulator transition might have glassy characteristics.
It is well known that the metal-insulator transition in two dimensions for non-interacting fermions takes place at infinitesimal disorder. In contrast, the superconductor-to-insulator transition takes place at a finite critical disorder (on the order of Vc ~ 2t), where V is the typical width of the distribution of random site energies and t is the hopping scale. In this article we compare the localization/delocalization properties of one and two particles. Whereas the metal-insulator transition is a consequence of single-particle Anderson localization, the superconductor-insulator transition (SIT) is due to pair localization – or, alternatively, fluctuations of the phase conjugate to pair density. The central question we address is how superconductivity emerges from localized single-particle states. We address this question using inhomogeneous mean field theory and quantum Monte Carlo techniques and make several testable predictions for local spectroscopic probes across the SIT. We show that with increasing disorder, the system forms superconducting blobs on the scale of the coherence length embedded in an insulating matrix. In the superconducting state, the phases on the different blobs are coherent across the system whereas in the insulator long-range phase coherence is disrupted by quantum fluctuations. As a consequence of this emergent granularity, we show that the single-particle energy gap in the density of states survives across the transition, but coherence peaks exist only in the superconductor. A characteristic pseudogap persists above the critical disorder and critical temperature, in contrast to conventional theories. Surprisingly, the insulator has a two-particle gap scale that vanishes at the SIT despite a robust single-particle gap.