Quantum simulation: no satisfaction A network is termed 'frustrated' when competing interactions between nodes prevent each bond from being satisfied. Frustration in quantum networks can lead to massively entangled ground states. The authors study this process by performing a quantum simulation of a frustrated spin system using three trapped atomic ions, whose interactions are precisely controlled using optical forces.
Quantum simulation: no satisfaction A network is termed 'frustrated' when competing interactions between nodes prevent each bond from being satisfied. Frustration in quantum networks can lead to massively entangled ground states. The authors study this process by performing a quantum simulation of a frustrated spin system using three trapped atomic ions, whose interactions are precisely controlled using optical forces.
A collection of trapped atomic ions represents one of the most attractive platforms for the quantum simulation of interacting spin networks and quantum magnetism. Spin-dependent optical dipole forces applied to an ion crystal create long-range eective spin-spin interactions and allow the simulation of spin Hamiltonians that possess nontrivial phases and dynamics. We trap linear chains of 171Yb+ ions in a Paul trap, and constrain the occupation of energy levels to the ground hyperne clock-states, creating a qubit or pseudo-spin 1/2 system. We proceed to implement spin-spin couplings between two ions using the far detuned Mlmer-Srenson scheme and perform adiabatic quantum simulations of Ising Hamiltonians with long-range couplings. We then demonstrate our ability to control the sign and relative strength of the interaction between three ions. Using this control, we simulate a frustrated triangular lattice, and for the first time establish an experimental connection between frustration and quantum entanglement. We then scale up our simulation to show phase transitions from paramagnetism to ferromagnetism for nine ions, and to anti-ferromagnetism for sixteen ions. The experimental work culminates with our most complicated Hamiltonian - a long range anti-ferromagnetic Ising interaction between 10 ions with a biasing axial field. Theoretical work presented in this thesis shows how the approach to quantum simulation utilized in this thesis can be further extended and improved. It is shown how appropriate design of laser elds can provide for arbitrary multidimensional spin-spin interaction graphs even for the case of a linear spatial array of ions. This scheme uses currently existing trap technology and is scalable to levels where classical methods of simulation are intractable.
Frustration, or the competition between interacting components of a network, is often responsible for the emergent complexity of many-body systems. For instance, frustrated magnetism is a hallmark of poorly understood systems such as quantum spin liquids, spin glasses, and spin ices, whose ground states can be massively degenerate and carry high degrees of quantum entanglement. Here, we engineer frustrated antiferromagnetic interactions between spins stored in a crystal of up to 16 trapped (171)Yb(+) atoms. We control the amount of frustration by continuously tuning the range of interaction and directly measure spin correlation functions and their coherent dynamics. This prototypical quantum simulation points the way toward a new probe of frustrated quantum magnetism and perhaps the design of new quantum materials.
The quantum simulation of complex many body systems holds promise for understanding the origin of emergent properties of strongly correlated systems, such as high-Tc superconductors and spin liquids. Cold atomic systems provide an almost ideal platform for quantum simulation due to their excellent quantum coherence, initialization and readout properties, and their ability to support several forms of interactions. In this thesis, I present experiments on the quantum simulation of long range Ising models in the presence of transverse magnetic fields with a chain of up to sixteen ultracold 171-Yb+ ions trapped in a linear radio frequency Paul trap. Two hyperfine levels in each of the 171-Yb+ ions serve as the spin-1/2 systems. We detect the spin states of the individual ions by observing state-dependent fluorescence with single site resolution, and can directly measure any possible spin correlation function. The spin-spin interactions are engineered by applying dipole forces from precisely tuned lasers whose beatnotes induce stimulated Raman transitions that couple virtually to collective phonon modes of the ion motion. The Ising couplings are controlled, both in sign and strength with respect to the effective transverse field, and adiabatically manipulated to study various aspects of this spin model, such as the emergence of a quantum phase transition in the ground state and spin frustration due to competing antiferromagnetic interactions. Spin frustration often gives rise to a massive degeneracy in the ground state, which can lead to entanglement in the spin system. We detect and characterize this frustration induced entanglement in a system of three spins, demonstrating the first direct experimental connection between frustration and entanglement. With larger numbers of spins we also vary the range of the antiferromagnetic couplings through appropriate laser tunings and observe that longer range interactions reduce the excitation energy and thereby frustrate the ground state order. This system can potentially be scaled up to study a wide range of fully connected spin networks with a few dozens of spins, where the underlying theory becomes intractable on a classical computer.
Quantum simulation of interacting many-body spin systems is routinely performed with cold trapped ions, and systems with hundreds of spins have been studied in one and two dimensions. In the most common realizations of these platforms, spin degrees of freedom are encoded in low-lying electronic levels, and interactions among the spins are mediated through crystal vibrations. Here we propose a new approach which enables the quantum simulation of two-dimensional spin systems with interaction strengths that are increased by orders of magnitude. This, together with the unprecedented longevity of trapped ions, opens an avenue for the exploration of phenomena that take place on long timescales, e.g., slow and collective relaxation in frustrated and kinetically constrained systems. Our platform makes use of the strong dipolar interactions among electronic Rydberg states and planar confinement provided by a Penning trap. We investigate how the strong electric and magnetic fields that form this trap affect the properties of the Rydberg states and show that spin-spin interaction strengths on the order of MHz are achievable under experimentally realistic conditions. As a brief illustration of the capabilities of this quantum simulator, we study the entanglement in a frustrated spin system realized by three ions.
In a proof-of-principle experiment, we simulate the dynamics of a quantum spin system in an ion trap. Following a theoretical proposal by D. Porras and I. Cirac, we use a system of ground state cooled trapped ions to simulate and study the dynamics of a quantum-mechanical system, or more precisely, the dynamics of a quantum spin Hamiltonian. We implement the smallest non-trivial quantum spin Hamiltonian, the quantum Ising model for two spins. Each spin is represented by two hyperfine ground levels of trapped 25Mg+ ions. The interaction with an external magnetic field is simulated by coherently coupling these hyperfine levels via laser and radiofrequency radiation. The spin-spin interaction is simulated via optical dipole forces, where the effective interaction is mediated by the phonons of the linear ion chain. We demonstrate the adiabatic evolution from a paramagnetically ordered system to ferromagnetic order. The final state of this adiabatic transition is a superposition state of the two degenerate spin configurations of ferromagnetic order Psi_final = 1/sqrt(2) (|up up> + |down down>) with a quantum magnetisation of 98%. We also show the transition from paramagnetic to antiferromagnetic order with the final state Psi_final = 1/sqrt(2) (|up down> + |down up>). Moreover, we prove that this transition which is to become a quantum phase transition in the thermodynamic limit of infinitely many spins, is driven by quantum fluctuations which dominate the dynamics of such systems at the absolute zero-point of temperature rather than thermal fluctuations which are absent at 0 K. This is verified by the fact that the final state of our adiabatic evolution is entangled, close to a Bell state at a fidelity exceeding 88%. The set of tools presented in this thesis might serve as a basis for larger scale quantum simulations which might help in gaining insight into many-particle effects that are intractable on classical computers such as spin frustration in triangular lattices or high-Tc superconductivity.
Quantum simulators are capable of calculating properties of quantum systems unfeasible for classical computers. Here we report the analog quantum simulation of arbitrary Heisenberg-type interactions among four spin-1/2 particles. This spin-1/2 tetramer is the two-dimensional archetype system whose ground state belongs to the class of valence-bond states. Depending on the interaction strength, frustration within the system emerges such that the ground state evolves from a localized to a resonating valence-bond state. This spin-1/2 tetramer is created using the polarization states of four photons. We utilize the particular advantages of the precise single-particle addressability and a tunable measurement-induced interaction to obtain fundamental insights into entanglement dynamics among individual particles. We also directly extract ground-state energies and pair-wise quantum correlations, which enable our quantum simulator to investigate the frustration of entanglement. Remarkably, the pair-wise correlations are restricted by quantum monogamy.