Quantum entanglement exhibits various interesting features that emerge only in high-dimensional systems. One of the most fascinating is bound entanglement, entanglement that cannot be extracted using local operations and classical communication. This thesis describes our work towards an experimental realization of the four-qubit bound-entangled Smolin state, using the polarization and spatial mode of photon pairs. We describe a number of interesting experimental challenges that this work faced. We present our results on entangled two-qubit spatial mode states and hyperentangled four-qubit polarization-spatial-mode states generated by spontaneous parametric down-conversion from a second-order TEM mode pump. Some of the subtleties involved in preparing genuine mixed states in the lab are discussed.
Quantum entanglement exhibits various interesting features that emerge only in high-dimensional systems. One of the most fascinating is bound entanglement, entanglement that cannot be extracted using local operations and classical communication. This thesis describes our work towards an experimental realization of the four-qubit bound-entangled Smolin state, using the polarization and spatial mode of photon pairs. We describe a number of interesting experimental challenges that this work faced. We present our results on entangled two-qubit spatial mode states and hyperentangled four-qubit polarization-spatial-mode states generated by spontaneous parametric down-conversion from a second-order TEM mode pump. Some of the subtleties involved in preparing genuine mixed states in the lab are discussed.
Multi-particle entangled states are becoming more and more interesting for different applications in quantum information, such as quantum multi-particle teleportation, entangled based cryptography and quantum communication schemes based on multi-particle states, but also for fundamental reasons such as testing local realism by means of the Greenberger-Horne-Zeilinger states (GHZ) arguments . The advantage of multiparticle entanglement versus the most common two particle one lies in the fact that the greater the number of particles involved in the entangled state, the more clearly the quantum effects are exhibited. Our final goal is to exploit the multi-photon entangled states for quantum metrology. By the interaction of those states with nanostructures (mostly nanoholes, but in a future also nanospheres), we expect to reach sub-wavelength sensitivity phase measurements beating the Standard Quantum Limit as well as to detect plasmonic effects. In this thesis we present our work consisting on designing and building an experimental setup for the generation of states of 4-photon entangled in the transverse linear momentum. In the first part we explain some basics in the form of a technical introduction. We then adapt a general theoretical model to our particular case, explaining the physics of the process of generation of entangled states of photons. We proceed explaining the details of our setup, as well as the procedure of measurement. We then present the results of our tests in a "standard" 2-photon regime to show the correct functioning of the setup itself. Some more sophisticated measurements using structured light in the form of a first-order Hermite-Gaussian mode has been performed to generate entanglement in higher spatial modes are also presented. We conclude with theoretical and experimental details regarding the 4-photon experiments feasible with our setup. Our source is based on Spontaneous Parametric Down-Conversion (SPDC). In the last two decades it has been extensively studied for the generation of two-photon entangled states, since Kwiat et al. published in 1995 the new scheme based on polarization entangled photons. Most of the studies regarding entangled states involving more than two photons are indeed based on quantum correlations in the polarization or in the path of the down converted beams. The great advantage of entangling a spatial degree of freedom (as we do) is related to the dimensionality of the Hilbert space in which the state is defined. In the particular case of linear momentum, which is a continuous variable, we are dealing with infinite dimensions. Since in each dimension of the state one quanta of information can be encoded, the advantage of having multidimension entanglement for the field of quantum communication and computing is clear. The specs of our setup include a periodically-poled KTP crystals offering high conversion efficiency and cut for type-0 SPDC. The photons generated are well known to be inherently entangled in different degrees of freedom such as polarization, energy-time, linear momentum, and orbital angular momentum. Since each single SPDC event generates one photon pair, in order to reach four photon we entangle two consecutive SPDC events per each state. Furthermore, it is possible to manipulate (to enhance) the dimensionality of the entanglement by properly tailoring the pump spatial profile. The key point for the generation of four-photon entangled states is that, under some conditions, two consecutive pairs generated via SPDC cannot be described as two independent pairs but necessarily as a four-photon state showing genuine entanglement. This can happen when using a pulsed laser to generate the entangled photons; in particular, in the regime in which the coherence time of the down-converted photons τc is (much) longer than the temporal length of the pumping pulse Δt. In this condition the emission of a second pair is stimulated by the presence of the first one. That effect can be ultimately seen as a constructive multi-particle interference effect, the deep origin of which has to be sought in the boson statistic of photons.
Entanglement in high-dimensional quantum systems, where one or more degrees of freedom of light are involved, offers increased information capacities and enables new quantum protocols.Here, we demonstrate a functional source of high-dimensional, noise-resilient hyperentangled states encoded in time-frequency and vector vortex structured modes, which in turn carry single-particle entanglement between polarization and orbital angular momentum.Pairing nonlinearity-engineered parametric downconversion in an interferometric scheme with spin-to-orbital-angular-momentum conversion, we generate highly entangled photon pairs at telecom wavelength that we characterize via two-photon interference and quantum state tomography, achieving near-unity visibilities and fidelities.While hyperentanglement has been demonstrated before in photonic qubits, here we present a rich entanglement structure involving spectrally and spatially structured light, where three different forms of entanglement coexist in the same biphoton state.
Quantum states of photons such as entangled and single photons are indispensable components for applications in optical quantum information processing. Being able to generate and manipulate quantum states of photons on a chip is a crucial step towards realizing real-world quantum information processing systems such as an optical quantum computer. In this thesis, theoretical and experimental research was carried out for on-chip generation of quantum states of photons via the nonlinear process of spontaneous parametric down-conversion (SPDC), including polarization entangled photons, hyperentangled photons and heralded pure single photons. A majority of the study was based on III-V semiconductor AlGaAs, which could lead to monolithic integration of pump lasers and enable electrically pump sources operating at room temperature. The generation of cross-polarized entangled photons via a type-II SPDC in an AlGaAs Bragg reflection waveguide (BRW) was first investigated. The lack of material birefringence enables the direct generation of wavelength-multiplexed polarization entangled photons with a concurrence of at least 0.77 in a bandwidth of 95 nm. Second, a technique using concurrent type-0 and type-I processes on an AlGaAs chip to generate polarization entangled photon was developed. This technique allows the generation of both co-polarized and cross-polarized entangled photons on the same chip without the need of off-chip compensation, interferometer and bandpass filter. Third, a technique of generating hyperentangled photons on an AlGaAs chip was developed by utilizing spatial modes of different guiding mechanisms. High quality entanglement could be achieved with bandpass filtering of a few nanometers without off-chip phase compensation. Four, a generic technique using nonlinear photonic nanowires to engineer two-photon quantum states was proposed. Via dispersion engineering which controls the group velocity of each mode, maximally entangled polarization entangled photons and pure heralded single photons can be generated on-chip. Design examples were applied to III-V semiconductor and ferroelectric materials. Last, a strategy to enhance the bandwidths of wavelength conversion and SPDC spectrum was developed by tapering the waveguides. Combined with further integration of pump lasers, photonic circuits and detectors, the techniques developed in this thesis provides a viable route to achieve fully integrated generation and manipulations of photonic quantum qubits.
Nowadays,the generation of multiphoton entangled states is almost realized by combining the coupled entangled photons emitted from spontaneous parametric down-conversion (SPDC) with the first-order term.In this case,one may focus mainly on the first-order term,and then avoid multipair emission events by restricting experimental parameters.On the other hand,for the higher-order terms in SPDC source,these emitted entangled photons have interesting features.For example,they are entangled maximally not only in photon number for the spatial modes,but also in polarization degree of freedom.In general,two photons,which are entangled in two or more degrees of freedom,are called hyperentangled pair of photons or hyperentangled state.We present a scheme to generate the four-photon hyperentangled state based on four indistinguishable photons emitted from SPDC source with the second-order term.Consider two SPDC sources with equal probability of emission of photons in respective spatial modes.With the passive linear optical devices,i.e., beam splitters,half wave plates,polarizing beam splitters,etc.,under the condition of registering a specified four-photon coincidence,we can obtain the four-photon hyperentangled state in which the photons are entangled in both polarization and spatial-mode degrees of freedom.Here,of course,for an arbitrary fourfold coincidence detection,one obtains a canonical four-photon Greenberger-Horne-Zeilinger (GHZ) state.Then we show the results of fourfold coincidence detections and the corresponding probabilities for the four-photon GHZ states,where the generation of the four-photon hyperentangled state is included as long as we are not to distinguish the two detectors located at the same locations. As a result,our scheme has two notable features.When we only consider the second-order emission,since it is not needed for us to distinguish between the two SPDC sources,the present scheme is simple and feasible.Also,based on the postselection with fourfold coincidence detection,our scheme is suitable for the normal first-order emission where we restrict the four photons emitted from the same source.In this sense,our scheme is efficient.In a word,we describe a method to generate the four-photon hyperentangled state with the second-order emission in SPDC source,which may contribute to the exploration of multipair entanglement with higher-order emissions from the SPDC source.
Multiphoton hyperentangement is fundamental in optical quantum information processing. Existing theory and experiments usually focus on producing two-photon hyperentanglement and multiphoton entangled states encoded in a single degree of freedom. Multiphoton entangled states have until now relied on the outcome postselection, a procedure where only the measurement results corresponding to the desired state are considered. Such an approach severely limits the usefulness of the resulting entangled states. We present the protocols of direct production of three- and four-photon hyperentanglement and extend the approach to an arbitrary number of photons through a straightforward cascade of spontaneous parametric down-conversion (SPDC) sources. The generated multiphoton hyperentangled states are encoded in polarization-spatial modes and polarization-time bin degrees of freedom, respectively. Numerical calculation shows that if the average photon number $\ensuremath{\mu}$ is 1, the down-conversion efficiency is $7.6\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}6}$ and the repetition frequency of the laser is 109 Hz, the number of the generation of three-photon and four-photon hyperentanglement after cascading can reach about $5.78\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}2}$ and $4.44\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}7}$ pairs per second, respectively. By eliminating the constraints of outcome postselection, our protocols may represent progresses for multiphoton hyperentangement generation and provide a pivotal role in future multiparty and high-capacity communication networks.