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Scientific Reports

Multi-copy quantifiers for single-photon states

Petr Zapletal, Radim Filip

Published Apr 27, 2017• 9 citations
Publisher

Abstract

Single-photon states are basic resources for hybrid quantum technology with non-Gaussian states of light. Accelerating quantum technology is already able to produce high-quality single-photon states. These states can be used for hybrid quantum information processing, based on a nonclassical phase-space interference represented by negativity of a Wigner function. Therefore, new quantifiers, capable of evaluating such high-quality single-photon states, are required. We propose and analyze quantifiers which process multiple estimates of single-photon state's statistics. The quantifiers simulate basic capability of single photons to conditionally bunch into a single mode and form a Fock state. This state exhibits complex nonclassical phase-space interference effects making its Wigner function negative in multiple areas. The quantifiers directly evaluate a presence of the multiple negativities corresponding to the Fock state. We verify applicability of the quantifiers by using them to single-photon states from recent experiments. The quantifiers can be further extended to also test indistinguishability of single-photon states. It allows to verify quantum interference of light from single-photon emitters more sensitively than in the traditional Hong-Ou-Mandel test. Besides quantum optics, the multi-copy quantifiers can be also applied to experiments with atomic memories and mechanical oscillators.

DOI
10.1038/s41598-017-01333-y

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Single-photon states are basic resources for hybrid quantum technology with non-Gaussian states of light. Accelerating quantum technology is already able to produce high-quality single-photon states. These states can be used for hybrid quantum information processing, based on a nonclassical phase-space interference represented by negativity of a Wigner function. Therefore, new quantifiers, capable of evaluating such high-quality single-photon states, are required. We propose and analyze quantifiers which process multiple estimates of single-photon state's statistics. The quantifiers simulate basic capability of single photons to conditionally bunch into a single mode and form a Fock state. This state exhibits complex nonclassical phase-space interference effects making its Wigner function negative in multiple areas. The quantifiers directly evaluate a presence of the multiple negativities corresponding to the Fock state. We verify applicability of the quantifiers by using them to single-photon states from recent experiments. The quantifiers can be further extended to also test indistinguishability of single-photon states. It allows to verify quantum interference of light from single-photon emitters more sensitively than in the traditional Hong-Ou-Mandel test. Besides quantum optics, the multi-copy quantifiers can be also applied to experiments with atomic memories and mechanical oscillators.
Advanced quantum technologies, as well as fundamental tests of quantum physics, crucially require the interference of multiple single photons in linear-optics circuits. This interference can result in the bunching of photons into higher Fock states, leading to a complex bosonic behavior. These challenging tasks timely require to develop collective criteria to benchmark many independent initial resources. Here we determine whether n independent imperfect single photons can ultimately bunch into the Fock state | n ⟩ . We thereby introduce an experimental Fock-state bunching capability for single-photon sources, which uses phase-space interference for extreme bunching events as a quantifier. In contrast to autocorrelation functions, this operational approach takes into account not only residual multi-photon components but also a vacuum admixture and the dispersion of individual photon statistics. We apply this approach to high-purity single photons generated from an optical parametric oscillator and show that they can lead to a Fock-state capability of at least 14. Our work demonstrates a novel collective benchmark for single-photon sources and their use in subsequent stringent applications.
Advanced quantum technologies, as well as fundamental tests of quantum physics, crucially require the interference of multiple single photons in linear-optics circuits. This interference can result in the bunching of photons into higher Fock states, leading to a complex bosonic behaviour. These challenging tasks timely require to develop collective criteria to benchmark many independent initial resources. Here we determine whether n independent imperfect single photons can ultimately bunch into the Fock state ∣n⟩|n\rangle∣n⟩. We thereby introduce an experimental Fock-state capability for single-photon sources, which uses phase-space interference for extreme bunching events as a quantifier. In contrast to autocorrelation functions, this operational approach takes into account not only residual multi-photon components but also vacuum admixture and the dispersion of the individual photon statistics. We apply this approach to high-purity single photons generated from an optical parametric oscillator and show that they can lead to a Fock-state capability of at least 14. Our work demonstrates a novel collective benchmark for single-photon sources and their use in subsequent stringent applications.
Highly nonclassical character of optical quantum detectors, such as single-photon detectors, is essential for preparation of quantum states of light and a vast majority of applications in quantum metrology and quantum information processing. Therefore, it is both fundamentally interesting and practically relevant to investigate the nonclassical features of optical quantum measurements. Here we propose and experimentally demonstrate a procedure for direct certification of quantum non-Gaussianity and Wigner function negativity, two crucial nonclassicality levels, of photonic quantum detectors. Remarkably, we characterize the highly nonclassical properties of the detector by probing it with only two classical thermal states and a vacuum state. We experimentally demonstrate the quantum non-Gaussianity of a single-photon avalanche diode even under the presence of background noise, and we also certify the negativity of the Wigner function of this detector. Our results open the way for direct benchmarking of photonic quantum detectors with a few measurements on classical states.
This thesis explores the interference of nonclassical states of light, particularly Fock and Gaussian states, in noisy linear interferometers, with applications to quantum information and quantum sensing. Using the phase-space formalism, analytical tools based on generating functions are developed to describe quantum optical interference in a unified way. For multiphoton Fock states, new zero probability events (suppression laws) are identified beyond the previously derived symmetry permutation principle, revealing rich interference structures that is degraded with photon distinguishability. For Gaussian states, the Hafnian-based description of Gaussian Boson Sampling is extended to include partial distinguishability via the overlap matrix of the internal state of the photons. Finally, the link between these interference effects and quantum multiparameter estimation is examined for the simultaneous estimation of phase and loss. This study shows that while probe incompatibility can vanish for optimized non-Gaussian states and some two-mode Gaussian states, at high photon number, measurement incompatibility remains a fundamental constraint even in this limit.
We experimentally demonstrate storage and on-demand release of phase-sensitive, photon-number superposition states of the form α|0⟩+βe^{iθ}|1⟩ for an optical quantized oscillator mode. For this purpose, we newly developed a phase-probing mechanism compatible with a storage system composed of two concatenated optical cavities, which was previously employed for storage of phase-insensitive single-photon states [Phys. Rev. X 3, 041028 (2013)PRXHAE2160-330810.1103/PhysRevX.3.041028]. This is the first demonstration of all-optically storing highly nonclassical and phase-sensitive quantum states of light. The strong nonclassicality of the states after storage becomes manifest as a negative region in the corresponding Wigner function shifted away from the origin in phase space. This negativity is otherwise, without the phase information of the memory system, unobtainable. While our scheme includes the possibility of optical storage, on-demand release and synchronization of arbitrary single-rail qubit states, it is not limited to such states. In fact, our technique is extendible to more general phase-sensitive states such as multiphoton superposition or entangled states, and thus it represents a significant step toward advanced optical quantum information processing, where highly nonclassical states are utilized as resources.
This review covers recent theoretical and experimental efforts to extend the application of the continuous-variable quantum technology of light beyond "Gaussian" quantum states, such as coherent and squeezed states, into the domain of "non-Gaussian" states with negative Wigner functions. Starting with basic Gaussian nonclassicality associated with single- and two-mode vacuum states produced by means of parametric down-conversion and applying a set of standard tools, such as linear interferometry, coherent state injection, and conditional homodyne and photon number measurements, one can implement a large variety of optical states and processes that are relevant in fundamental quantum physics as well as quantum optical information processing. We present a systematic review of these methods, paying attention to both fundamental and practical aspects of their implementation, as well as a comprehensive overview of the results achieved therewith.