Advanced quantum technologies, as well as fundamental tests of quantum physics, crucially require the interference of multiple single photons in linear-optics circuits. This interference can result in the bunching of photons into higher Fock states, leading to a complex bosonic behaviour. These challenging tasks timely require to develop collective criteria to benchmark many independent initial resources. Here we determine whether n independent imperfect single photons can ultimately bunch into the Fock state $|n\rangle$ . We thereby introduce an experimental Fock-state capability for single-photon sources, which uses phase-space interference for extreme bunching events as a quantifier. In contrast to autocorrelation functions, this operational approach takes into account not only residual multi-photon components but also vacuum admixture and the dispersion of the individual photon statistics. We apply this approach to high-purity single photons generated from an optical parametric oscillator and show that they can lead to a Fock-state capability of at least 14. Our work demonstrates a novel collective benchmark for single-photon sources and their use in subsequent stringent applications.Advanced quantum technologies, as well as fundamental tests of quantum physics, crucially require the interference of multiple single photons in linear-optics circuits. This interference can result in the bunching of photons into higher Fock states, leading to a complex bosonic behaviour. These challenging tasks timely require to develop collective criteria to benchmark many independent initial resources. Here we determine whether n independent imperfect single photons can ultimately bunch into the Fock state $|n\rangle$. We thereby introduce an experimental Fock-state capability for single-photon sources, which uses phase-space interference for extreme bunching events as a quantifier. In contrast to autocorrelation functions, this operational approach takes into account not only residual multi-photon components but also vacuum admixture and the dispersion of the individual photon statistics. We apply this approach to high-purity single photons generated from an optical parametric oscillator and show that they can lead to a Fock-state capability of at least 14. Our work demonstrates a novel collective benchmark for single-photon sources and their use in subsequent stringent applications.

Dec 15, 20201 citation

Realization of photon correlations beyond the linear optics limit

Geobae Park, Issei Matsumoto, Takayuki Kiyohara +3 more

Linear optical transformations of multiple single-photon inputs are fundamental for the development of photonic quantum technologies. Various nonclassical correlations can already be observed directly in states generated using only single-photon inputs and linear optics transformations. However, some quantum correlations require additional operations, and states that exhibit such correlations are classified as non-Fock states. Here, we demonstrate the generation of a two-photon three-mode non-Fock state that exhibits conditional quantum coherences that can only be achieved by non-Fock states. We determine the fidelity of the non-Fock state based on experimentally observed conditional visibilities that characterize the state and compare the result to the fidelity bounds for different classes of Fock and non-Fock states. Our experimental verification of the non-Fock character of the state provides insights into the technological requirements needed to achieve nonclassical correlations in multiphoton quantum optics.Linear optical transformations of multiple single-photon inputs are fundamental for the development of photonic quantum technologies. Various nonclassical correlations can already be observed directly in states generated using only single-photon inputs and linear optics transformations. However, some quantum correlations require additional operations, and states that exhibit such correlations are classified as non-Fock states. Here, we demonstrate the generation of a two-photon three-mode non-Fock state that exhibits conditional quantum coherences that can only be achieved by non-Fock states. We determine the fidelity of the non-Fock state based on experimentally observed conditional visibilities that characterize the state and compare the result to the fidelity bounds for different classes of Fock and non-Fock states. Our experimental verification of the non-Fock character of the state provides insights into the technological requirements needed to achieve nonclassical correlations in multiphoton quantum optics.

Science AdvancesDec 22, 20238 citations

Quantum non-Gaussian high Fock states of light pulses and their superpositions

G. P. Teja, Chandan Kumar, Lukáš Lachman +1 more

The generation of high Fock states of light pulses and their superpositions with provable quantum non-Gaussian features is still very challenging, although the power of conditional methods to herald the approximate state from the available Gaussian states is growing. The atom-light interaction in the high- cavity has been considered a viable alternative to the heralded Fock states of the light pulses from nonlinear optics limited to three-photon Fock states for the last decade. Here, by optimizing the realistic protocol combining it with available optical delay elements, we conclusively predict filtering of Fock states up to ten photons with a high success rate of 20 % using a hierarchy of quantum non-Gaussian criteria. Moreover, the filtering protocol enables the preparation of superposition of Fock states, and we analyze this emerging case up to two photons with provable quantum non-Gaussian coherence and high success rate of 50 % . To demonstrate their quality for applications, we evaluate the robustness of such features, the bunching capability in a linear network, and the sensing capability to estimate the magnitude of unknown force, noise, and phase. These assessments outline the essential conditions and application criteria for realistic optical cavity QED interaction on light pulses to outperform photon detection methods.The generation of high Fock states of light pulses and their superpositions with provable quantum non-Gaussian features is still very challenging, although the power of conditional methods to herald the approximate state from the available Gaussian states is growing. The atom-light interaction in the high- cavity has been considered a viable alternative to the heralded Fock states of the light pulses from nonlinear optics limited to three-photon Fock states for the last decade. Here, by optimizing the realistic protocol combining it with available optical delay elements, we conclusively predict filtering of Fock states up to ten photons with a high success rate of 20 % using a hierarchy of quantum non-Gaussian criteria. Moreover, the filtering protocol enables the preparation of superposition of Fock states, and we analyze this emerging case up to two photons with provable quantum non-Gaussian coherence and high success rate of 50 % . To demonstrate their quality for applications, we evaluate the robustness of such features, the bunching capability in a linear network, and the sensing capability to estimate the magnitude of unknown force, noise, and phase. These assessments outline the essential conditions and application criteria for realistic optical cavity QED interaction on light pulses to outperform photon detection methods.

arXiv:2509.04891Physical Review ResearchSep 4, 20252 citations

Direct observation of photon bunching in thermal light in quantum Fourier transform spectroscopy

Dianwen Zhang

In quantum mechanics, photons are bosons -- there is no restriction on the number of them that occupy the same quantum state, so many of them can bunch together, and this is well known as photon bunching effect. However, photon bunching and multiphoton interference of bunched photons have never been directly observed from a broadband thermal chaotic light source. Nevertheless, it has been known that the interference intensity of a number N of bunched photons oscillates with a wavelength of N times shorter than the wavelength of the constituent single photons, which should be observable in Fourier transform spectroscopy. A quantum Fourier transform spectrometer was made based on a Michelson interferometer and a diffraction spectrometer to observe the photon bunching from multiphoton interference of the bunched photons in thermal light. The results demonstrates 2 to 12 bunched photons were observed simultaneously from thousands of wavelengths in the light of a tungsten halogen lamp. The experiment discloses some interesting properties of the bunched photons. The results will provide new insights for advancing the theories of quantum optics, and the new technology opens the way for new precise measurement of photon bunching and multiphoton interference of bunched photons that are in all kinds of light sources or that are generated with quantum entangled photons.In quantum mechanics, photons are bosons -- there is no restriction on the number of them that occupy the same quantum state, so many of them can bunch together, and this is well known as photon bunching effect. However, photon bunching and multiphoton interference of bunched photons have never been directly observed from a broadband thermal chaotic light source. Nevertheless, it has been known that the interference intensity of a number N of bunched photons oscillates with a wavelength of N times shorter than the wavelength of the constituent single photons, which should be observable in Fourier transform spectroscopy. A quantum Fourier transform spectrometer was made based on a Michelson interferometer and a diffraction spectrometer to observe the photon bunching from multiphoton interference of the bunched photons in thermal light. The results demonstrates 2 to 12 bunched photons were observed simultaneously from thousands of wavelengths in the light of a tungsten halogen lamp. The experiment discloses some interesting properties of the bunched photons. The results will provide new insights for advancing the theories of quantum optics, and the new technology opens the way for new precise measurement of photon bunching and multiphoton interference of bunched photons that are in all kinds of light sources or that are generated with quantum entangled photons.

arXiv:2103.03419Mar 5, 20210 citations

Distillation of continuous variable qudits from single photon sources: A cascaded approach

Devibala Esakkimuthu, Basherrudin Mahmud Ahmed Abduljaffer

Creation of high fidelity photonic quantum states in the continuous variable regime is indispensable for the implementation of quantum technologies universally. However, this is a challenging task as it requires higher nonlinearity or larger Fock states. In this article, we surmount this necessity by using a linear optical setup with a cascaded arrangement of beam splitters that relies solely on single photon sources and single photon detectors to tailor desired single mode nonclassical states. To show the utility of this setup, we demonstrate the generation of displaced higher photon states with unit fidelity and the family of Schrodinger cat states above $98\%$ fidelity. In addition, we manifest the generation of GKP resource states, such as ON states and weak cubic phase states with $99\%$ fidelity. Creating such a variety of important states in this single setup is made feasible by stating the output in the form of displaced qudits. This figure of merit facilitates efficient identification and optimization of input parameters required to generate the target single mode quantum states. We also account for the experimental imperfections by incorporating detector inefficiencies and non-unit single photon sources. This cascaded setup will assist the experimentalists to explore the feasible creation of target states using currently available resources, such as single photon sources and single photon detectors.Creation of high fidelity photonic quantum states in the continuous variable regime is indispensable for the implementation of quantum technologies universally. However, this is a challenging task as it requires higher nonlinearity or larger Fock states. In this article, we surmount this necessity by using a linear optical setup with a cascaded arrangement of beam splitters that relies solely on single photon sources and single photon detectors to tailor desired single mode nonclassical states. To show the utility of this setup, we demonstrate the generation of displaced higher photon states with unit fidelity and the family of Schrodinger cat states above $98\%$ fidelity. In addition, we manifest the generation of GKP resource states, such as ON states and weak cubic phase states with $99\%$ fidelity. Creating such a variety of important states in this single setup is made feasible by stating the output in the form of displaced qudits. This figure of merit facilitates efficient identification and optimization of input parameters required to generate the target single mode quantum states. We also account for the experimental imperfections by incorporating detector inefficiencies and non-unit single photon sources. This cascaded setup will assist the experimentalists to explore the feasible creation of target states using currently available resources, such as single photon sources and single photon detectors.

quant-pharXiv:2512.13264Dec 16, 20250 citations

Super-bunching light with giant high-order correlations and extreme multi-photon events

Chengbing Qin, Yuanyuan Li, Yan, Yu +14 more

Non-classical light sources emitting bundles of N-photons with strong correlation represent versatile resources of interdisciplinary importance with applications ranging from fundamental tests of quantum mechanics to quantum information processing. Yet, high-order correlations, gN(0),quantifying photon correlation, are still limited to hundreds. Here, we report the generation of a super-bunching light source in photonic crystal fiber with g2(0) reaching 5.86*104 and g5(0) up to 2.72*108, through measuring its photon number probability distributions. under giant g2(0) values, the super-bunching light source presents upturned-tail photon distributions and ubiquitous extreme multi-photon events, where 31 photons from a single light pulse at a mean of 1.99*10-4 photons per pulse have been determined. The probability of this extreme event has been enhanced by 10139 folds compared to a coherent laser with Poissonian distribution. By varying the power of the pumping laser, both photon number distributions and corresponding high-order correlations of this light source can be substantially tailored from Poissonian to super-bunching distributions. These phenomena are attributed to the synchronized nonlinear interactions in photonic crystal fibers pumping by bright squeezed light, and the theoretical simulations agree well with the experimental results. Our research showcases the ability to achieve non-classical light sources with giant high-order correlations and extreme multi-photon events, paving the way for high-order correlation imaging, extreme nonlinear optical effects, quantum information processing, and exploring light-matter interactions with multi-photon physics.Non-classical light sources emitting bundles of N-photons with strong correlation represent versatile resources of interdisciplinary importance with applications ranging from fundamental tests of quantum mechanics to quantum information processing. Yet, high-order correlations, gN(0),quantifying photon correlation, are still limited to hundreds. Here, we report the generation of a super-bunching light source in photonic crystal fiber with g2(0) reaching 5.86*104 and g5(0) up to 2.72*108, through measuring its photon number probability distributions. under giant g2(0) values, the super-bunching light source presents upturned-tail photon distributions and ubiquitous extreme multi-photon events, where 31 photons from a single light pulse at a mean of 1.99*10-4 photons per pulse have been determined. The probability of this extreme event has been enhanced by 10139 folds compared to a coherent laser with Poissonian distribution. By varying the power of the pumping laser, both photon number distributions and corresponding high-order correlations of this light source can be substantially tailored from Poissonian to super-bunching distributions. These phenomena are attributed to the synchronized nonlinear interactions in photonic crystal fibers pumping by bright squeezed light, and the theoretical simulations agree well with the experimental results. Our research showcases the ability to achieve non-classical light sources with giant high-order correlations and extreme multi-photon events, paving the way for high-order correlation imaging, extreme nonlinear optical effects, quantum information processing, and exploring light-matter interactions with multi-photon physics.

arXiv:2409.05419Sep 9, 20243 citations

|n\rangle

. We thereby introduce an experimental Fock-state capability for single-photon sources, which uses phase-space interference for extreme bunching events as a quantifier. In contrast to autocorrelation functions, this operational approach takes into account not only residual multi-photon components but also vacuum admixture and the dispersion of the individual photon statistics. We apply this approach to high-purity single photons generated from an optical parametric oscillator and show that they can lead to a Fock-state capability of at least 14. Our work demonstrates a novel collective benchmark for single-photon sources and their use in subsequent stringent applications.

98\%

fidelity. In addition, we manifest the generation of GKP resource states, such as ON states and weak cubic phase states with

99\%

fidelity. Creating such a variety of important states in this single setup is made feasible by stating the output in the form of displaced qudits. This figure of merit facilitates efficient identification and optimization of input parameters required to generate the target single mode quantum states. We also account for the experimental imperfections by incorporating detector inefficiencies and non-unit single photon sources. This cascaded setup will assist the experimentalists to explore the feasible creation of target states using currently available resources, such as single photon sources and single photon detectors.