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Nature Communications

Single-photon test of hyper-complex quantum theories using a metamaterial

Lorenzo M. Procopio, Lee A. Rozema, Zi Jing Wong, Deny R. Hamel, Kevin P. O’Brien, Xiang Zhang, Borivoje Dakić, Philip John Walther

Published Apr 21, 2017• 41 citations
Publisher

Abstract

In standard quantum mechanics, complex numbers are used to describe the wavefunction. Although this has so far proven sufficient to predict experimental results, there is no theoretical reason to choose them over real numbers or generalizations of complex numbers, that is, hyper-complex numbers. Experiments performed to date have proven that real numbers are insufficient, but the need for hyper-complex numbers remains an open question. Here we experimentally probe hyper-complex quantum theories, studying one of their deviations from complex quantum theory: the non-commutativity of phases. We do so by passing single photons through a Sagnac interferometer containing both a metamaterial with a negative refractive index, and a positive phase shifter. To accomplish this we engineered a fishnet metamaterial to have a negative refractive index at 780 nm. We show that the metamaterial phase commutes with other phases with high precision, allowing us to place limits on a particular prediction of hyper-complex quantum theories.

DOI
10.1038/ncomms15044

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In standard quantum mechanics, complex numbers are used to describe the wavefunction. Although this has so far proven sufficient to predict experimental results, there is no theoretical reason to choose them over real numbers or generalizations of complex numbers, that is, hyper-complex numbers. Experiments performed to date have proven that real numbers are insufficient, but the need for hyper-complex numbers remains an open question. Here we experimentally probe hyper-complex quantum theories, studying one of their deviations from complex quantum theory: the non-commutativity of phases. We do so by passing single photons through a Sagnac interferometer containing both a metamaterial with a negative refractive index, and a positive phase shifter. To accomplish this we engineered a fishnet metamaterial to have a negative refractive index at 780 nm. We show that the metamaterial phase commutes with other phases with high precision, allowing us to place limits on a particular prediction of hyper-complex quantum theories.
In standard quantum mechanics, complex numbers are used to describe the wavefunction. Although complex numbers have proven sufficient to predict the results of existing experiments, there is no apparent theoretical reason to choose them over real numbers or generalizations of complex numbers, i.e. hyper-complex numbers. Experiments performed to date have proven that real numbers are insufficient, but whether or not hyper-complex numbers are required remains an open question. Quantum theories based on hyper-complex numbers are one example of a post-quantum theory, which must be put on a firm experimental foundation. Here we experimentally probe hyper-complex quantum theories, by studying one of their deviations from complex quantum theory: the non-commutativity of phases. We do so by passing single photons through a Sagnac interferometer containing two physically different phases, having refractive indices of opposite sign. By showing that the phases commute with high precision, we place limits on a particular prediction of hyper-complex quantum theories.
The axioms of quantum mechanics provide limited information regarding the structure of the Hilbert space, such as the underlying number system. The latter is generally regarded as complex, but generalizations of complex numbers, so-called hypercomplex numbers, cannot be ruled out in theory. Therefore, specialized experiments to test for hypercomplex quantum mechanics are needed. To date, experimental tests are limited to single-particle interference exploiting a closed phase relation in a three-path interferometer called the Peres test. The latter distinguishes complex quantum mechanics from quaternionic quantum mechanics. Here, we propose a general matrix formalism putting the Peres test on a solid mathematical ground. On this basis, we introduce multipath and multiparticle interference tests, which provide a direct probe for any dimension of the number system of quantum mechanics.
Quantum theory is commonly formulated in complex Hilbert spaces. However, the question of whether complex numbers need to be given a fundamental role in the theory has been debated since its pioneering days. Recently it has been shown that tests in the spirit of a Bell inequality can reveal quantum predictions in entanglement swapping scenarios that cannot be modeled by the natural real-number analog of standard quantum theory. Here, we tailor such tests for implementation in state-of-the-art photonic systems. We experimentally demonstrate quantum correlations in a network of three parties and two independent EPR sources that violate the constraints of real quantum theory by over 4.5 standard deviations, hence disproving real quantum theory as a universal physical theory.
Metamaterials have been a major research area for more than two decades now, involving artificial structures with predesigned electromagnetic properties constructed from deep subwavelength building blocks. They have been used to demonstrate a wealth of fascinating phenomena ranging from negative refractive index and epsilon-near-zero to cloaking, emulations of general relativity effects, and super-resolution imaging, to name a few. In the past few years, metamaterials have been suggested as a new platform for quantum optics, and several pioneering experiments have already been carried out with single photons. Here, we employ a dielectric metasurface to generate entanglement between spin and orbital angular momentum of single photons. We demonstrate experimentally the generation of the four Bell states by utilizing the geometric phase arising from the photonic spin-orbit interaction. These are the first experiments with entangled states with metasurfaces, and as such they are paving the way to the new area of quantum metamaterials.
Multiple photon absorption processes typically have a nonlinear dependence on the amplitude of the incident optical field. On the other hand, quantum technologies rely on single photon events. It has therefore been of great technical difficulty to achieve nonlinear devices using single photons. This is due to the small cross-section of absorption in room temperature devices, with multi-photon absorption events occurring with extremely low probability. The lack of access to nonlinear processes severely inhibits the use of optics for a large number of applications surrounding quantum technologies. We demonstrate experimentally that by exploiting a coherent absorption mechanism for N=2 N00N states, outlined theoretically by Jeffers in 2000 [1] and experimentally explored by Roger et. al. in 2016 [2], that it is possible to determine and enhance the number of two photon states that are absorbed. Here a 50% absorbing metasurface is placed inside a Sagnac interferometer into which we inject a N00N state. We show that by tuning the phase φ of the input state, |2,0〉 + exp(-ί2φ) |0,2〉, we can selectively tune the output state. For an input phase of φ = π/2 or 3π/2 we find that a single photon is absorbed with 100% probability. However, when we tune the input phase to φ = 0 or π we see that either 0 or 2 photons are absorbed with equal probability. We have developed a theoretical model that, with no free parameters, fits the experimentally measured two-photon contribution and finds the maximum contribution of |0,0) (0,0| to the output state to be 40.5%.
Standard quantum mechanics has been formulated with complex-valued Schrodinger equations, wave functions, operators, and Hilbert spaces. However, previous work has shown possible to simulate quantum systems using only real numbers by adding extra qubits and exploiting an enlarged Hilbert space. A fundamental question arises: are the complex numbers really necessary for the quantum mechanical description of nature? To answer this question, a non-local game has been developed to reveal a contradiction between a multiqubit quantum experiment and a player using only real numbers. Here, based on deterministic and high-fidelity entanglement swapping with superconducting qubits, we experimentally implement the Bell-like game and observe a quantum score of 8.09(1), which beats the real number bound of 7.66 by 43 standard deviations. Our results disprove the real-number description of nature and establish the indispensable role of complex numbers in quantum mechanics.