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Bulletin of the American Physical Society

Unconventional spin-Peierls state in the quantum magnet TiOBr

J. P. Castellan, J. P. Clancy, Jacob P. C. Ruff, Stephan Rosenkranz, R. Osborn, B. D. Gaulin, F. C. Chou, S. H. -Y. Huang

Published Feb 28, 2012• 0 citations
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In the present work we aim to characterize the lattice configurations and the magnetic behavior in the incommensurate phase of spin-Peierls systems. This phase emerges when the magnetic exchange interaction is coupled to the distortions of an underlying triangular lattice and has its experimental realization in the quasi-one-dimensional compound family TiOXXX (X=ClX=\text{Cl}X=Cl, Br). With a simple model of spin-1/21/21/2 chains inserted in a planar triangular geometry which couples them elastically, we are able to obtain the uniform-incommensurate and incommensurate-dimerized phase transitions seen in these compounds. Moreover, we follow the evolution of the wave vector of the distortions with temperature inside the incommensurate phase. Finally, we predict gapless spin excitations for the intermediate phase of TiOXXX compounds along with incommensurate spin-spin correlations, offering to experimentalists a candidate to observe an exotic Luttinger liquidlike behavior.
A spin-Peierls order emerges in a one-dimensional S=1S=1S=1 Heisenberg antiferromagnetic model with single-ion anisotropy, coupled to finite frequency bond phonons, in a magnetic field. Our results indicate that for the pure Heisenberg model, any Peierls transition is suppressed by quantum fluctuations of the phonon field. However, a magnetic field-induced spin-Peierls order is realized in the presence of strong single-ion anisotropy. Contrary to the standard Peierls state, the periodicity of bond strength modulation in this field-induced spin-Peierls state is variable and depends on the strength of the applied field. The nature of the ground state in this new phase and the associated field-driven transitions to and out of this phase are explored using extensive numerical simulations. In particular, we explore the spin and bond correlations and the evolution of bond order modulation with varying magnetic field.
Field-induced Peierls phase in S=1S=1S=1 Heisenberg spins coupled to quantum phonons
Spin-Peierls transition occurs in a one-dimensional S=1S=1S=1 Heisenberg antiferromagnetic model with single-ion anisotropy, coupled to finite frequency bond phonons, in a magnetic field. Our results indicate that for the pure Heisenberg model, any Peierls transition is suppressed by quantum fluctuations of the phonon field. However, a novel magnetic field-induced Spin-Peierls phase is realized in the presence of strong single-ion anisotropy. Contrary to the standard Peierls state, the periodicity of bond strength modulation in this field-induced Spin-Peierls state is variable and depends on the strength of the applied field. The nature of the ground state in this new phase and the associated field-driven transitions to and out of this phase are explored using extensive numerical simulations. In particular, we explore the spin and bond correlations and the evolution of bond order modulation with varying magnetic field.