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Physical Review Letters

Nonlocalized Generation of Correlated Photon Pairs in Degenerate Down-Conversion

Kayn A. Forbes, Jack Ford, Davıd L. Andrews

Published Mar 30, 2017• 16 citations
Publisher

Abstract

The achievement of optimum conversion efficiency in conventional spontaneous parametric down-conversion requires consideration of quantum processes that entail multisite electrodynamic coupling, actively taking place within the conversion material. The physical mechanism, which operates through virtual photon propagation, provides for photon pairs to be emitted from spatially separated sites of photon interaction; occasionally pairs are produced in which each photon emerges from a different point in space. The extent of such nonlocalized generation is influenced by individual variations in both distance and phase correlation. Mathematical analysis of the global contributions from this mechanism provides a quantitative measure for a degree of positional uncertainty in the origin of down-converted emission.

DOI
10.1103/physrevlett.118.133602

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The achievement of optimum conversion efficiency in conventional spontaneous parametric down-conversion requires consideration of quantum processes that entail multisite electrodynamic coupling, actively taking place within the conversion material. The physical mechanism, which operates through virtual photon propagation, provides for photon pairs to be emitted from spatially separated sites of photon interaction; occasionally pairs are produced in which each photon emerges from a different point in space. The extent of such nonlocalized generation is influenced by individual variations in both distance and phase correlation. Mathematical analysis of the global contributions from this mechanism provides a quantitative measure for a degree of positional uncertainty in the origin of down-converted emission.
The generation of correlated photon pairs is a key to the production of entangled quantum states, which have a variety of applications within the area of quantum information. In spontaneous parametric down-conversion---the primary method of generating correlated photon pairs---the associated photon annihilation and creation events are generally thought of as being colocated: The correlated pair of photons is localized with regards to the pump photon and its positional origin. A detailed quantum electrodynamical analysis highlights a mechanism exhibiting the possibility of a delocalized origin for paired output photons: The spatial extent of the region from which the pair is generated can be much larger than previously thought. The theory of both localized and nonlocalized degenerate down-conversion is presented, followed by a quantitative analysis using discrete-volume computational methods. The results may have significant implications for quantum information and imaging applications, and the design of nonlinear optical metamaterials.
Efficient Generation of Entangled Photon-Pairs The first experiments with correlated photons have been performed in the context of EPR-Bell experiments on the realistic and local properties of quantum mechanics. The source used there produced pairs of polarization entangled photons from a 2-photon decay of Calcium atoms. The technical requirements of these experiments were high (vacuum systems, stronge dye-lasers, etc.) whereas the efficiency of the source was quite low. An important step forward was the introduction of spontaneous parametric down conversion (SPDC), which has become the most common source in quantum optics for generating correlated or entangled photon pairs. In this process photons of an intense pump laser convert to photon pairs in an optical nonlinear crystal. Conservation of energy and momentum leads to strong correlations between the generated photons. With this kind of two-photon source it was possible to realize or improve many experiments on the foundations of quantum mechanics addressing the EPR-Paradoxon and in the new field of quantum information. But again, more advanced experiments and applications suffer from the limited ef- ficiency of the fluorescence process. Many photon pairs are lost by spatial and spectral filtering, which is necessary to achieve polarization entanglement and long coherence times. Different techniques have been implemented to increase the number of photon pairs using two-crystal arrangements, focusing techniques or periodically poled crystals. Most of these methods have the disadvantage that no entangled photons have been observed. It is the aim of this work to increase the yield and to improve the mode definition of entangled photon pairs generated by resonant enhancement of the pump mode and the fluorescence modes. As a first step a linear cavity for the pump mode was realized. Since the conversion probability is proportional to the pump power it was possible to increase the photon pair count rate by factor of 7 over the previous source. Besides the possibility of further improvement on already established pair correlation experiments, such an enhancement allows to build a compact source for photon pairs, in which an expensive argon-ion laser is replaced by a cheap diode laser. Among other applications such sources are of strong interest for quantum cryptography. 3 In many quantum information experiments optical fibers are use to carry the photons over long distance. Therefore, light from the parametric down-conversion source has to be efficiently coupled into fibers. In the second part we report on a new method to optimize collection efficiency by matching the angular distribution of the parametric fluorescence to the spatial mode of an optical fiber. By using this technique, we detected 366500 polarization-entangled photon pairs per second in the near-infrared region in single-mode optical fibers for 465 mW pump power (at 351.1 nm) with a 2 mm BBOcrystal. The entanglement of the photon pairs was verified by measuring polarization correlations of more than 96% in a HV-basis and in a ±45◦-basis. To our knowledge, such enormous count rates of highly entangled photon pairs have not been reached yet with any other technique. In the third part of this thesis we investigated the process of parametric downconversion in a cavity which is resonant to certain longitudinal down-conversion modes only. The idea of placing the parametric down-conversion source inside a cavity is not new. Such a device is usually referred to as a single or double resonant optical parametric oscillator (OPO) and is mainly used to generate squeezed quantum states. In that kind of application the system is operating close to but still under the threshold of oscillation. In our application the situation is quite different. The system is operating far below threshold so that mainly spontaneous emission occurs. In that mode correlations between single photons can still be observed. But bouncing the light back and forth inside the cavity increases the interaction length and hence enhances the signal levels of the down-conversion fields. Further, by resonating two certain modes only, the bandwidth is reduced by orders of magnitude and the coherence time is found to be inverse proportional to the bandwidth. A similar experiment has already been realized with a type-I parametric down-converter in the resonator. We have tried to realize a compact double resonant OPO far below threshold with a type-II parametric down-converter in a high-finesse cavity to realize a bright source of entangled photon pairs with extremely narrow bandwidth.
Metasurfaces are emerging as a promising platform for photon-pair generation through spontaneous parametric down-conversion, thanks to their compactness, integrability, and intrinsic multifunctionality, which enables the engineering of complex quantum states. However, their full potential remains only partially exploited because the physical mechanisms governing key properties of the generated photon pairs, such as generation efficiency and emission directionality, are not yet fully understood. As a result, metasurface designs and experimental configurations are often optimized through trial-and-error procedures. Here, we theoretically investigate the main mechanisms that control photon-pair generation and detection by studying how different pump configurations and measurement geometries affect the generation efficiency, emission directionality, and collection efficiency of the emitted photon pairs. This framework allows us to interpret existing experimental results and to provide general guidelines for the design of metasurfaces and the choice of experimental configurations in future experiments. Finally, we show that substrate thickness and multilayer configurations represent additional degrees of freedom for quantum metasurface design and can be engineered to enhance the generation efficiency and control the emission directionality, providing a new route for the optimization of photon-pair sources based on metasurfaces.
A theory is presented for the quantum state of photon pairs generated from spontaneous parametric down-conversion nonlinear process. In this theory, the influence of the final sizes of nonlinear optical crystals on optical eigenmodes is explicitly taken into consideration. It was found that these photon pairs are not in entangled quantum states. Polarization correlations between the signal beam and the idler beam are explained. It is also shown that the two photons generated from SPDC are not spatially separated, therefore the polarization correlation between the signal and idler beams is not an evidence for quantum non-locality.
Phase singularities are topological defects around which the phase winds by an integer multiple of 2π2π2π. In entangled multiphoton states, they can emerge nonlocally in the joint wavefunction rather than in the field of either subsystem alone. Here we show that the quantum Gouy phase generates nonlocal phase singularities (NPSs) in the two-dimensional longitudinal propagation space of entangled photon pairs. We consider photon pairs produced via spontaneous parametric down-conversion pumped by a Laguerre--Gaussian beam, with the signal and idler photons propagating independently over different longitudinal distances. The accumulated radial-mode-dependent Gouy phases induce destructive interference among biphoton spatial-mode components, producing isolated intensity nulls with quantized phase winding. For a pump with radial mode number ppp, the NPS topological charges have magnitude ppp, whereas their propagation positions and charge signs are governed by the Rayleigh ranges of the pump and phase-matching functions. We further identify the radial-mode structure required for their formation, showing that separable biphoton states cannot support isolated longitudinal NPSs. Our results extend nonlocal singular optics from transverse spatial correlations to longitudinal propagation dynamics and establish propagation distance as a coordinate space for topological structures in entangled photon pairs.