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arXiv:2608.08962 · New Journal of Physics

Quantum Gouy phase singularities in a propagating biphoton state

Takumi Jinushi, Hirokazu Kobayashi

quant-phSubmitted Aug 9, 2026• Announced Aug 11, 2026• 0 citations
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Abstract

Phase singularities are topological defects around which the phase winds by an integer multiple of $2π$. In entangled multiphoton states, they can emerge nonlocally in the joint wavefunction rather than in the field of either subsystem alone. Here we show that the quantum Gouy phase generates nonlocal phase singularities (NPSs) in the two-dimensional longitudinal propagation space of entangled photon pairs. We consider photon pairs produced via spontaneous parametric down-conversion pumped by a Laguerre--Gaussian beam, with the signal and idler photons propagating independently over different longitudinal distances. The accumulated radial-mode-dependent Gouy phases induce destructive interference among biphoton spatial-mode components, producing isolated intensity nulls with quantized phase winding. For a pump with radial mode number $p$, the NPS topological charges have magnitude $p$, whereas their propagation positions and charge signs are governed by the Rayleigh ranges of the pump and phase-matching functions. We further identify the radial-mode structure required for their formation, showing that separable biphoton states cannot support isolated longitudinal NPSs. Our results extend nonlocal singular optics from transverse spatial correlations to longitudinal propagation dynamics and establish propagation distance as a coordinate space for topological structures in entangled photon pairs.

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Phase singularities are topological defects around which the phase winds by an integer multiple of 2π2π2π. In entangled multiphoton states, they can emerge nonlocally in the joint wavefunction rather than in the field of either subsystem alone. Here we show that the quantum Gouy phase generates nonlocal phase singularities (NPSs) in the two-dimensional longitudinal propagation space of entangled photon pairs. We consider photon pairs produced via spontaneous parametric down-conversion pumped by a Laguerre--Gaussian beam, with the signal and idler photons propagating independently over different longitudinal distances. The accumulated radial-mode-dependent Gouy phases induce destructive interference among biphoton spatial-mode components, producing isolated intensity nulls with quantized phase winding. For a pump with radial mode number ppp, the NPS topological charges have magnitude ppp, whereas their propagation positions and charge signs are governed by the Rayleigh ranges of the pump and phase-matching functions. We further identify the radial-mode structure required for their formation, showing that separable biphoton states cannot support isolated longitudinal NPSs. Our results extend nonlocal singular optics from transverse spatial correlations to longitudinal propagation dynamics and establish propagation distance as a coordinate space for topological structures in entangled photon pairs.
In this work, we demonstrate the effect of self-splitting spatial quantum correlations induced by Gouy phase engineering. In the process of spontaneous parametric down conversion the pump beam is structured with a mode superposition that produces a dynamical splitting and recombination of the light beam. This structure is transferred to the quantum correlations between signal and idler photons. As a result the joint two-photon probability distribution propagates like a self-splitting and recombining light beam, implementing a Mach-Zehnder-like interferometer. We observe heralded single-photon interference and two-photon NOON state interference. These results open new avenues for applications in quantum metrology.
High-dimensional entanglement in the form of transverse spatial correlation between a pair of photons generated via spontaneous parametric downconversion is not only a valuable resource in many academic and real-life applications but also provides access to several intriguing quantum phenomena. One such non-intuitive phenomenon is phase entanglement, in which the biphoton state is correlated in the complex phase of its wavefunction. This state, which emerges during the propagation of the biphoton wavefunction, exhibits neither position nor momentum correlation, yet retains full entanglement. In this work, we experimentally explore this state in two distinct ways. The first is by tracking the vanishing spatial photon number correlation over propagation distances lying in [0,∞)\left[0,\infty\right)[0,∞), folded into a finite range using single-lens imaging. These observations show excellent agreement with our theoretical predictions based on the Double Gaussian (DG) approximation of the biphoton state. The second approach involves performing a two-photon interference experiment using a double slit and this state, which reveals the correlated phase front. We show, both theoretically and experimentally, that the observed two-photon interference structure is markedly different from that produced by position-correlated photons, as confirmed by computing the joint probability distribution of photons (JPD) and related metrics. Such interference using phase-entangled light has not been attempted before and opens avenues for advanced experiments and applications in the field of spatial entanglement.
Quantum correlations encoded in photonic Laguerre-Gaussian modes were shown to be related to the Gouy-phase shifts [Kawase et al., Phys. Rev. Lett. 101, 050501 (2008)], allowing for a nondestructive manipulation of photonic quantum states. In this work, we exploit the relation between phase-space correlations of biphotons produced by spontaneously parametric down-conversion (SPDC) as encoded in the logarithmic negativity (LN) and the Gouy phase as they are diffracted through an asymmetrical double-slit setup. Using an analytical approach based on a double-Gaussian approximation for type-I SPDC biphotons, we show that measurements of Gouy-phase differences provide information on their phase-space entanglement variation, governed by the physical parameters of the experiment and expressed by the LN via covariance matrix elements.
Partially coherent quantum-entangled beams combine quantum correlation with partial coherence, allowing them to maintain quantum characteristics while being more resistant to distortions caused by random media during propagation. In this study, we investigate the effect of coherence variation of such beams on non-local double-slit quantum interference. The spatial coherence variation is achieved by controlling the transverse coherence length of the Gaussian Schell model pump in the spontaneous parametric down conversion process. For a fixed beam size, the momentum correlation width of partially coherent biphotons increases with the decrease in the transverse coherence length. This results in a biphoton beam exhibiting multiple spatial modes, making it more suitable for studying the non-local features of quantum states in imaging, interference, and diffraction experiments. Our findings infer both high-quality and near-unity visibility of nonlocal interference using the partially coherent twin beams, even with the substantial decrease in the coherence of the pump. We believe these results can enhance robustness against the deleterious effects of the medium during propagation and can have potential applications in optical image cryptography, biomedical imaging, quantum lithography, and quantum holography.
An advanced wave model is applied to a two-photon interference experiment to show that the observed interference effect is due to the geometrical phase of a two-photon state produced in spontaneous parametric down-conversion. The polarization state of the signal-idler pair is changed adiabatically so that the ``loop'' on the Poincar\'e sphere is opened in the signal channel and closed in the idler channel. Therefore, we observed an essentially nonlocal geometrical phase, shared by the entangled photon pair, or a biphoton.
Spontaneous parametric down-conversion (SPDC) is a widely used source for photonic entanglement. Years of focused research have led to a solid understanding of the process, but a cohesive analytical description of the paraxial biphoton state has yet to be achieved. We derive a general expression for the spatio-temporal biphoton state that applies universally across common experimental settings and correctly describes the nonseparability of spatial and spectral modes. We formulate a criterion on how to decrease the coupling of the spatial from the spectral degree of freedom by taking into account the Gouy phase of interacting beams. This work provides new insights into the role of the Gouy phase in SPDC, and also into the preparation of engineered entangled states for multidimensional quantum information processing.