Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Two-Pulse Coherent Population of Quantum States in Inhomogeneous Ensemble Detected by the Phonon-Assisted Resonant Luminescence

Alexander V. Baranov, V. Davydov, Hong-Da Ren, S. Sugou, Yasuaki Masumoto, Федоров Анатолий Валентинович

Published Jun 23, 2000• 0 citations
OpenAlex

Abstract

The novel technique of coherent control of quantum states in semiconductor nanostructures was applied to the inhomogeneously broadened ensemble of quantum dots. By taking an advantage of the interaction between electronic states in quantum dots and phonons in the host matrix the inhomogeneous broadening was effectively eliminated. The coherence decay rate was measured.

Related papers

Coherent control of optical-phonon-assisted resonance secondary emission in semiconductor quantum dots

Федоров Анатолий Валентинович, Alexander V. Baranov, Yasuaki Masumoto

A new optical effect, the coherent control of spontaneous secondary emission with the participation of optical phonons in systems with discrete spectra of electronic transitions, is studied theoretically. Analytical formulas are obtained that describe the time-integrated signals of secondary emission excited resonantly by a pair of phase-locked pulses in the homogeneously and inhomogeneously broadened systems of semiconductor quantum dots. It is shown that coherent control is a promising method for measuring the total dephasing rates of a resonance optical transition. A physically justified criterion for discriminating between scattering and luminescence in the secondary emission is found. The role of spectral filtering of the signal in the measurements of phase and energy relaxation parameters is elucidated.

Optics and Spectroscopy•Jul 1, 2002•18 citations

Coherent control of thermalized luminescence in semiconductor quantum dots

Федоров Анатолий Валентинович, Alexander V. Baranov, Yasuaki Masumoto

A theoretical study of the time-integrated signal of thermalized luminescence excited by a pair of phase-locked light pulses shows that the idea of coherent control should be efficient for measuring the total dephasing rates of high-energy excitonic transitions. This approach can be used for studying both the homogeneously and inhomogeneously broadened systems, which is highly important in studies of the semiconductor quantum dots. It is found that the method of coherent control makes it possible not only to obtain information about the relaxation constants but also to make conclusions about the statistical properties of frequency distributions of the excitonic transitions responsible for broadening the optical spectra.

Optics and Spectroscopy•Oct 1, 2002•7 citations

Coherent Control of Stress-Induced InGaAs Quantum Dots by Means of Phonon-Assisted Resonant Photoluminescence

Alexander V. Baranov, V. Davydov, Федоров Анатолий Валентинович +3 more

We report the control of coherent status of the lowest energy electronic state of InGaAs/GaAs stress-induced quantum dots in an inhomogeneously broadened system by time-integrated detection of narrow Raman-like lines in resonant photoluminescence spectra. The dephasing time of 18.5 ps has been found at 2K.

physica status solidi (b)•Mar 1, 2001•15 citations

Coherent control of the quasi-elastic resonant secondary emission: Semiconductor quantum dots

Федоров Анатолий Валентинович, Alexander V. Baranov, Yasuaki Masumoto

A detailed theoretical study of the time-integrated signal of spontaneous quasi-elastic secondary emission excited by a pair of phase-locked pulses has shown that coherent control is a promising method for measuring the total dephasing rate of a resonant optical transition. This method may be used to study both the homogeneously and inhomogeneously broadened systems, which is highly important in studies of semiconductor quantum dots. Analysis of components of the secondary emission in the framework of the developed theory has allowed us to find a physically justified criterion for separating the scattering and luminescence signals. The role of spectral filtering of the measured signal in determination of the phase and energy relaxation parameters is elucidated.

Optics and Spectroscopy•May 1, 2002•12 citations

Optical coherent control in semiconductors

John Erland, Vadim G. Lyssenko, J. M. Hvam

Summary form only given. The developments with coherent control (CC) techniques in optical spectroscopy have recently demonstrated population control and coherence manipulations when the induced optical phase is explored with phase-locked laser pulses. These and other developments have been guiding the new research field of quantum control including the recent applications to semiconductors and nanostructures. We study the influence of inhomogeneous broadening in semiconductors on CC results. Photoluminescence (PL) and the coherent emission in four-wave mixing (FWM) is recorded after resonant excitation with phase-locked laser pulses. The sample is a narrow GaAs single quantum well.

Quantum Electronics and Laser Science Conference•Nov 13, 2002•0 citations

Coherent spectroscopy of single quantum dots

John H. Quilter

This thesis presents experiments carried out into the coherent properties of charge carriers confined within a single InGaAs/GaAs quantum dot. Specifically the ground state - single exciton qubit system is controlled with ultrafast optical pulses and then the population of the dot is measured by a high-sensitivity photocurrent detection technique. There are two principal results of these experiments, firstly by modulating the bias applied to the quantum dot diode, the detection efficiency of the photocurrent measurement technique is enhanced. The enhancement is possible as the modulated bias allows fast switching of the voltage-dependent carrier tunneling rates. Secondly, when the transition is addressed by an intense, positively detuned laser, the qubit system can be driven to a population inversion. This occurs due to phonon-assisted relaxation of the optical dressed states of the system. Here, the rapid thermalization due to the exciton-phonon interaction actually enables the population inversion, instead of simply being a source of decoherence.

•Dec 4, 2014•1 citation
The novel technique of coherent control of quantum states in semiconductor nanostructures was applied to the inhomogeneously broadened ensemble of quantum dots. By taking an advantage of the interaction between electronic states in quantum dots and phonons in the host matrix the inhomogeneous broadening was effectively eliminated. The coherence decay rate was measured.
A new optical effect, the coherent control of spontaneous secondary emission with the participation of optical phonons in systems with discrete spectra of electronic transitions, is studied theoretically. Analytical formulas are obtained that describe the time-integrated signals of secondary emission excited resonantly by a pair of phase-locked pulses in the homogeneously and inhomogeneously broadened systems of semiconductor quantum dots. It is shown that coherent control is a promising method for measuring the total dephasing rates of a resonance optical transition. A physically justified criterion for discriminating between scattering and luminescence in the secondary emission is found. The role of spectral filtering of the signal in the measurements of phase and energy relaxation parameters is elucidated.
A theoretical study of the time-integrated signal of thermalized luminescence excited by a pair of phase-locked light pulses shows that the idea of coherent control should be efficient for measuring the total dephasing rates of high-energy excitonic transitions. This approach can be used for studying both the homogeneously and inhomogeneously broadened systems, which is highly important in studies of the semiconductor quantum dots. It is found that the method of coherent control makes it possible not only to obtain information about the relaxation constants but also to make conclusions about the statistical properties of frequency distributions of the excitonic transitions responsible for broadening the optical spectra.
A detailed theoretical study of the time-integrated signal of spontaneous quasi-elastic secondary emission excited by a pair of phase-locked pulses has shown that coherent control is a promising method for measuring the total dephasing rate of a resonant optical transition. This method may be used to study both the homogeneously and inhomogeneously broadened systems, which is highly important in studies of semiconductor quantum dots. Analysis of components of the secondary emission in the framework of the developed theory has allowed us to find a physically justified criterion for separating the scattering and luminescence signals. The role of spectral filtering of the measured signal in determination of the phase and energy relaxation parameters is elucidated.
Summary form only given. The developments with coherent control (CC) techniques in optical spectroscopy have recently demonstrated population control and coherence manipulations when the induced optical phase is explored with phase-locked laser pulses. These and other developments have been guiding the new research field of quantum control including the recent applications to semiconductors and nanostructures. We study the influence of inhomogeneous broadening in semiconductors on CC results. Photoluminescence (PL) and the coherent emission in four-wave mixing (FWM) is recorded after resonant excitation with phase-locked laser pulses. The sample is a narrow GaAs single quantum well.
This thesis presents experiments carried out into the coherent properties of charge carriers confined within a single InGaAs/GaAs quantum dot. Specifically the ground state - single exciton qubit system is controlled with ultrafast optical pulses and then the population of the dot is measured by a high-sensitivity photocurrent detection technique. There are two principal results of these experiments, firstly by modulating the bias applied to the quantum dot diode, the detection efficiency of the photocurrent measurement technique is enhanced. The enhancement is possible as the modulated bias allows fast switching of the voltage-dependent carrier tunneling rates. Secondly, when the transition is addressed by an intense, positively detuned laser, the qubit system can be driven to a population inversion. This occurs due to phonon-assisted relaxation of the optical dressed states of the system. Here, the rapid thermalization due to the exciton-phonon interaction actually enables the population inversion, instead of simply being a source of decoherence.